Search results for "Quantum"

showing 10 items of 9714 documents

Encapsulation of Xenon by a Self-Assembled Fe4L6 Metallosupramolecular Cage

2015

We report (129)Xe NMR experiments showing that a Fe4L6 metallosupramolecular cage can encapsulate xenon in water with a binding constant of 16 M(-1). The observations pave the way for exploiting metallosupramolecular cages as economical means to extract rare gases as well as (129)Xe NMR-based bio-, pH, and temperature sensors. Xe in the Fe4L6 cage has an unusual chemical shift downfield from free Xe in water. The exchange rate between the encapsulated and free Xe was determined to be about 10 Hz, potentially allowing signal amplification via chemical exchange saturation transfer. Computational treatment showed that dynamical effects of Xe motion as well as relativistic effects have signific…

Xenon010405 organic chemistryChemistryChemical exchangechemistry.chemical_elementGeneral Chemistry010402 general chemistry01 natural sciencesBiochemistryBinding constantCatalysis0104 chemical sciencesSelf assembledColloid and Surface ChemistryXenon13. Climate actionComputational chemistrySaturation transferChemical physicsmetallosupramolecular cagesmolecular encapsulationCageRelativistic quantum chemistrySignal amplificationta116Journal of the American Chemical Society
researchProduct

Three-dimensional splitting dynamics of giant vortices in Bose-Einstein condensates

2018

We study the splitting dynamics of giant vortices in dilute Bose-Einstein condensates by numerically integrating the three-dimensional Gross-Pitaevskii equation in time. By taking advantage of tetrahedral tiling in the spatial discretization, we decrease the error and increase the reliability of the numerical method. An extensive survey of vortex splitting symmetries is presented for different aspect ratios of the harmonic trapping potential. The symmetries of the splitting patterns observed in the simulated dynamics are found to be in good agreement with predictions obtained by solving the dominant dynamical instabilities from the corresponding Bogoliubov equations. Furthermore, we observe…

YEE-LIKE SCHEMESDiscretizationGROSS-PITAEVSKII EQUATIONEFFICIENTFOS: Physical sciencesHarmonic (mathematics)GASES114 Physical sciences01 natural sciences010305 fluids & plasmaslaw.inventionsymbols.namesakelaw0103 physical sciencesSUPERFLOW010306 general physicsNUMERICAL-SOLUTIONVORTEXta113PhysicsCondensed Matter::Quantum GasesSTABILITYta114Condensed Matter::OtherNumerical analysisTime evolutionMONOPOLESBose-Einstein condensatesVortexMAXWELLS EQUATIONSGross–Pitaevskii equationClassical mechanicsMaxwell's equationsQuantum Gases (cond-mat.quant-gas)symbolsCondensed Matter - Quantum Gasesvortices in superfluidsBose–Einstein condensate
researchProduct

IV-Curves of tunnel junction arrays at lowered temperature by numerical simulation

1996

We have numerically investigated the effect of lowered T on the performance of the Coulomb blockade thermometer, which has been demostrated to yield primary thermometry in the high T limit where thermal excitations compete with the Coulomb blockade. The thermometer is formed by an array of tunnel junctions whose differentiated IV—curve is used to determine the temperature. The IV—curves were calculated by computer simulations and we have obtained corrections to the analytic high T behaviour due to the lowered temperature.

Yield (engineering)Materials scienceComputer simulationCondensed matter physicsTunnel junctionThermometerThermalGeneral Physics and AstronomyCoulomb blockadeTemperature correctionCondensed Matter::Mesoscopic Systems and Quantum Hall EffectCzechoslovak Journal of Physics
researchProduct

Highly Efficient Holmium-Doped All-Fiber ∼2.07-μm Laser Pumped by Ytterbium-Doped Fiber Laser at ∼1.13 μm

2018

We report a 2.07-μm Holmium-doped all-fiber laser (HDFL) pumped by a 1.13-μm Ytterbium-doped fiber laser (YDFL). Home-made alumino–germano–silicate holmium-doped fiber (HDF) served here as an active medium, optimized in terms of chemical composition and co-dopants’ concentrations. Laser action at 2.07 μm was assessed in simple Fabry–Perot cavity, formed by a couple of home-made fiber Bragg gratings (FBGs), inscribed directly in the HDF; this allowed notable diminishing of intracavity loss of the 2.07-μm laser. HDF was in-core pumped by the 1.13-μm double-clad YDFL with a power of ∼12.5 W, in turn pumped in-clad by a laser diode (LD) operated at 0.97 μm with ∼24.5-W output. Using optimal len…

