0000000000444905

AUTHOR

Tomoya Yamauchi

Elucidation of the Two-Step Damage Formation Process of Latent Tracks in Poly(allyl diglycol carbonate), PADC: Role of Secondary Low-Energy Electrons

The aim of the present study is to evaluate the mechanisms by which secondary electrons of low energy degrade poly(allyl diglycol carbonate) (PADC) when it is used as a Solid State Nuclear Track De...

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Role of intermediate species in the formation of ion tracks in PADC: A review

Abstract This review paper intends at identifying the early processes arising during the formation of a latent ion track in Poly Allyl Diglycol Carbonate (PADC). We briefly summarize the physical and chemical processes specific to the description of the interaction of ionizing radiation with matter. Then we gather published information in relation to PADC response regarding energy absorption and further transient species formation. Emphasis is given to the chemistry of radicals. Due to a lack of available data in relation with clearly identified unpaired electron carriers in PADC, we use data stemming from surrogate molecules. Based on such data we suggest mechanisms for the decomposition o…

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Evidence for a critical dose above which damage to carbonate ester bonds in PADC appear after gamma ray and ultra soft X-ray exposures

Abstract It has been confirmed that the density of carbonate ester in poly(allyl diglycol carbonate) (PADC), which is a well-known polymeric nuclear track detector CR-39, begins decreasing above a critical dose of about 60 kGy during exposures to Co-60 gamma rays and Ultra Soft X-rays (USX: Kα (Al) with energy 1.49 keV). After exposure to Co-60 gamma rays at 77 K and room temperature (RT), a significant difference in Electron Spin Resonance (ESR) spectra has been observed at both sides of a critical dose of 60 kGy, where is a threshold for the degradation of carbonate ester in PADC. Namely, the types of free radicals in PADC are different from each other below and above this critical dose. …

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Radial electron fluence around ion tracks as a new physical parameter for the detection threshold of PADC using Geant4-DNA toolkit

International audience; The detection threshold of poly(allyl dyglycol carbonate), PADC, for C ions is determined as 55 eV/nm in stopping power, which is significantly higher than that for proton and He ions. The stopping power is not a universal parameter for expressing the detection threshold of PADC. A new physical parameter of Radial Electron Fluence around Ion Tracks, REFIT, is proposed to describe the detection threshold of PADC. It is defined as the number density of electrons passing through the surface of a cylinder of a certain radius that is co-axial with the trajectory. Furthermore, preliminary calculations are presently being performed using the Monte Carlo simulation code of G…

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