Search results for " Spectroscopy"

showing 10 items of 6851 documents

Thermally Induced Structural Modification of Silica Nanoparticles Investigated by Raman and Infrared Absorption Spectroscopies

2010

We report an experimental investigation by Raman and infrared (IR) absorption spectroscopies on the structural modifications induced by isochronal thermal treatments on amorphous SiO2 nanoparticles (fumed silica). In particular, three different commercial types of this material, characterized by particle mean diameters of 7, 14, and 40 nm, were subjected to thermal treatments from 100 up to 1000 °C. We found that some properties of fumed silica, such as the SiOSi mean bond angle, ring size distribution, and surface adsorbed water content, are drastically different from those of common bulk silica materials and intimately related to the particles' dimension. The SiOSi mean bond angle, probed…

Core shellSintering effectAnalytical chemistryDehydroxylationSilica nanoparticleSurface shellThermal treatmentTypical valueNanoparticleSinteringFumed silicaThermal treatmentThree-membered ringeducation.field_of_studyWater contentAdsorbed waterRaman lineAtomic networkSilicaThermally inducedSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsSurfaceGeneral EnergysymbolsNetwork structureAbsorption (chemistry)IR measurementMaterials scienceAbsorption spectroscopyStrained structurePopulationInfrared imagingInfrared spectroscopyAbsorptionsymbols.namesakeAdsorptionAbsorption spectroscopyHighly strainedShells (structures)Physical and Theoretical ChemistryeducationFumed silicaNano silica Raman proprieta' strutturaliExperimental investigationParticle mean diameterBond angleStructural modificationSilica materialRaman spectroscopy
researchProduct

Example of a technique for evaluation of interferences caused by complicated sample matrix elements in ICP-AES determination

2001

An example of a useful and rapid procedure for the evaluation of interferences caused by complicated sample matrices in inductively coupled plasma atomic emission spectrometry (ICP-AES) is described. Using simple acid-base standards, all the elements investigated were determined separately in complicated matrices with satisfactory results. Multiple linear regression was used to calculate the linear correction coefficients for each matrix element analyzed. Good analytical results improved still further when this correction method was used.

Correction methodChemistryInductively coupled plasma atomic emission spectroscopyLinear regressionAnalytical chemistryMatrix elementInductively coupled plasmaError detection and correctionInterference (wave propagation)Biological systemBiochemistrySample (graphics)Fresenius' Journal of Analytical Chemistry
researchProduct

Quantitative analysis of mixtures of metal-carbonyl complexes by Fourier-transform infrared spectroscopy: application to the simultaneous double immu…

1996

Abstract The feasibility of a double immunoassay of haptens by the nonisotopic carbonyl metalloimmunoassay (CMIA) method is demonstrated. Three different pairings of antiepileptic medications from the groups carbamazepine, diphenylhydantoin, and phenobarbital (for each of which a mono-CMIA is already available) were assayed by double CMIA. The assay method employs as tracers metal–carbonyl complexes that give very strong signals in the range of 1850–2200 cm −1 in the infrared spectrum, permitting quantitative analysis by Fourier-transform infrared spectroscopy. The fact that the signals are individually assignable and of comparable intensity permits quantitative analysis of mixtures of two …

Correlation coefficientInfraredBiophysicsAnalytical chemistryInfrared spectroscopyMetal carbonylBiochemistryAbsorbanceSpectroscopy Fourier Transform InfraredmedicineOrganometallic CompoundsAnimalsHumansFourier transform infrared spectroscopyMolecular BiologyImmunoassayChromatographymedicine.diagnostic_testMolecular StructureChemistryCell BiologyCarbamazepineEvaluation Studies as TopicImmunoassayPhenobarbitalPhenytoinAnticonvulsantsQuantitative analysis (chemistry)HaptensAnalytical biochemistry
researchProduct

Local structure of A-atom in ABO3 perovskites studies by RMC-EXAFS

2020

The measurements of Sr K-edge XAFS were performed under the approval of Proposal No. 97G042 of Photon Factory (KEK) and partially supported by the Research Grants of Hirosaki University. This work was supported by Bruce Ravel providing data for BTO. Boby Joseph acknowledges IISc Bangalore and ICTP Trieste for financial support through the award of the IISc-ICTP fellowship.

