0000000000478078
AUTHOR
K. Rytkönen
showing 22 related works from this author
Total absorption γ -ray spectroscopy of niobium isomers
2019
15 pags. 17 figs., 5 tabs.
Total absorption studies of high priority decays for reactor applications: 86Br and 91Rb
2017
Preliminary results from beta decay studies of nuclei that are important for reactor applications are presented. The beta decays have been studied using the total absorption technique (TAS) and the pure beams provided by the JYFLTRAP system at the IGISOL facility of the University of Jyväskylä. peerReviewed
Metallic evolution of small magnesium clusters
2001
Structural and electronic properties of small magnesium clusters (N≤13) are studied using a first-principles simulation method in conjunction with the density functional theory and generalized gradient correction approximation for the exchange-correlation energy functional. It is observed that the onset of metallization of magnesium clusters is hard to assign since both the s-p hybridization and the energy gap between the valence and conduction bands do not evolve rapidly towards the known bulk properties. Instead these quantities show a slow and nonmonotonic evolution.
Total absorption γ -ray spectroscopy of the β -delayed neutron emitters I137 and Rb95
2019
The decays of the β-delayed neutron emitters I137 and Rb95 have been studied with the total absorption γ-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyvaskyla allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption γ-ray spectrometer, a segmented detector composed of 18 NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt γ rays and delayed neutron interactions to eliminate this source of contamination. Due to the s…
Determination of β -decay ground state feeding of nuclei of importance for reactor applications
2020
12 pags., 6 figs., 3 tabs.
Strong γ-ray emission from neutron unbound states populated in β-decay: Impact on (n,γ) cross-section estimates
2017
J. L. Taín et al. -- 6 pags., 7 figs., 1 tab. -- Open Access funded by Creative Commons Atribution Licence 4.0
Electronic properties of single-walled carbon nanotubes inside cyclic supermolecules
2006
Possible ways for manipulating carbon nanotubes (CNTs) with cyclic supermolecules are studied using density functional theory. Electronic structure calculations with structure optimizations have been performed for the (4,4) and (8,0) single-walled carbon nanotubes (SWNTs) complexed with crown ethers as well as for the (4,0) SWNT with beta-cyclodextrin. A slight polarization of charge in both the nanotube and the supermolecule is observed upon rotaxane complexation, but the interaction is mainly repulsive, and the systems stay 2.8-3.5 A apart. The supermolecule does not affect the electronic band structure of the nanotube significantly within such a configuration. The situation differs notic…
Results of DTAS Campaign at IGISOL : Overview
2023
The β decays of more than twenty fission fragments were measured in the first experiments with radioactive-ion beams employing the Decay Total Absorption γ-ray Spectrometer. In this work, we summarize the main results obtained so far from this experimental campaign carried out at the Ion Guide Isotope Separator On-Line facility. The advances introduced for these studies represent the state-of-the-art of our analysis methodology for segmented spectrometers. peerReviewed
Sodium atoms and clusters on graphite by density functional theory
2004
Sodium atoms and clusters $(Nl~5)$ on graphite (0001) are studied using density functional theory, pseudopotentials and periodic boundary conditions. A single Na atom is observed to bind at a hollow site 2.45 \AA{} above the surface with an adsorption energy of 0.51 eV. The small diffusion barrier of 0.06 eV indicates a flat potential energy surface. Increased Na coverage results in a weak adsorbate-substrate interaction, which is evident in the larger separation from the surface in the cases of ${\mathrm{Na}}_{3},$ ${\mathrm{Na}}_{4},$ ${\mathrm{Na}}_{5},$ and the $(2\ifmmode\times\else\texttimes\fi{}2)$ Na overlayer. The binding is weak for ${\mathrm{Na}}_{2},$ which has a full valence el…
Density functional study of alkali-metal atoms and monolayers on graphite (0001)
2007
Alkali metal atoms (Li, Na, K, Rb, Cs), dimers and (2$\times$2) monolayers on a graphite (0001) surface have been studied using density functional theory, pseudopotentials, and a periodic substrate. The adatoms bind at the hollow site (graphite hexagon), with Li lying closest to (1.84 ��) and Cs farthest (3.75 ��) from the surface. The adsorption energies range between $0.55-1.21$ eV, and the energy ordering of the alkali adatoms is Li$>$Cs$\ge$Rb$\ge$K$>$Na. The small diffusion barriers (0.02-0.21 eV for the C-C bridge) decrease as the atom size increases, indicating a flat potential energy surface. The formation (cohesion) energies of (2$\times$2) monolayers range between 0.55-0.81 …
Summation Calculations for Reactor Antineutrino Spectra, Decay Heat and Delayed Neutron Fractions Involving New TAGS Data and Evaluated Databases
2018
9 pags., 3 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Characterization and performance of the DTAS detector
2018
11 pags., 16 figs., 3 tabs.
