0000000000135569

AUTHOR

G. Neyens

Isomer shift and magnetic moment of the long-lived 1/2$^{+}$ isomer in $^{79}_{30}$Zn$_{49}$: signature of shape coexistence near $^{78}$Ni

Collinear laser spectroscopy has been performed on the $^{79}_{30}$Zn$_{49}$ isotope at ISOLDE-CERN. The existence of a long-lived isomer with a few hundred milliseconds half-life was confirmed, and the nuclear spins and moments of the ground and isomeric states in $^{79}$Zn as well as the isomer shift were measured. From the observed hyperfine structures, spins $I = 9/2$ and $I = 1/2$ are firmly assigned to the ground and isomeric states. The magnetic moment $\mu$ ($^{79}$Zn) = $-$1.1866(10) $\mu_{\rm{N}}$, confirms the spin-parity $9/2^{+}$ with a $\nu g_{9/2}^{-1}$ shell-model configuration, in excellent agreement with the prediction from large scale shell-model theories. The magnetic mo…

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Quadrupole moment of Fr 203

The spectroscopic electric quadrupole moment of the neutron-deficient francium isotope 203Fr was measured by using high-resolution collinear resonance ionization spectroscopy (CRIS) at the CERN Isotope Separation On-Line Device (ISOLDE)facility. A remeasurement of the 207Fr quadrupole momentwas also performed, resulting in a departure from the established literature value. A sudden increase in magnitude of the 203Fr quadrupole moment, with respect to the general trend in the region, points to an onset of static deformation at N =116 in the 87Fr isotopic chain. Calculation of the static and total deformation parameters show that the increase in static deformation only cannot account for the o…

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Dipole and quadrupole moments of $^{73-78}$Cu as a test of the robustness of the $Z=28$ shell closure near $^{78}$Ni

Nuclear spins and precise values of the magnetic dipole and electric quadrupole moments of the ground states of neutron-rich Cu73–78 isotopes were measured using the Collinear Resonance Ionization Spectroscopy (CRIS) experiment at the CERN On-Line Isotope Mass Separator (ISOLDE) facility. The nuclear moments of the less exotic Cu73,75 isotopes were remeasured with similar precision, yielding values that are consistent with earlier measurements. The moments of the odd-odd isotopes, and 2978Cu (N=49) in particular, are used to investigate excitations of the assumed doubly magic Ni78 core through comparisons with large-scale shell-model calculations. Despite the narrowing of the Z=28 shell gap…

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Spins and magnetic moments of 58;60;62;64Mn ground states and isomers

The odd-odd 54;56;58;60;62;64Mn isotopes (Z = 25) were studied using bunched-beam collinear laser spectroscopy at ISOLDE, CERN. From the measured hyperfine spectra the spins and magnetic moments of Mn isotopes up to N = 39 were extracted. The previous tentative ground state spin assignments of 58;60;62;64Mn are now firmly determined to be I = 1 along with an I = 4 assignment for the isomeric states in 58;60;62Mn. The I = 1 magnetic moments show a decreasing trend with increasing neutron number while the I = 4 moments remain quite constant between N = 33 and N = 37. The results are compared to large-scale shell-model calculations using the GXPF1A and LNPS effective interactions. The excellen…

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Nuclear Charge Radius of $^{12}$Be

The nuclear charge radius of $^{12}$Be was precisely determined using the technique of collinear laser spectroscopy on the $2s_{1/2}\rightarrow 2p_{1/2, 3/2}$ transition in the Be$^{+}$ ion. The mean square charge radius increases from $^{10}$Be to $^{12}$Be by $\delta ^{10,12} = 0.69(5) \fm^{2}$ compared to $\delta ^{10,11} = 0.49(5) \fm^{2}$ for the one-neutron halo isotope $^{11}$Be. Calculations in the fermionic molecular dynamics approach show a strong sensitivity of the charge radius to the structure of $^{12}$Be. The experimental charge radius is consistent with a breakdown of the N=8 shell closure.

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Spins and Magnetic Moments of $^{49}$K and $^{51}$K: establishing the 1/2$^+$ and 3/2$^+$ level ordering beyond $N$ = 28

The ground-state spins and magnetic moments of $^{49,51}$K have been measured using bunched-beam high-resolution collinear laser spectroscopy at ISOLDE-CERN. For $^{49}$K a ground-state spin $I = 1/2$ was firmly established. The observed hyperfine structure of $^{51}$K requires a spin $I > 1/2$ and from its magnetic moment $\mu(^{51}\text{K})= +0.5129(22)\, \mu_N$ a spin/parity $I^\pi=3/2^+$ with a dominant $\pi 1d_{3/2}^{-1}$ hole configuration was deduced. This establishes for the first time the re-inversion of the single-particle levels and illustrates the prominent role of the residual monopole interaction for single-particle levels and shell evolution.

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An innovative Superconducting Recoil Separator for HIE-ISOLDE

International audience; The ISOLDE Scientific Infrastructure at CERN offers a unique range of post-accelerated radioactive beams. The scientific program can be improved with the “Isolde Superconducting Recoil Separator” (ISRS), an innovative spectrometer able to deliver unprecedented (A, Z) resolution. In this paper we present an overview of the physics and ongoing technical developments.

