0000000000105963
AUTHOR
Andreas Petzold
showing 24 related works from this author
Desert dust aerosol air mass mapping in the western Sahara, using particle properties derived from space-based multi-angle imaging
2009
Coincident observations made over the Moroccan desert during the Sahara mineral dust experiment (SAMUM) 2006 field campaign are used both to validate aerosol amount and type retrieved from multi-angle imaging spectroradiometer (MISR) observations, and to place the suborbital aerosol measurements into the satellite's larger regional context. On three moderately dusty days during which coincident observations were made, MISR mid-visible aerosol optical thickness (AOT) agrees with field measurements point-by-point to within 0.05–0.1. This is about as well as can be expected given spatial sampling differences; the space-based observations capture AOT trends and variability over an extended regi…
Partitioning of Aerosol Particles in Mixed-phase Clouds at a High Alpine Site
2007
6 German Aerospace Centre, D-82234, Wessling, Germany * Now at Institute for Atmospheric and Climate Science, ETH Zurich, 8092 Zurich, Switzerland Abstract The partitioning of aerosol particles between the cloud and the interstitial phase (i.e., unactivated aerosol) has been investigated during several Cloud and Aerosol Characterization Experiments (CLACE) conducted in winter and summer 2004 and winter 2005 at the high alpine research station Jungfraujoch (3,580 m altitude, Switzerland). Ambient air was sampled using different inlets in order to determine the scavenged fraction of aerosol particles, F Scav , and of black carbon, F Scav,BC . They denote the fraction of the aerosol volume con…
Dust mobilization and transport in the northern Sahara during SAMUM 2006 – a meteorological overview
2009
The SAMUM field campaign in southern Morocco in May/June 2006 provides valuable data to study the emission, and the horizontal and vertical transports of mineral dust in the Northern Sahara. Radiosonde and lidar observations show differential advection of air masses with different characteristics during stable nighttime conditions and up to 5-km deep vertical mixing in the strongly convective boundary layer during the day. Lagrangian and synoptic analyses of selected dust periods point to a topographic channel from western Tunisia to central Algeria as a dust source region. Significant emission events are related to cold surges from the Mediterranean in association with eastward passing upp…
State of mixing, shape factor, number size distribution, and hygroscopic growth of the Saharan anthropogenic and mineral dust aerosol at Tinfou, Moro…
2009
The Saharan Mineral Dust Experiment (SAMUM) was conducted in May and June 2006 in Tinfou, Morocco. A H-TDMA system and a H-DMA-APS system were used to obtain hygroscopic properties of mineral dust particles at 85% RH. Dynamic shape factors of 1.11, 1.19 and 1.25 were determined for the volume equivalent diameters 720, 840 and 960 nm, respectively. During a dust event, the hydrophobic number fraction of 250 and 350 nm particles increased significantly from 30 and 65% to 53 and 75%, respectively, indicating that mineral dust particles can be as small as 200 nm in diameter. Log-normal functions for mineral dust number size distributions were obtained from total particle number size distributio…
Saharan dust absorption and refractive index from aircraft-based observations during SAMUM 2006
2009
During the Saharan Mineral Dust Experiment (SAMUM) conducted in summer 2006 in southeast Morocco, the complex refractive index of desert dust was determined from airborne measurements of particle size distributions and aerosol absorption coefficients at three different wavelengths in the blue (467 nm), green (530 nm) and red (660 nm) spectral regions. The vertical structure of the dust layers was analysed by an airborne high spectral resolution lidar (HSRL). The origin of the investigated dust layers was estimated from trajectory analyses, combined with Meteosat 2nd Generation (MSG) scenes and wind field data analyses. The real part n of the dust refractive index was found almost constant w…
General overview: European Integrated project on Aerosol Cloud Climate and Air Quality interactions (EUCAARI)-integrating aerosol research from nano …
2011
In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical properties of aerosol particles over Europe, (b) comprehensive aerosol measurements in four developing countries, (c) a database of airborne measurements of aerosols and clouds over Europe during May 2008, (d) comprehensive modeling tools to study aerosol processes fron nano to global scale and their effects on climate and air quality. In addition a new Pan…
