Search results for "Cholin"

showing 10 items of 1261 documents

Characterization of Acylating and Deacylating Activities of an Extracellular Phospholipase A2 in a Water-Restricted Environment

1994

The behavior of porcine pancreatic phospholipase A2 (ppPLA2) in monophasic low-water media has been explored, for the first time, in a systematic manner. It has been investigated how a number of variables can modulate both acylating and deacylating activities of the enzyme, and several interesting, unexpected results are presented. Among the most relevant, when placing ppPLA2 in the water-restricted environment, are the following: (i) it displays a remarkable alteration of its specificity toward the substrate polar head relative to all-water medium; (ii) it is quite severely inhibited by lysophosphatidylcholine (LPC), which has important implications, particularly concerning its acylation a…

Hot TemperatureSwineStereochemistryAcylationOleic AcidsBinding CompetitiveBiochemistryPhospholipases ASubstrate SpecificityAcylationchemistry.chemical_compoundPhospholipase A2Enzyme StabilityExtracellularAnimalsPancreasEdetic Acidchemistry.chemical_classificationEsterificationbiologyChemistryHydrolysisLysophosphatidylcholinesWaterSubstrate (chemistry)In vitroKineticsPhospholipases A2LysophosphatidylcholineEnzymeBiochemistryYield (chemistry)Phosphatidylcholinesbiology.proteinCalciumExtracellular SpaceOleic AcidBiochemistry
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New folate-functionalized biocompatible block copolymer micelles as potential anti-cancer drug delivery systems

2006

Abstract The main objective of this study was to synthesize novel folic acid-functionalized diblock copolymer micelles and evaluate their solubilization of two poorly water-soluble anti-tumor drugs, tamoxifen and paclitaxel, which suffer from low water solubility and/or poor hydrolytic stability. The diblock copolymer consisted of a permanently hydrophilic block comprising 2-(methacryloyloxy)ethyl phosphorylcholine (MPC) residues and a pH-sensitive hydrophobic block comprising 2-(diisopropylamino)ethyl methacrylate (DPA) residues. Folic acid (FA) was conjugated to the end of the MPC block so that this group was located on the micelle periphery. Tamoxifen- and paclitaxel-loaded micelles were…

Hydrodynamic radiusAqueous solutionPolymers and PlasticsChemistryOrganic ChemistryMethacrylateMicelleCombinatorial chemistryPolyphosphorylcholineEnd-grouppH-Responsive micelleDynamic light scatteringFolate-functionalizedPolymer chemistryMaterials ChemistryCopolymerDrug carrierPolymer
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Reduction of clozapine-induced hypersalivation by pirenzepine is safe.

2004

Introduction Hypersalivation is known as a frequent, disturbing, and socially stigmatizing side effect of therapy with the atypical antipsychotic clozapine. It has been shown that the addition of the anticholinergic pirenzepine is able to reduce clozapine-induced hypersalivation, probably by blocking M4-receptors. Nevertheless, a pharmacokinetic interaction between both compounds cannot be excluded. Methods In this pilot study, 29 schizophrenic patients (ICD-10; 51.7 % female; age: 36.7 +/- 8.7 years [mean +/- SD]) were included. Serum concentrations of clozapine and its pharmacologically active metabolite N-desmethylclozapine were determined under steady-state conditions by automated HPLC …

HypersalivationAdultMalemedicine.medical_specialtySide effectmedicine.drug_classAtypical antipsychoticPilot ProjectsMuscarinic AntagonistsPharmacologyInternal medicinemedicineAnticholinergicHumansPharmacology (medical)Drug InteractionsClozapineClozapineActive metaboliteChromatography High Pressure LiquidCross-Over StudiesDose-Response Relationship DrugChemistryGeneral MedicinePirenzepineSialorrheaMiddle AgedPirenzepinePsychiatry and Mental healthDose–response relationshipEndocrinologySchizophreniaFemaleSpectrophotometry Ultravioletmedicine.symptommedicine.drugAntipsychotic AgentsPharmacopsychiatry
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Liquid structure and dynamics in the choline acetate:urea 1:2 deep eutectic solvent