First experiment with the NUSTAR/FAIR Decay Total Absorption γ-Ray Spectrometer (DTAS) at the IGISOL IV facility
2015
V. Guadilla et al. ; 4 págs.; 4 figs.; 1 tab.
Characterization of a cylindrical plastic {\beta}-detector with Monte Carlo simulations of optical photons
2017
V. Guadilla et al. -- 5 pags., 8 figs., tab.
Large Impact of the Decay of Niobium Isomers on the Reactor ν¯e Summation Calculations
2019
Even mass neutron-rich niobium isotopes are among the principal contributors to the reactor antineutrino energy spectrum. They are also among the most challenging to measure due to the refractory nature of niobium, and because they exhibit isomeric states lying very close in energy. The beta-intensity distributions of Nb-100gs,Nb-100m and Nb-102gs,Nb-02m beta decays have been determined using the total absorption.-ray spectroscopy technique. The measurements were performed at the upgraded Ion Guide Isotope Separator On-Line facility at the University of Jyvaskyla. Here, the double Penning trap system JYFLTRAP was employed to disentangle the beta decay of the isomeric states. The new data ob…
TAGS measurements of $^{100}$Nb ground and isomeric states and $^{140}$Cs for neutrino physics with the new DTAS detector
2016
V. Guadilla et al. -- 4 pags., 6 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
Disentangling decaying isomers and searching for signatures of collective excitations in β decay
2019
6 pags., 3 figs., 1 tab. -- 27th International Nuclear Physics Conference (INPC2019) 29 July - 2 August 2019, Glasgow, UK
Experimental study of $^{100}$Tc $\beta$ decay with total absorption $\gamma$-ray spectroscopy
2017
International audience; The β decay of Tc100 has been studied by using the total absorption γ-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. In this work the new Decay Total Absorption γ-ray Spectrometer in coincidence with a cylindrical plastic β detector has been employed. The β intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first-excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random-phase approximatio…
Total absorption γ-ray spectroscopy of the β decays of 96gs,mY
2022
The β decays of the ground state (gs) and isomeric state (m) of 96Y have been studied with the total absorption γ-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8+ isomeric state from the 0− ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The β-intensity distributions of both decays have been independently determined. In the analyses the deexcitation of the 1581.6 keV level in 96Zr, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the β-detector efficiency, influencing the β-intensity di…
Determination of β-decay ground state feeding of nuclei of importance for reactor applications
2020
In β-decay studies the determination of the decay probability to the ground state (g.s.) of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed γ-ray emission. In this work we revisit the 4πγ−β method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the β-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large g.s. branches. The method is…
Study of the $\beta$-decay of $^{100}$Tc with Total Absorption $\gamma$-Ray Spectroscopy
2017
The \b{eta}-decay of 100 Tc has been studied using the Total Absorption {\gamma}-Ray Spectroscopy technique at IGISOL. In this work the new DTAS spectrometer in coincidence with a cylindrical plastic \b{eta} detector has been employed. The \b{eta}-intensity to the ground state obtained from the analysis is in good agreement with previous high-resolution measurements. However, differences in the feeding to the first excited state as well as weak feeding to a new level at high excitation energy have been deduced from this experiment. Theoretical calculations performed in the quasiparticle random- phase approximation (QRPA) framework are also reported. Comparison of these calculations with our…
Total absorption γ-ray spectroscopy of the β-delayed neutron emitters 137I and 95Rb
2019
The decays of the β-delayed neutron emitters 137I and 95Rb have been studied with the total absorption γ-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyväskylä allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption γ-ray spectrometer, a segmented detector composed of 18 NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt γ rays and delayed neutron interactions to eliminate this source of contamination. Due to the s…