ML-CIRRUS: The Airborne Experiment on Natural Cirrus and Contrail Cirrus with the High-Altitude Long-Range Research Aircraft HALO
2017
Abstract The Midlatitude Cirrus experiment (ML-CIRRUS) deployed the High Altitude and Long Range Research Aircraft (HALO) to obtain new insights into nucleation, life cycle, and climate impact of natural cirrus and aircraft-induced contrail cirrus. Direct observations of cirrus properties and their variability are still incomplete, currently limiting our understanding of the clouds’ impact on climate. Also, dynamical effects on clouds and feedbacks are not adequately represented in today’s weather prediction models. Here, we present the rationale, objectives, and selected scientific highlights of ML-CIRRUS using the G-550 aircraft of the German atmospheric science community. The first combi…
Single particle characterization of black carbon aerosols at a tropospheric alpine site in Switzerland
2010
The refractory black carbon (rBC) mass, size distribution (190–720 nm) and mixing state in sub-micron aerosols were characterized from late February to March 2007 using a single particle incandescence method at the high alpine research station Jungfraujoch (JFJ), Switzerland (46.33° N, 7.59° E, 3580 m a.s.l.). JFJ is a ground based location, which is at times exposed to continental free tropospheric air. A median mass absorption coefficient (MAC) of 10.2&plusmn;3.2 m<sup>2</sup> g<sup>−1</sup> at &lambda;=630 nm was derived by comparing single particle incandescence measurements of black carbon mass with continuous measurements of absorption coefficient. This…
In-situ observations of young contrails – overview and selected results from the CONCERT campaign
2010
Lineshaped contrails were detected with the research aircraft Falcon during the CONCERT – CONtrail and Cirrus ExpeRimenT – campaign in October/November 2008. The Falcon was equipped with a set of instruments to measure the particle size distribution, shape, extinction and chemical composition as well as trace gas mixing ratios of sulfur dioxide (SO<sub>2</sub>), reactive nitrogen and halogen species (NO, NO<sub>y</sub>, HNO<sub>3</sub>, HONO, HCl), ozone (O<sub>3</sub>) and carbon monoxide (CO). During 12 mission flights over Europe, numerous contrails, cirrus clouds and a volcanic aerosol layer were probed at altitudes between 8.5 and 11.6 km…
Regional Saharan dust modelling during the SAMUM 2006 campaign
2011
The regional dust model system LM-MUSCAT-DES was developed in the framework of the SAMUM project. Using the unique comprehensive data set of near-source dust properties during the 2006 SAMUM field campaign, the performance of the model system is evaluated for two time periods in May and June 2006. Dust optical thicknesses, number size distributions and the position of the maximum dust extinction in the vertical profiles agree well with the observations. However, the spatio-temporal evolution of the dust plumes is not always reproduced due to inaccuracies in the dust source placement by the model. While simulated winds and dust distributions are well matched for dust events caused by dry syn…
Evaluation of the MOZAIC Capacitive Hygrometer during the airborne field study CIRRUS-III
2018
The MOZAIC Capacitive Hygrometer (MCH) is usually operated aboard passenger aircraft in the framework of MOZAIC (Measurement of Ozone by Airbus In-Service Aircraft) for measuring atmospheric relative humidity (RH). In order to evaluate the performance of the MCH, the instrument was operated aboard a Learjet 35A research aircraft as part of the CIRRUS-III field study together with a closed-cell Lyman-α fluorescence hygrometer (Fast in situ Stratospheric Hygrometer, or FISH) and an open-path tunable diode laser system (Open-path Jülich Stratospheric TDL ExpeRiment, or OJSTER) for water vapour measurement. After reducing the CIRRUS-III data set to data corresponding to MOZAIC aircraft operatio…
Intercomparison and evaluation of global aerosol microphysical properties among AeroCom models of a range of complexity
2014
Many of the next generation of global climate models will include aerosol schemes which explicitly simulate the microphysical processes that determine the particle size distribution. These models enable aerosol optical properties and cloud condensation nuclei (CCN) concentrations to be determined by fundamental aerosol processes, which should lead to a more physically based simulation of aerosol direct and indirect radiative forcings. This study examines the global variation in particle size distribution simulated by 12 global aerosol microphysics models to quantify model diversity and to identify any common biases against observations. Evaluation against size distribution measurements from…
Upper tropospheric water vapour and its interaction with cirrus clouds as seen from IAGOS long-term routine in-situ observations