2021

We report on the thermodynamic, structural, and dynamic properties of a recently proposed deep eutectic solvent, formed by choline acetate (ChAc) and urea (U) at the stoichiometric ratio 1:2, hereinafter indicated as ChAc:U. Although the crystalline phase melts at 36-38 degrees C depending on the heating rate, ChAc:U can be easily supercooled at sub-ambient conditions, thus maintaining at the liquid state, with a glass-liquid transition at about -50 degrees C. Synchrotron high energy x-ray scattering experiments provide the experimental data for supporting a reverse Monte Carlo analysis to extract structural information at the atomistic level. This exploration of the liquid structure of ChA…

IONIC LIQUIDMONTE-CARLO CHLORIDE SCATTERING WATER NANOSTRUCTURE NANOSCALEsynchrotron radiationeutecticnuclear relaxationX-ray scatteringhydrogen bondingNMRcholine acetatemolecular dynamicsX-rayMOLECULAR-DYNAMICScholinedeep eutectic solvents X-ray scattering synchrotron radiation NMR nuclear relaxation molecular dynamics choline acetateNUCLEAR-MAGNETIC-RESONANCE MOLECULAR-DYNAMICS IONIC LIQUID SFREE ANALYZER MONTE-CARLO CHLORIDE SCATTERING WATER NANOSTRUCTURE NANOSCALESFREE ANALYZERdeep eutectic solvent thermodynamic properties structural properties dynamic propertiesNUCLEAR-MAGNETIC-RESONANCEdeep eutectic solventsSettore CHIM/02 - Chimica Fisica
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Kinetics of the lipoperoxyl radical-scavenging activity of indicaxanthin in solution and unilamellar liposomes

2007

Abstract The reaction of the phytochemical indicaxanthin with lipoperoxyl radicals generated in methyl linoleate methanol solution by 2,20-azobis(2,4-dimethylvaleronitrile), and in aqueous soybean phosphatidylcholine unilamellar liposomes by 2,20-azobis(2- amidinopropane)hydrochloride, was studied. The molecule acts as a chain-terminating lipoperoxyl radical scavenger in solution, with a calculated inhibition constant of 3.63 £ 105M21 s21, and a stoichiometric factor approaching 2. Indicaxanthin incorporated in liposomes prevented lipid oxidation, inducing clear-cut lag periods and decrease of the propagation rate. Both effects were concentration-dependent, but not linearly related to the p…

Indicaxanthin membranes radical scavenger liposomesLipid PeroxidesAntioxidant12-DipalmitoylphosphatidylcholinePyridinesmedicine.medical_treatmentRadicalLipid Bilayersalpha-TocopherolAmidinesContext (language use)In Vitro TechniquesBiochemistryAntioxidantsLipid peroxidationchemistry.chemical_compoundLipid oxidationSuspensionsPhosphatidylcholineNitrilesmedicineOrganic chemistryLiposomeDose-Response Relationship DrugMolecular StructureMethanolDrug SynergismGeneral MedicineFree Radical ScavengersBetaxanthinsSolutionsKineticschemistryLinoleic AcidsLiposomesPhosphatidylcholinesSolventsLipid PeroxidationIndicaxanthinAzo CompoundsOxidation-ReductionNuclear chemistry
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Construction of Spirooxindole Analogues Engrafted with Indole and Pyrazole Scaffolds as Acetylcholinesterase Inhibitors

2021

Twenty-five new hits of spirooxindole analogs 8a–y engrafted with indole and pyrazole scaffolds were designed and constructed via a [3+2]cycloaddition (32CA) reaction starting from three components: new chalcone-based indole and pyrazole scaffolds 5a–d, substituted isatins 6a–c, and secondary amines 7a–d. The potency of the compounds were assessed in modulating cholinesterase (AChE) activity using Ellman’s method. Compounds 8i and 8y showed the strongest acetylcholine esterase inhibition (AChEI) with IC50 values of 24.1 and 27.8 μM, respectively. Molecular docking was used to study their interaction with the active site of hAChE. peerReviewed

Indole testChemistryStereochemistrybioaktiiviset yhdisteetGeneral Chemical EngineeringGeneral ChemistryPyrazoleindolespeptides and proteinsAcetylcholinesterasemolecular mechanicsArticleinhibitionchemistry.chemical_compoundChemistryscaffoldsQD1-999orgaaniset yhdisteetinhibiittorit
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Liver X Receptor Regulates Arachidonic Acid Distribution and Eicosanoid Release in Human Macrophages

