0000000000625385

AUTHOR

Zilong Wang

showing 2 related works from this author

Intravalley spin-flip relaxation dynamics in single-layer WS2

2019

Two-dimensional Transition Metal Dichalcogenides (TMDs) have been widely studied because of the peculiar electronic band structure and the strong excitonic effects [1]. In these materials the large spin-orbit coupling lifts the spin degeneracy of the valence (VB) and the conduction band (CB) giving rise to the A and B interband excitonic transitions. In monolayer WS2, the spins of electrons in the lowest CB and in the highest VB at K/K' point of the Brillouin zone are antiparallel resulting in an intravalley dark exciton state at a lower energy than the bright exciton, see left panel of Fig.1. On the one hand, the presence of dark excitons has been revealed indirectly from the observation o…

PhysicsValence (chemistry)Condensed matter physicsSpinsScatteringExciton02 engineering and technologyElectronCondensed Matter::Mesoscopic Systems and Quantum Hall Effect021001 nanoscience & nanotechnology01 natural sciencesBrillouin zoneCondensed Matter::Materials Science0103 physical sciencesSpin-flip010306 general physics0210 nano-technologyElectronic band structure
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Real-time observation of the intravalley spin-flip process in single-layer WS2

2019

We use helicity-resolved transient absorption spectroscopy to track intravalley scattering dynamics in monolayer WS2. We find that spin-polarized carriers scatter from upper to lower conduction band by reversing their spin orientation on a sub-ps timescale.

Materials scienceCondensed matter physicsScatteringPhysicsQC1-999MonolayerUltrafast laser spectroscopySettore FIS/01 - Fisica SperimentaleProcess (computing)ReversingSpin-flipSpectroscopySpin-½
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