0000000000065130
AUTHOR
G. Savard
High-accuracy mass determination of unstable cesium and barium isotopes
Direct mass measurements of short-lived Cs and Ba isotopes have been performed with the tandem Penning trap mass spectrometer ISOLTRAP installed at the on-line isotope separator ISOLDE at CERN. Typically, a mass resolving power of 600 000 and an accuracy of $\delta \mbox{m} \approx 13$ keV have been obtained. The masses of $^{123,124,126}$Ba and $^{122m}$Cs were measured for the first time. A least-squares adjustment has been performed and the experimental masses are compared with theoretical ones, particularly in the frame of a macroscopic-microscopic model.
The Inchworm as a precision translator in a high magnetic field and UHV environment
Abstract A new set-up has been designed and tested for on-line, high-precision mass measurements of short-lived radioactive isotopes via a determination of the ion cyclotron resonance. Ions delivered by the on-line isotope separator ISOLDE at CERN/Geneva are stored in a Penning trap installed in a superconducting solenoid. Due to severe space limitations in the bore of the solenoid, it is impossible to use conventional mechanical feedthroughs for the necessary manipulations inside the uhv chamber. Instead, a number of Inchworms, a high-precision positioning device based on the piezo-electric effect are employed. This publication reports on the first application of this device in a uhv envir…
High-accuracy mass determination of neutron-rich rubidium and strontiumiIsotopes
The penning-trap mass spectrometer ISOLTRAP, installed at the on-line isotope separator ISOLDE at CERN, has been used to measure atomic masses of $^{88,89,90m,91,92,93,94}$Rb and $^{91- 95}$Sr. Using a resolving power of R $\!\scriptstyle\approx$1 million a mass accuracy of typically 10 keV was achieved for all nuclides. Discrepancies with older data are analyzed and discussed, leading to corrections to those data. Together with the present ISOLTRAP data these corrected data have been used in the general mass adjustment.
Ramsey technique applied in a Penning trap mass spectrometer
Abstract The Ramsey method has been applied in an experiment aiming for accurate mass determination of unstable isotopes. The ion motion in a Penning trap has been excited with time-separated oscillatory fields and Ramsey fringes were observed in the case of dipole and quadrupole excitation. The experimental resonances are in good agreement with theory. Further applications of the technique are discussed.
Mass measurements of very high accuracy by time-of-flight ion cyclotron resonance of ions injected into a penning trap
Abstract The possibility of absolute mass measurements using time-of-flight detection of ion cyclotron resonance on ions injected into a Penning trap has been demonstrated. Resolving powers of 2 million have been achieved, with accuracies of about 0.5 ppm. Absolute accuracy is obtained by direct observation of the sum frequency of the cyclotron and the magnetron motions through the use of an azimuthal quadrupole r.f. field to transform initial magnetron motion into cyclotron motion. Imperfections of the Penning trap leading to systematic errors are discussed. The system has been designed specifically to measure the masses of radionuclides produced at the on-line isotope separator ISOLDE. Wi…
Penning-trap mass measurements of neutron-deficient Rb and Sr isotopes
Abstract The Penning-trap mass spectrometer ISOLTRAP installed at the on-line mass separator ISOLDE 2 at CERN has been used for mass determination of 75–87 Rb and 78–83,87 Sr. Ions are captured in a Penning trap and their cyclotron frequency ω c = ( q m )B in the trapping field B is measured. Ratios of these frequencies lead to the determination of the atomic mass of these isotopes. A resolving power of typically m Δm = 10 6 and an accuracy of δm ≈10 keV is obtained. The mass of 78 Sr is measured for the first time and, in most cases, the mass values of the other isotopes are significantly improved. The experimental masses are compared with theoretical predictions.
High-Accuracy Mass Determination of Unstable Rb, Sr, Cs, Ba, Fr and Ra Isotopes with a Penning Trap Mass Spectrometer
The majority of masses of radioactive isotopes has been measured by determination of Q-values in nuclear reactions or in nuclear decay. For a long time the use of direct mass determination has been limited to stable isotopes or isotopes close to stability. This changed in the 70’s with magnetic spectrometers put on-line to isotope separators. The Orsay group (Audi et al., 1986) succeeded in measuring the masses in long isotope chains of alkali elements. They impressively demonstrated the possibilities embedded in direct mass determination of isotopes far from stability. The persisting demand for more precise masses of short-lived isotopes (or exotic particles) has prompted during recent yea…
Mass Determination of Francium and Radium Isotopes by a Penning Trap Mass Spectrometer
Abstract A tandem Penning trap mass spectrometer is used for mass measurement of radioactive isotopes produced at the on-line isotope separator ISOLDE/CERN. The mass is determined directly and with high accuracy by measuring the cyclotron frequency of the stored ions. Measurements were performed on 209 210 211 212 221 222Fr and 226 230Ra. A resolving power of 5 × 105 was used and an accuracy of 1·8 × 10−7 has been achieved.
Accurate mass determination of short-lived isotopes by a tandem Penning-trap mass spectrometer
A mass spectrometer consisting of two Penning traps has been set up for short-lived isotopes at the on-line mass separator ISOLDE at CERN. The ion beam is collected and cooled in the first trap. After delivery to the second trap, high-accuracy direct mass measurements are made by determining the cyclotron frequency of the stored ions. Measurements have been performed for $^{118}--^{137}$Cs. A resolving power of over ${10}^{6}$ and an accuracy of 1.4\ifmmode\times\else\texttimes\fi{}${10}^{\mathrm{\ensuremath{-}}7}$ have been achieved, corresponding to about 20 keV.
Resolution of nuclear ground and isomeric states by a Penning trap mass spectrometer.
Ground and isomeric states of a nucleus have been resolved for the first time by mass spectrometry. Measurements on $^{78}\mathrm{Rb}^{\mathit{m},}$g and $^{84}\mathrm{Rb}^{\mathit{m},}$g were performed using a tandem Penning trap mass spectrometer on-line with the isotope separator ISOLDE/CERN. The effects of ion-ion interaction were investigated for two ion species differing in mass and stored simultaneously in the trap.
Collection, cooling and delivery of ISOL beams
Abstract The collection of an ISOL beam in a Penning trap using implantation on a surface that is subsequently manipulated so as to become part of an end electrode of a Penning trap and reionization of the implanted material by heat has already been very productive for high-precision nuclear-mass measurements, even though it is limited to elements that are surface ionizable and the collection efficiencies are never better than about 0.1%. More recently, in 1990 a Paul trap system for electric collection of ions was installed at the ISOLDE-3 facility and collection was demonstrated for a 60 kV beam of 132 Xe ions. The purpose of this test setup was to determine the relationship between phase…