2013

Objective— Liver X receptors (LXRs) are oxysterol-activated nuclear receptors that are highly expressed in macrophages and regulate lipid homeostasis and inflammation. Among putative LXR target genes, lysophosphatidylcholine acyltransferase 3 (LPCAT3) involved in the Lands cycle controls the fatty acid composition at the sn-2 position of glycerophospholipids and, therefore, the availability of fatty acids, such as arachidonic acid (AA), used for eicosanoid synthesis. The aim of our study was to determine whether LXRs could regulate the Lands cycle in human macrophages, to assess the consequences in terms of lipid composition and inflammatory response, and to work out the relative contribut…

InflammationBiologySensitivity and SpecificityDinoprostoneMonocyteschemistry.chemical_compoundDownregulation and upregulationmedicineHumansDimethyl SulfoxideRNA MessengerLiver X receptorReceptorCells CulturedLiver X ReceptorsInflammationArachidonic AcidMacrophagesLysophospholipid acyltransferase activity1-Acylglycerophosphocholine O-AcyltransferaseMicroarray AnalysisOrphan Nuclear ReceptorsUp-RegulationchemistryEicosanoidNuclear receptorBiochemistryEicosanoidslipids (amino acids peptides and proteins)Arachidonic acidmedicine.symptomCardiology and Cardiovascular MedicineArteriosclerosis, Thrombosis, and Vascular Biology
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Papaverine enhances the negative inotropic effect of acetylcholine in rat auricles

1978

The negative inotropic effect of acetylcholine in rat left auricles is enhanced in the presence of the phosphodiesterase inhibitor papaverine. This result favours the idea of a cyclic GMP-mediated action of acetylcholine in the heart.

Inotropemedicine.medical_specialtyAction PotentialsIn Vitro TechniquesCellular and Molecular NeurosciencePapaverineInternal medicinemedicineAnimalsHeart AtriaPhosphodiesterase inhibitorCyclic GMPMolecular BiologyPharmacologyPapaverineChemistryPhosphodiesteraseDrug SynergismCell BiologyMyocardial ContractionAcetylcholineRatsEndocrinologyDepression ChemicalMolecular MedicineAcetylcholinemedicine.drugExperientia
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A negative inotropic effect of acetylcholine in the presence of several phosphodiesterase inhibitors.

1981

The phosphodiesterase inhibitors papaverine, theophylline and 3-isobutyl-1-methylxanthine (IBMX) reveal a negative inotropic effect of acetylcholine in cat ventricular heart muscle. This effect in unrelated to beta-adrenoceptor stimulation and possibly mediated by the accumulation of cyclic GMP.

Inotropemedicine.medical_specialtyIBMXPhosphodiesterase InhibitorsStimulationCellular and Molecular Neurosciencechemistry.chemical_compoundCyclic gmpTheophyllineInternal medicine1-Methyl-3-isobutylxanthinePapaverinemedicineAnimalsTheophyllineMolecular BiologyPharmacologyPapaverineDose-Response Relationship DrugPhosphodiesteraseCell BiologyMyocardial ContractionAcetylcholineEndocrinologychemistryDepression ChemicalCatsMolecular MedicineAcetylcholinemedicine.drugExperientia
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Cyclic AMP and cyclic GMP may play opposing roles in influencing force of contraction in mammalian myocardium.

1976

CYCLIC AMP and cyclic GMP have been suggested to play opposing regulatory roles in several biological systems1. Supporting evidence for the yin yang hypothesis of opposing biological regulation has been obtained in sympathetic ganglia2,3 and pyramidal neurones in the rat cerebral cortex4. In the mammalian heart, the role of cyclic AMP in mediating the positive inotropic response to catecholamines was advanced by the observation that the inotropic effect was preceded by an increase in cyclic AMP levels5. On the other hand, the levels of cyclic GMP were found to be increased after cholinergic stimulation6. In frog, oscillations of cyclic AMP7 and cyclic changes in the levels of cyclic AMP and…

Inotropemedicine.medical_specialtyMultidisciplinaryCATSContraction (grammar)ChemistryIn Vitro TechniquesPapillary MusclesMyocardial ContractionMammalian heartRatsCyclic gmpEndocrinologyHeart RateInternal medicinemedicineCatsCyclic AMPCholinergicAnimalsHeart AtriaBiological regulationCyclic GMPNature
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