YtterbiumMaterials sciencechemistry.chemical_element02 engineering and technology01 natural scienceslaw.invention010309 opticsHolmium020210 optoelectronics & photonicsFiber Bragg gratinglawFiber laser0103 physical sciences0202 electrical engineering electronic engineering information engineeringElectrical and Electronic EngineeringLaser diodebusiness.industrySlope efficiencyLaserUNESCO::FÍSICA::Óptica ::Fibras ópticasAtomic and Molecular Physics and Opticschemistry:FÍSICA::Óptica ::Fibras ópticas [UNESCO]OptoelectronicsOptical fiber lasersQuantum efficiencybusinessHolmiumIEEE Journal of Selected Topics in Quantum Electronics
researchProduct

Magnetic exchange interaction in clusters of orbitally degenerate ions. II. Application of the irreducible tensor operator technique

2001

Abstract The irreducible tensor operator technique in R3 group is applied to the problem of kinetic exchange between transition metal ions possessing orbitally degenerate ground states in the local octahedral surrounding. Along with the effective exchange Hamiltonian, the related interactions (low-symmetry crystal field terms, Coulomb interaction between unfilled electronic shells, spin–orbit coupling and Zeeman interaction) are also taken into account within a unified computational scheme. Extension of this approach to high-nuclearity systems consisting of transition metal ions in the orbital triplet ground states is also demonstrated. As illustrative examples, the corner-shared D4h dimers…

Zeeman effectChemistryDegenerate energy levelsGeneral Physics and AstronomyKinetic energyIonsymbols.namesakeMagnetic anisotropysymbolsCoulombPhysical and Theoretical ChemistryAtomic physicsHamiltonian (quantum mechanics)Tensor operatorChemical Physics
researchProduct

SELECTIVE AMPLIFICATION OF NARROW RESONANCE FORMED IN TRANSMISSION SPECTRUM OF Rb NANO-CELL IN MAGNETIC FIELD

2012

Recently it was shown that "λ-Zeeman Technique" (λ-ZT) is a convenient tool to study individual transitions between the Zeeman sublevels of hyperfine levels in an external magnetic field. λ-ZT is based on resonant transmission spectrum of nanometric thin cell (NTC) of thickness L = λ, where λ is the resonant wavelength 794 nm for Rb D1 line. Narrow velocity selective optical pumping (VSOP) resonances in the transmission spectrum of the NTC are split into several components in a magnetic field. Examination of VSOP resonances allows one to identify and investigate an atomic transition in the range of magnetic fields 10 - 5000 G. Here we present a new method for selective addressing of VSOP r…

Zeeman effect[ PHYS.QPHY ] Physics [physics]/Quantum Physics [quant-ph]ChemistryRb atomResonancemagnetic fieldVSOP01 natural sciencesnarrow optical resonanceMagnetic field010309 opticsOptical pumpingWavelengthsymbols.namesake[PHYS.QPHY]Physics [physics]/Quantum Physics [quant-ph]0103 physical sciencessymbolsPhysics::Atomic PhysicsAtomic physics010306 general physicsHyperfine structureLine (formation)nano-metric thin cell
researchProduct

Numerical Evidences of Polarization Switching in PMN Type Relaxor Ferroelectrics

2011

We present a conceptual and computational framework for chemically ordered Pb(Mg 1/3 Nb 2/3 O 3) (PMN) type supercells violating disorder of the host lattice. The effective Hamiltonian is specified by invariance under permutations of supercells and by the dipole-dipole interaction supporting both local nonzero and zero mean polarization of the structure. Statistics treated in canonical ensemble within the mean field approach reveals emergence of polar nanoregions as supported by interplay between the (random) initial state polarization of supercells and their interactions increased at cooling.