2017
IAGOS (In-service Aircraft for a Global Observing System) performs long-term routinein situobservations of atmospheric chemical composition (O3, CO, NOx, NOy, CO2, CH4), water vapour, aerosols, clouds, and temperature on a global scale by operating compact instruments on board of passenger aircraft. The unique characteristics of the IAGOS data set originate from the global scale sampling on air traffic routes with similar instrumentation such that the observations are truly comparable and well suited for atmospheric research on a statistical basis. Here, we present the analysis of 15 months of simultaneous observations of relative humidity with respect to ice (RHice) and ice crystal number …
The evolution of microphysical and optical properties of an A380 contrail in the vortex phase
2012
A contrail from a large-body A380 aircraft at cruise in the humid upper troposphere has been probed with in-situ instruments onboard the DLR research aircraft Falcon. The contrail was sampled during 700 s measurement time at contrail ages of about 1–4 min. The contrail was in the vortex regime during which the primary wake vortices were sinking 270 m below the A380 flight level while the secondary wake remained above. Contrail properties were sampled separately in the primary wake at 90 and 115 s contrail age and nearly continously in the secondary wake at contrail ages from 70 s to 220 s. The scattering phase functions of the contrail particles were measured with a polar nephelometer. The …
Particle chemical properties in the vertical column based on aircraft observations in the vicinity of Cape Verde Islands
2011
During the second Saharan Mineral Dust Experiment (SAMUM-2) field campaign, particles with geometric diameters (d) between ∼0.1 and 25 μm were collected on board of the Deutsches Zentrum für Luft- und Raumfahrt (German Aerospace Center, DLR) Falcon aircraft. Size, chemical composition and mixing state of aerosols sampled (spatially and vertically resolved) along the West African coastline and in the Cape Verde Islands region were determined by electron microscopy. A pronounced layer structure of biomass-burning aerosol and desert dust was present for all days during the sampling period from 23 January to 6 February. The aerosol composition of the small particles (d < 0.5 μm) was highly v…
Ice supersaturated regions: properties and validation of ERA-Interim reanalysis with IAGOS in situ water vapour measurements
2020
Cirrus clouds and their potential formation regions, so-called ice supersaturated regions (ISSRs), with values of relative humidity with respect to ice exceeding 100 %, occur frequently in the tropopause region. It is assumed that ISSRs and cirrus clouds can change the tropopause structure by diabatic processes, driven by latent heating due to phase transition and interaction with radiation. For many research questions, a three-dimensional picture including a sufficient temporal resolution of the water vapour fields in the tropopause region is required. This requirement is fulfilled nowadays by reanalysis products such as the European Centre for Medium-Range Weather Forecasts (ECMWF)…
Airborne survey of trace gases and aerosols over the Southern Baltic Sea: from clean marine boundary layer to shipping corridor effect
2020
The influence of shipping on air quality over the Southern Baltic Sea was investigated by characterizing the horizontal and vertical distribution of aerosols and trace gases using airborne measurements in the summer of 2015. Generally, continental and anthropogenic emissions affected the vertical distribution of atmospheric pollutants, leading to pronounced stratification in and above the marine boundary layer and controlling the aerosol extinction. Marine traffic along the shipping corridor “Kadet Fairway” in the Arkona Basin is shown to influence the presence and properties of both trace gases and aerosol particles in the lowest atmospheric layer. Total particle number concentration and N…
Size distribution, mass concentration, chemical and mineralogical composition and derived optical parameters of the boundary layer aerosol at Tinfou,…
2009
During the SAMUM 2006 field campaign in southern Morocco, physical and chemical properties of desert aerosols were measured. Mass concentrations ranging from 30 Ã�¼g m-3 for PM2.5 under desert background conditions up to 300,000 Ã�¼g m-3 for total suspended particles (TSP) during moderate dust storms were measured. TSP dust concentrations are correlated with the local wind speed, whereas PM10 and PM2.5 concentrations are determined by advection from distant sources. Size distributions were measured for particles between 20 nm and 500 Ã�¼m diameter (parameterizations are given). Two major regimes of the size spectrum can be distinguished. Smaller than 500 nm particle diameter, the distrib…
