0000000000123955

AUTHOR

Thorsten Schumm

showing 8 related works from this author

Internal conversion from excited electronic states of $^{229}{\mathrm Th}$ ions

2016

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of $^{229}{\mathrm Th}$. Due to the very low transition energy, the $^{229}{\mathrm Th}$ nucleus offers the unique possibility to open the otherwise forbidden internal conversion nuclear decay channel for thorium ions via optical laser excitation of the electronic shell. We show that this feature can be exploited to investigate the isomeric state properties via observation of internal conversion from excited electronic configurations of ${\mathrm Th}^+$ and ${\mathrm Th}^{2+}$ ions. A possible experimental realization of the proposed scena…

Nuclear Theory (nucl-th)Nuclear TheoryAtomic Physics (physics.atom-ph)FOS: Physical sciencesNuclear ExperimentPhysics - Atomic Physics
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Internal conversion from excited electronic states of 229Th ions

2017

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of 229Th. Due to the very low transition energy, the 229Th nucleus offers the unique possibility to open the otherwise forbidden internal conversion nuclear decay channel for thorium ions via optical laser excitation of the electronic shell. We show that this feature can be exploited to investigate the isomeric state properties via observation of internal conversion from excited electronic configurations of Th+ and Th2+ ions. A possible experimental realization of the proposed scenario at the nuclear laser spectroscopy facility IGISOL in J…

PhysicsExcited electronic stateIsotopeta114010308 nuclear & particles physicsNuclear stateoptical laser excitationIonic bondingLaserInternal conversion (chemistry)01 natural sciences7. Clean energylaw.inventionIonexcited electronic stateslawExcited stateResearch group A. Pálffy – Division C. H. Keitel0103 physical sciencesAtomic physicsNuclear Experiment010306 general physicsthorium ionsinternal conversionPhysical Review A
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Measurement of the $^{229}$Th isomer energy with a magnetic micro-calorimeter

2020

We present a measurement of the low-energy (0--60$\,$keV) $\gamma$ ray spectrum produced in the $\alpha$-decay of $^{233}$U using a dedicated cryogenic magnetic micro-calorimeter. The energy resolution of $\sim$$10\,$eV, together with exceptional gain linearity, allow us to measure the energy of the low-lying isomeric state in $^{229}$Th using four complementary evaluation schemes. The most accurate scheme determines the $^{229}$Th isomer energy to be $8.10(17)\,$eV, corresponding to 153.1(37)$\,$nm, superseding in precision previous values based on $\gamma$ spectroscopy, and agreeing with a recent measurement based on internal conversion electrons. We also measure branching ratios of the r…

Nuclear Theory (nucl-th)Physics - Instrumentation and DetectorsNuclear TheoryFOS: Physical sciencesInstrumentation and Detectors (physics.ins-det)Nuclear Experiment (nucl-ex)Nuclear Experiment
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Energy of the $^{229}$Th nuclear clock transition

2019

The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary technology and is expected to outperform current electronic-shell based atomic clocks. The development of a nuclear clock was so far impeded by an imprecise knowledge of the energy of the $^{229}$Th nuclear excited state. In this letter we report a direct excitation energy measurement of this elusive state and constrain this to 8.28$\pm$0.17 eV. The energy is determined by spectroscopy of the internal conversion electrons emitted in-flight during the decay of the …

Physics - Instrumentation and DetectorsNuclear TheoryNuclear TheoryFOS: Physical sciencesElectron01 natural scienceslaw.inventionNuclear Theory (nucl-th)Internal conversionlaw0103 physical sciencesNuclear Experiment (nucl-ex)010306 general physicsSpectroscopyNuclear ExperimentPhysicsMultidisciplinary010308 nuclear & particles physicsInstrumentation and Detectors (physics.ins-det)LaserAtomic clockExcited stateResearch group A. Pálffy – Division C. H. Keitelddc:500Atomic physicsEnergy (signal processing)Excitation
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Gas cell studies of thorium using filament dispensers at IGISOL

2020

Abstract Filament-based dispensers of thorium have been investigated at the IGISOL facility, Jyvaskyla, for potential use as a thorium ion source for future collinear laser spectroscopy experiments. Several different filaments were manufactured in the Institute of Atomic and Subatomic Physics of TU Wien, with 232Th and 229Th prepared on tantalum substrates either by drying thorium nitrate solution or via molecular plating, while adding a layer of zirconium for oxide reduction. The filaments were characterized in a helium-filled gas cell by performing selective and efficient in-gas-cell resonance laser ionization and by analyzing the resulting ion beams by mass spectrometry. Additionally, th…

DECOMPOSITIONNuclear and High Energy PhysicsTechnologyEFFICIENCYAnalytical chemistrychemistry.chemical_elementOFF-LINEPhysics Atomic Molecular & ChemicalMass spectrometry01 natural sciencesIonlaw.inventionProtein filamentlawIonization0103 physical sciences010306 general physicsNuclear Science & TechnologyLANTHANIDEInstrumentationInstruments & InstrumentationRESONANCE IONIZATIONScience & TechnologySPECTROSCOPYResonance laser ionization010308 nuclear & particles physicsPhysicsThoriumThoriumLASER ION-SOURCEActinideLaserIon sourceIon sourceWORK-FUNCTIONSPhysics NuclearchemistryACTINIDE ELEMENTSPhysical SciencesGas cellTRANSITION
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Internal conversion from excited electronic states of 229Th ions

2017

The process of internal conversion from excited electronic states is investigated theoretically for the case of the vacuum-ultraviolet nuclear transition of 229 Th . Due to the very low transition energy, the 229 Th nucleus offers the unique possibility to open the otherwise forbidden internal conversion nuclear decay channel for thorium ions via optical laser excitation of the electronic shell. We show that this feature can be exploited to investigate the isomeric state properties via observation of internal conversion from excited electronic configurations of Th + and Th 2 + ions. A possible experimental realization of the proposed scenario at the nuclear laser spectroscopy facility IGISO…

optical laser excitationNuclear Experimentthorium ionsinternal conversionexcited electronic states
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Measurement of the Th229 Isomer Energy with a Magnetic Microcalorimeter

2020

We present a measurement of the low-energy (0-60 keV) γ-ray spectrum produced in the α decay of ^{233}U using a dedicated cryogenic magnetic microcalorimeter. The energy resolution of ∼10  eV, together with exceptional gain linearity, allows us to determine the energy of the low-lying isomeric state in ^{229}Th using four complementary evaluation schemes. The most precise scheme determines the ^{229}Th isomer energy to be 8.10(17) eV, corresponding to 153.1(32) nm, superseding in precision previous values based on γ spectroscopy, and agreeing with a recent measurement based on internal conversion electrons. We also measure branching ratios of the relevant excited states to be b_{29}=9.3(6)%…

PhysicsExcited state0103 physical sciencesGeneral Physics and AstronomyLinearityElectronAtomic physics010306 general physicsSpectroscopy01 natural sciencesNuclear theoryPhysical Review Letters
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Study of the radiative decay of the low-energy isomer in ${}^{229}$Th

2020

Detectors and Experimental Techniques
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