Correlation effectsDiffractionX-ray absorption spectroscopyRadiationMaterials scienceExtended X-ray absorption fine structureAbsorption spectroscopy010308 nuclear & particles physicsReverse Monte CarloExtended X-ray absorption fine structure (EXAFS)01 natural sciencesMolecular physicsSpectral line030218 nuclear medicine & medical imagingCondensed Matter::Materials Science03 medical and health sciences0302 clinical medicine0103 physical sciencesAtom:NATURAL SCIENCES:Physics [Research Subject Categories]PerovskitesReverse Monte CarloSpectroscopyX-ray absorption near edge structure (XANES)Radiation Physics and Chemistry
researchProduct

Nrg1 haploinsufficiency alters inhibitory cortical circuits

2021

Neuregulin 1 (NRG1) and its receptor ERBB4 are schizophrenia (SZ) risk genes that control the development of both excitatory and inhibitory cortical circuits. Most studies focused on the characterization ErbB4 deficient mice. However, ErbB4 deletion concurrently perturbs the signaling of Nrg1 and Neuregulin 3 (Nrg3), another ligand expressed in the cortex. In addition, NRG1 polymorphisms linked to SZ locate mainly in non-coding regions and they may partially reduce Nrg1 expression. Here, to study the relevance of Nrg1 partial loss-of-function in cortical circuits we characterized a recently developed haploinsufficient mouse model of Nrg1 (Nrg1tm1Lex). These mice display SZ-like behavioral d…

Cortical neuronsReceptor ErbB-4Neuregulin-1Gene ExpressionneuronsNeurosciences. Biological psychiatry. NeuropsychiatryHaploinsufficiencyBiologyInhibitory postsynaptic potentialHippocampusMagnetic&nbspMiceInterneuronsNeuregulin 3mental disordersMagnetic resonance spectroscopyAnimalsRNA MessengerneurotransmissionNeuregulin 1GABAergic Neuronsgamma-Aminobutyric AcidInhibitory&nbspCerebral CortexNrg1resonance spectroscopyNeural InhibitionMagnetic Resonance ImagingCortex (botany)Inhibitory neurotransmissionParvalbuminsNeurologyInhibitory Postsynaptic PotentialsCalbindin 2Vesicular Glutamate Transport Protein 1biology.proteinExcitatory postsynaptic potentialSchizophreniaCalretininHaploinsufficiencyCortical&nbspNeuroscienceParvalbuminRC321-571Neurobiology of Disease
researchProduct

Euclid Preparation. XIV. The Complete Calibration of the Color–Redshift Relation (C3R2) Survey: Data Release 3

2021

Stanford, S. A., et al.

Cosmology and Nongalactic Astrophysics (astro-ph.CO)[PHYS.ASTR.IM]Physics [physics]/Astrophysics [astro-ph]/Instrumentation and Methods for Astrophysic [astro-ph.IM]Calibration (statistics)FOS: Physical sciencesAstrophysicsAstrophysics::Cosmology and Extragalactic AstrophysicsColor space217101 natural sciencesCosmologyLarge-scale structure010309 optics[PHYS.ASTR.CO]Physics [physics]/Astrophysics [astro-ph]/Cosmology and Extra-Galactic Astrophysics [astro-ph.CO]galaxy spectroscopySettore FIS/05 - Astronomia e AstrofisicaSpitzer Space Telescope0103 physical sciencesDISTRIBUTIONSAstrophysics::Solar and Stellar AstrophysicsInstrumentation and Methods for Astrophysics (astro-ph.IM)PHOTOMETRIC REDSHIFTS010303 astronomy & astrophysicsWeak gravitational lensingAstrophysics::Galaxy AstrophysicsPhysicsHardware_MEMORYSTRUCTURESAstrophysics::Instrumentation and Methods for AstrophysicsEuclidAstronomy and AstrophysicsRedshiftGalaxyCosmologySpace and Planetary ScienceGalaxy spectroscopyDark energyAstrophysics - Instrumentation and Methods for AstrophysicsAstrophysics - Cosmology and Nongalactic Astrophysics
researchProduct

