0000000000385340
AUTHOR
Jasper Hauer
Observation of an excitonic Mott transition through ultrafast core-cum-conduction photoemission spectroscopy
Time-resolved soft-X-ray photoemission spectroscopy is used to simultaneously measure the ultrafast dynamics of core-level spectral functions and excited states upon excitation of excitons in WSe$_2$. We present a many-body approximation for the Green's function, which excellently describes the transient core-hole spectral function. The relative dynamics of excited-state signal and core levels reveals a delayed core-hole renormalization due to screening by excited quasi-free carriers, revealing an excitonic Mott transition. These findings establish time-resolved core-level photoelectron spectroscopy as a sensitive probe of subtle electronic many-body interactions and an ultrafast electronic…
Time-resolved core-level photoemission data of tungsten diselenide
Pump-probe core-level photoemission spectroscopy data of tungsten diselenide (WSe2) measured using an electron momentum microscope at the FLASH Free-electron laser.