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Spectroscopy of short-lived radioactive molecules: A sensitive laboratory for new physics

The study of molecular systems provides exceptional opportunities for the exploration of the fundamental laws of nature and for the search for physics beyond the Standard Model of particle physics. Measurements of molecules composed of naturally occurring nuclei have provided the most stringent upper bounds to the electron electric dipole moment to date, and offer a route to investigate the violation of fundamental symmetries with unprecedented sensitivity. Radioactive molecules - where one or more of their atoms possesses a radioactive nucleus - can contain heavy and deformed nuclei, offering superior sensitivity for EDM measurements as well as for other symmetry-violating effects. Radium …

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Nuclear Moments of Germanium Isotopes around $N$ = 40

Collinear laser spectroscopy measurements were performed on $^{69,71,73}$Ge isotopes ($Z = 32$) at ISOLDE-CERN. The hyperfine structure of the $4s^2 4p^2 \, ^3P_1 \rightarrow 4s^2 4p 5s \, ^3P_1^o$ transition of the germanium atom was probed with laser light of 269 nm, produced by combining the frequency-mixing and frequency-doubling techniques. The hyperfine fields for both atomic levels were calculated using state-of-the-art atomic relativistic Fock-space coupled-cluster calculations. A new $^{73}$Ge quadrupole moment was determined from these calculations and previously measured precision hyperfine parameters, yielding $Q_{\rm s}$ = $-$0.198(4) b, in excellent agreement with the literatu…

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Electromagnetic moments of scandium isotopes and $N=28$ isotones in the distinctive $0f_{7/2}$ orbit

The electric quadrupole moment of $^{49}$Sc was measured by collinear laser spectroscopy at CERN-ISOLDE to be $Q_{\rm s}=-0.159(8)$ $e$b, and a nearly tenfold improvement in precision was reached for the electromagnetic moments of $^{47,49}$Sc. The single-particle behavior and nucleon-nucleon correlations are investigated with the electromagnetic moments of $Z=21$ isotopes and $N=28$ isotones as valence neutrons and protons fill the distinctive $0f_{7/2}$ orbit, respectively, located between magic numbers, 20 and 28. The experimental data are interpreted with shell-model calculations using an effective interaction, and ab-initio valence-space in-medium similarity renormalization group calcu…

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Nuclear mean-square charge radii of $^{63,64,66,68−82}$Ga nuclei: No anomalous behavior at N=32

Collinear laser spectroscopy was performed on the 63,64,66,68−82Ga isotopes with neutron numbers from N = 32 to N = 51. These measurements were carried out at the ISOLDE radioactive ion beam facility at CERN. Here we present the nuclear mean-square charge radii extracted from the isotope shifts and, for the lighter isotopes, new spin and moment values. New ground-state nuclear spin and moments were extracted from the hyperfine spectra of 63,70Ga, measured on an atomic transition in the neutral atom. The ground-state spin of 63Ga is determined to be I = 3/2. Analysis of the trend in the change in mean-square charge radii of the gallium isotopes demonstrates that there is no evidence of anoma…

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Investigating the large deformation of the 5/2(+) isomeric state in Zn-73: An indicator for triaxiality

Recently reported nuclear spins and moments of neutron-rich Zn isotopes measured at ISOLDE-CERN [C. Wraith et al., Phys. Lett. B 771, 385 (2017)PYLBAJ0370-269310.1016/j.physletb.2017.05.085] show an uncommon behavior of the isomeric state in Zn73. Additional details relating to the measurement and analysis of the Zn73m hyperfine structure are addressed here to further support its spin-parity assignment 5/2+ and to estimate its half-life. A systematic investigation of this 5/2+ isomer indicates that significant collectivity appears due to proton/neutron E2 excitations across the proton Z = 28 and neutron N = 50 shell gaps. This is confirmed by the good agreement of the observed quadrupole mo…

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Charge radius of the short-lived $^{68}$Ni and correlation with the dipole polarizability

We present the first laser spectroscopic measurement of the neutron-rich nucleus $^{68}$Ni at the \mbox{$N=40$} subshell closure and extract its nuclear charge radius. Since this is the only short-lived isotope for which the dipole polarizability $\alpha_{\rm D}$ has been measured, the combination of these observables provides a benchmark for nuclear structure theory. We compare them to novel coupled-cluster calculations based on different chiral two- and three-nucleon interactions, for which a strong correlation between the charge radius and dipole polarizability is observed, similar to the stable nucleus $^{48}$Ca. Three-particle--three-hole correlations in coupled-cluster theory substant…

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High-resolution laser spectroscopy of $^{27-32}$Al

Physical review / C 103(1), 014318 (2021). doi:10.1103/PhysRevC.103.014318

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Nuclear moments of indium isotopes reveal abrupt change at magic number 82

In spite of the high-density and strongly correlated nature of the atomic nucleus, experimental and theoretical evidence suggests that around particular 'magic' numbers of nucleons, nuclear properties are governed by a single unpaired nucleon1,2. A microscopic understanding of the extent of this behaviour and its evolution in neutron-rich nuclei remains an open question in nuclear physics3-5. The indium isotopes are considered a textbook example of this phenomenon6, in which the constancy of their electromagnetic properties indicated that a single unpaired proton hole can provide the identity of a complex many-nucleon system6,7. Here we present precision laser spectroscopy measurements perf…

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