0000000000588417

AUTHOR

Youness El Bakri

Growth, single crystal investigation, hirshfeld surface analysis, DFT studies, molecular docking, physico-chemical characterization and, in vitro, antioxidant activity of a novel hybrid complex

Abstract Interaction of the diphosphoric acid (H4P2O7) and organic ligand (3.4-dimethylaniline) with transition metal ions, cobalt (II) chloride leads to the formation of novel stable Co(II)-diphosphate cluster with empirical formula (C8H12N)2[Co(H2P2O7)2(H2O)2].2H2O. The structure of the synthesized material was confirmed by single crystal XRD at 120 ​K. The crystal was plate and crystallized in the triclinic P 1 ¯ space group with a ​= ​7.5340(4) A, b ​= ​7.5445(4) A, c ​= ​13.6896(8) A, α ​= ​84.215(5)°, β ​= ​76.038(5)°, γ ​= ​74.284(5)°, V ​= ​726.38(7) A3 and Z ​= ​1. Full-matrix least-squares refinement converged at R ​= ​0.035 and Rw ​= ​0.088 for 3636 independent observed reflectio…

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Self-assembly of new cobalt complexes based on [Co(SCN)4], synthesis, empirical, antioxidant activity, and quantum theory investigations

The cobalt (II) complexes have been synthesized from the reaction of the cationic entities (3,4-dimethylaniline (1) and histamine (2)) with metallic salt CoCl2⋅6H2O and thiocyanate ion (SCN−) as a ligand in H2O/ethanolic solution and processing by the evaporation crystal growth method at room temperature to get crystals. The synthesized complex has been fully characterized by single-crystal X-ray diffraction. UV–Visible, FTIR spectroscopy, TGA analysis, and DFT circulations were also performed. The crystal structural analysis reveals that the solid (1) {[Co(SCN)4] (C8H12N)3}·Cl crystallizes in the monoclinic system with the space group P21/n and the solid (2) {[Co(SCN)4](C5H11N3)2}·2Cl crys…

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CCDC 2059295: Experimental Crystal Structure Determination

Related Article: Yathreb Oueslati, Youness El Bakri, Arto Valkonen, Carlos J. Gómez García, El Hassane Anouar, Wajda Smirani|2021|J.Solid State Chem.|301|122319|doi:10.1016/j.jssc.2021.122319

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