Zero meanCanonical ensemblePhysicsCondensed matter physicsCondensed Matter PhysicsPolarization (waves)Electronic Optical and Magnetic MaterialsCondensed Matter::Materials Sciencesymbols.namesakeMean field theoryControl and Systems EngineeringLattice (order)Materials ChemistryCeramics and CompositessymbolsPolarElectrical and Electronic EngineeringHamiltonian (quantum mechanics)Integrated Ferroelectrics
researchProduct

Internally Contracted Multireference Coupled Cluster Calculations with a Spin-Free Dirac-Coulomb Hamiltonian: Application to the Monoxides of Titaniu…

2017

We combine internally contracted multireference coupled cluster theory with a four-component treatment of scalar-relativistic effects based on the spin-free Dirac–Coulomb Hamiltonian. This strategy allows for a rigorous treatment of static and dynamic correlation as well as scalar-relativistic effects, which makes it viable to describe molecules containing heavy transition elements. The use of a spin-free formalism limits the impact of the four-component treatment on the computational cost to the non-rate-determining steps of the calculations. We apply the newly developed method to the lowest singlet and triplet states of the monoxides of titanium, zirconium, and hafnium and show how the in…

Zirconium010304 chemical physicsElectronic correlationComputer Science Applications1707 Computer Vision and Pattern Recognition; Physical and Theoretical Chemistrychemistry.chemical_elementComputer Science Applications1707 Computer Vision and Pattern RecognitionElectronic structure010402 general chemistry01 natural sciences0104 chemical sciencesComputer Science ApplicationsHafniumsymbols.namesakeCoupled clusterchemistry0103 physical sciencessymbolsSinglet statePhysics::Chemical PhysicsAtomic physicsPhysical and Theoretical ChemistryRelativistic quantum chemistryHamiltonian (quantum mechanics)
researchProduct

The dual and the double of a Hopf algebroid are Hopf algebroids

2017

Let $H$ be a $\times$-bialgebra in the sense of Takeuchi. We show that if $H$ is $\times$-Hopf, and if $H$ fulfills the finiteness condition necessary to define its skew dual $H^\vee$, then the coopposite of the latter is $\times$-Hopf as well. If in addition the coopposite $\times$-bialgebra of $H$ is $\times$-Hopf, then the coopposite of the Drinfeld double of $H$ is $\times$-Hopf, as is the Drinfeld double itself, under an additional finiteness condition.

[ MATH ] Mathematics [math]Pure mathematicsGeneral Computer ScienceDuality (optimization)01 natural sciencesTheoretical Computer ScienceMathematics::Category TheoryMathematics::Quantum AlgebraMathematics - Quantum Algebra0103 physical sciencesFOS: Mathematics[MATH.MATH-RA] Mathematics [math]/Rings and Algebras [math.RA]Quantum Algebra (math.QA)[ MATH.MATH-CT ] Mathematics [math]/Category Theory [math.CT]0101 mathematics[MATH]Mathematics [math]Hopf algebroid[MATH.MATH-CT]Mathematics [math]/Category Theory [math.CT]Mathematics[MATH.MATH-QA] Mathematics [math]/Quantum Algebra [math.QA]Algebra and Number TheoryMSC: 16T99 18D10[ MATH.MATH-QA ] Mathematics [math]/Quantum Algebra [math.QA]010308 nuclear & particles physicsbialgebroid[MATH.MATH-RA]Mathematics [math]/Rings and Algebras [math.RA]010102 general mathematicsMathematics::Rings and AlgebrasSkewMathematics - Rings and Algebras[MATH.MATH-CT] Mathematics [math]/Category Theory [math.CT][ MATH.MATH-RA ] Mathematics [math]/Rings and Algebras [math.RA]Dual (category theory)Rings and Algebras (math.RA)Theory of computation[MATH.MATH-QA]Mathematics [math]/Quantum Algebra [math.QA]duality
researchProduct

Categorical action of the extended braid group of affine type $A$

2017

Using a quiver algebra of a cyclic quiver, we construct a faithful categorical action of the extended braid group of affine type A on its bounded homotopy category of finitely generated projective modules. The algebra is trigraded and we identify the trigraded dimensions of the space of morphisms of this category with intersection numbers coming from the topological origin of the group.

[ MATH ] Mathematics [math]Pure mathematicsGeneral MathematicsCategorificationBraid groupGeometric intersection01 natural sciencesMathematics - Geometric TopologyMorphismMathematics::Category TheoryQuiverMathematics - Quantum Algebra0103 physical sciencesFOS: MathematicsQuantum Algebra (math.QA)Representation Theory (math.RT)0101 mathematics[MATH]Mathematics [math]MathematicsHomotopy categoryGroup (mathematics)Applied Mathematics010102 general mathematicsQuiverBraid groupsGeometric Topology (math.GT)16. Peace & justiceCategorificationCategorical actionBounded functionMSC: 20F36 18E30 57M99 13D99010307 mathematical physicsAffine transformationMathematics - Representation Theory
researchProduct