Aircraft type influence on contrail properties
2013
The investigation of the impact of aircraft parameters on contrail properties helps to better understand the climate impact from aviation. Yet, in observations, it is a challenge to separate aircraft and meteorological influences on contrail formation. During the CONCERT campaign in November 2008, contrails from 3 Airbus passenger aircraft of types A319-111, A340-311 and A380-841 were probed at cruise under similar meteorological conditions with in situ instruments on board DLR research aircraft Falcon. Within the 2 min-old contrails detected near ice saturation, we find similar effective diameters Deff (5.2–5.9 μm), but differences in particle number densities nice (162–235 cm−3) and…
Recent progress in understanding physical and chemical properties of African and Asian mineral dust
2011
International audience; This paper presents a review of recently acquired knowledge on the physico-chemical properties of mineral dust from Africa and Asia based on data presented and discussed during the Third International Dust Workshop, held in Leipzig (Germany) in September 2008. Various regional field experiments have been conducted in the last few years, mostly close to source regions or after short-range transport. Although significant progress has been made in characterising the regional variability of dust properties close to source regions, in particular the mineralogy of iron and the description of particle shape and mixing state, difficulties remain in estimating the range of va…
Extinction and optical depth of contrails
2011
[1] One factor limiting the understanding of the climate impact from contrails and aircraft induced cloud modifications is the accurate determination of their optical depth. To this end, 14 contrails were sampled for 2756 s with instruments onboard the research aircraft Falcon during the CONCERT (CONtrail and Cirrus ExpeRimenT) campaign in November 2008. The young (<10 min old) contrails were produced by 9 commercial aircraft with weights of 47 to 508 t, among them the largest operating passenger aircraft, the Airbus A380. The contrails were observed at temperatures between 214 and 224 K and altitudes between 8.8 and 11.1 km. The measured mean in-contrail relative humidity with respect to i…
Aircraft-based operation of an aerosol mass spectrometer: Measurements of tropospheric aerosol composition
2006
The Aerodyne quadrupole aerosol mass spectrometer was deployed on the Falcon twin jet research aircraft operated by Deutsches Zentrum für Luft- und Raumfahrt (DLR). This was the first deployment of an AMS in a jet aircraft. Aerosol mass concentration measurements in the troposphere up to altitudes of about 11 km were performed within two measurement flights on 12 and 14 May 2003 over southern Germany. Background aerosol data were gained up to 6 km, while aircraft exhaust aerosol was be sampled at higher altitudes on 14 May, indicating the presence of sulfuric acid and unburned hydrocarbons in the exhaust particles. The boundary layer aerosol on 12 May was found to be composed of 49% organic…
Airborne measurements of dust layer properties, particle size distribution and mixing state of Saharan dust during SAMUM 2006
2009
The Saharan Mineral Dust Experiment (SAMUM) was conducted in May/June 2006 in southern Morocco. As part of SAMUM, airborne in situ measurements of the particle size distribution in the diameter range 4 nm < Dp < 100 μm were conducted. The aerosol mixing state was determined below Dp < 2.5 μm. Furthermore, the vertical structure of the dust layers was investigated with a nadir-looking high spectral resolution lidar (HSRL). The desert dust aerosol exhibited two size regimes of different mixing states: below 0.5 μm, the particles had a non-volatile core and a volatile coating; larger particles above 0.5 μm consisted of non-volatile components and contained light absorbing material. In…
Thermodynamic correction of particle concentrations measured by underwing probes on fast-flying aircraft
2016
Particle concentration measurements with underwing probes on aircraft are impacted by air compression upstream of the instrument body as a function of flight velocity. In particular, for fast-flying aircraft the necessity arises to account for compression of the air sample volume. Hence, a correction procedure is needed to invert measured particle number concentrations to ambient conditions that is commonly applicable to different instruments to gain comparable results. In the compression region where the detection of particles occurs (i.e. under factual measurement conditions), pressure and temperature of the air sample are increased compared to ambient (undisturbed) conditions in certain …