Theoretical absorption spectrum of the Ar–CO van der Waals complex

2003

The three-dimensional intermolecular electric dipole moment surface of Ar–CO is calculated at the coupled cluster singles and doubles level of theory with the aug-cc-pVTZ basis set extended with a 3s3p2d1f1g set of midbond functions. Using the rovibrational energies and wave functions of our recent study [J. Chem. Phys. 117, 6562 (2002)], temperature-dependent spectral intensities are evaluated and compared to available experimental data. Based on the theoretical spectrum, alternative assignments of the experimentally observed lines in the fundamental band of CO around 2160 and 2166 cm−1 are suggested. Thomas.Bondo@uv.es

Coupled Cluster CalculationsAbsorption spectroscopyGeneral Physics and AstronomySpectral Line IntensitySpectral linesymbols.namesakePhysics and Astronomy (all)Argon ; Carbon Compounds ; Quasimolecules ; Molecular Moments ; Coupled Cluster Calculations ; Rotational-Vibrational States ; Spectral Line Intensity ; SpectraQuasimoleculesPhysics::Atomic and Molecular ClustersArgonPhysics::Chemical PhysicsPhysical and Theoretical Chemistry:FÍSICA::Química física [UNESCO]Rotational-Vibrational StatesBasis setMolecular MomentsChemistryIntermolecular forceRotational–vibrational spectroscopySpectraCarbon CompoundsUNESCO::FÍSICA::Química físicaElectric dipole momentCoupled clusterPhysics::Space Physicssymbolsvan der Waals forceAtomic physics
researchProduct

Importance of Triples Contributions to NMR Spin–Spin Coupling Constants Computed at the CC3 and CCSDT Levels

2016

We present the first analytical implementation of CC3 second derivatives using the spin-unrestricted approach. This allows, for the first time, the calculation of nuclear spin–spin coupling constants (SSCC) relevant to NMR spectroscopy at the CC3 level of theory in a fully analytical manner. CC3 results for the SSCCs of a number of small molecules and their fluorine substituted derivatives are compared with the corresponding coupled cluster singles and doubles (CCSD) results obtained using specialized basis sets. For one-bond couplings the change when going from CCSD to CC3 is typically 1–3%, but much higher corrections were found for 1JCN in FCN, 15.7%, and 1JOF in OF2, 6.4%. The changes v…

Coupling constant010304 chemical physicsBasis (linear algebra)ChemistryNuclear magnetic resonance spectroscopy010402 general chemistry01 natural sciences0104 chemical sciencesComputer Science ApplicationsCoupled cluster0103 physical sciencesPhysical and Theoretical ChemistryAtomic physicsSpin-½Second derivativeJournal of Chemical Theory and Computation
researchProduct

1H and13C NMR spectroscopy of brominated diphenyl ethers. A multiple linear regression analysis

2000

The 1H and 13C NMR chemical shifts and 1H, 1H coupling constants of 27 brominated diphenyl ethers are reported. The increment models for the bromine substituent effects on the 1H and 13C NMR chemical shifts were constructed based on a multiple linear regression analysis. In addition to the single substituent effects, two particle increments and corrective terms for conformational effects are included in these models in order to obtain a reliable prediction of chemical shifts. Copyright © 2000 John Wiley & Sons, Ltd.

Coupling constantBromineChemical shiftSubstituentAnalytical chemistrychemistry.chemical_elementGeneral ChemistryNuclear magnetic resonance spectroscopyCarbon-13 NMRchemistry.chemical_compoundchemistryComputational chemistryProton NMRGeneral Materials ScienceMultiple linear regression analysisMagnetic Resonance in Chemistry
researchProduct

13C NMR spectroscopy of four tertiary methyl norbornenols and norbornanols

1975

Carbon chemical shifts and direct 13C1H coupling constants of 2-endo-methyl-5-norbornen-2-exo-ol, 2-exo-methyl-5-norbornen-2-endo-ol, 2-endo-methylnorbornan-2-exo-ol and 2-exo-methylnorbornan-2-endo-ol have been measured from single samples using a dual probe pulse Fourier transform method.

Coupling constantCarbon-13 NMR satelliteChemistryChemical shiftAnalytical chemistrychemistry.chemical_elementGeneral ChemistryFluorine-19 NMRsymbols.namesakeFourier transform13c nmr spectroscopysymbolsGeneral Materials ScienceTransverse relaxation-optimized spectroscopyCarbonOrganic Magnetic Resonance
researchProduct