0000000000638077
AUTHOR
T. Clauss
showing 3 related works from this author
Irreversible loss of ice nucleation active sites in mineral dust particles caused by sulphuric acid condensation
2010
Abstract. During the FROST-2 (FReezing Of duST) measurement campaign conducted at the Leipzig Aerosol Cloud Interaction Simulator (LACIS), we investigated changes in the ice nucleation properties of 300 nm Arizona Test Dust mineral particles following thermochemical processing by varying amounts and combinations of exposure to sulphuric acid vapour, ammonia gas, water vapour, and heat. The processed particles' heterogeneous ice nucleation properties were determined in both the water subsaturated and supersaturated humidity regimes at −30 °C and −25 °C using Colorado State University's continuous flow diffusion chamber. The amount of sulphuric acid coating material was estimated by an aeroso…
Corrigendum to "Experimental study of the role of physicochemical surface processing on the IN ability of mineral dust particles" published in Atmos.…
2011
Atmospheric Chemistry and Physics, 11 (22)
Surface modification of mineral dust particles by sulphuric acid processing: implications for CCN and IN abilities
2011
Abstract. The ability of coated mineral dust particles to act as cloud condensation nuclei (CCN) and ice nuclei (IN) was investigated at LACIS (Leipzig Aerosol Cloud Interaction Simulator) during the FROST1- and FROST2-campaigns (Freezing of dust). Sulphuric acid was condensed on the particles which afterwards were optionally humidified, treated with ammonia vapour and/or heat. By means of aerosol mass spectrometry we found evidence that processing of mineral dust particles with sulphuric acid leads to surface modifications of the particles. These surface modifications are responsible for the observed reduction of the IN activation of the particles. The observed particle mass spectra sugges…