Enhanced Quadrupole and Octupole Strength in Doubly Magic ^{132}Sn.

International audience; The first $2^+$ and $3^-$ states of the doubly magic nucleus $^{132}$Sn are populated via safe Coulomb excitation employing the recently commissioned HIE-ISOLDE accelerator at CERN in conjunction with the highly efficient MINIBALL array. The $^{132}$Sn ions are accelerated to an energy of 5.49  MeV/nucleon and impinged on a $^{206}$Pb target. Deexciting $\gamma$ rays from the low-lying excited states of the target and the projectile are recorded in coincidence with scattered particles. The reduced transition strengths are determined for the transitions $0_{g.s.}^+ \rightarrow 2_1^+$, $0_{g.s.}^+ \rightarrow 3_1^-$, and $2_1^+ \rightarrow 3_1^-$ in $^{132}$Sn. The res…

Shape coexistence in Hg-178

Lifetime measurements of excited states in Hg-178 have been performed using the Rh-103(Kr-78, p2n) reaction at a beam energy of 354 MeV. The recoil-decay tagging (RDT) technique was applied to select the Hg-178 nuclei and associate the prompt gamma rays with the correlated characteristic ground-state alpha decay. Lifetimes of the four lowest yrast states of Hg-178 have been determined using the recoil distance Doppler-shift (RDDS) method. The experimental data are compared to theoretical predictions with focus on shape coexistence. The results confirm the shift of the deformed prolate structures to higher lying states but also indicate their increasing deformation with decreasing neutron nu…

Evolution of quadrupole collectivity in N=80 isotones toward the Z=64 subshell gap: The B(E2;2+1→0+1) value of 142Sm

It was shown that the evolution of the B(E2; 2+ 1 → 0+ 1 ) values in N = 80 isotones from Te to Nd is affected by the underlying subshell structure. This manifests itself in the observation of the local suppression of the B(E2) value at Z = 58 with respect to the neighboring nuclei 136Ba and 140Nd. To investigate this shell sensitivity toward the Z = 64 subshell gap, the B(E2; 2+ 1 → 0+ 1 ) value of the unstable nucleus 142Sm was measured utilizing the projectile Coulomb excitation technique. The radioactive ion beam (RIB) experiment was performed at the REX-ISOLDE facility at CERN. The B(E2) value of 32 (4) W.u. reflects the impact of the π(1g7/2 2d5/2) subshell closure at Z = 64 with resp…

Shape coexistence in the neutron-deficient even-even Hg182-188 isotopes studied via Coulomb excitation

Coulomb-excitation experiments to study electromagnetic properties of radioactive even-even Hg isotopes were performed with 2.85  MeV/nucleon mercury beams from REX-ISOLDE. Magnitudes and relative signs of the reduced E2 matrix elements that couple the ground state and low-lying excited states in Hg182-188 were extracted. Information on the deformation of the ground and the first excited 0+ states was deduced using the quadrupole sum rules approach. Results show that the ground state is slightly deformed and of oblate nature, while a larger deformation for the excited 0+ state was noted in Hg182,184. The results are compared to beyond mean field and interacting-boson based models and interp…

Local suppression of collectivity in theN=80isotones at theZ=58subshell closure

) transition strengths [1] and thenumber of nucleons in the valence shell. The global behaviorof these quantities between the major shells as a function ofthe nucleon number is well understood in the frameworks ofboth collective and microscopic models. One could expect thatthese general trends in the collective properties between themajorshellsaremodulated bythesubshellstructure.However,it is usually thought that the pairing correlations with anenergy scale of about 2 MeV, smear out and dissolve thesubshell structure as long as the separation energies betweenthe subshells are only about a few hundred keV.The recently observed evolution of the isovectorquadrupole-collective valence-shell exc…

New developments on the recoil distance doppler-shift method

Absolute transition probabilities are fundamental observables for nuclear structure. The recoil-distance-Doppler-shift (RDDS) technique, also called plunger technique, is a well established tool for the determination of these important experimental quantities via the measurement of lifetimes of excited nuclear states. Nowadays nuclear structure investigations are concentrated on exotic nuclei which are often produced with extremely small cross sections or with very low beam intensities. In order to use the RDDS technique also for the investigation of very exotic nuclei this method has to be adapted to the specific needs of these special reactions. This article gives an overview on recent RD…

Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes

Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po196,198,200,202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po200,202, the transitional and diagonal matrix elements of the 2+1 state are determined. In Po196,198 multistep Coulomb excitation is observed, populating the 4+1,0+2, and 2+2 states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from Po196 onwards. Three model descriptions are used to compare to the data. Calculati…

β−-delayed spectroscopy of neutron-rich tantalum nuclei: Shape evolution in neutron-rich tungsten isotopes

The low-lying structure of W-188,W-190,W-192 has been studied following beta decays of the neutron-rich mother nuclei Ta-188,Ta-190,Ta-192 produced following the projectile fragmentation of a 1-GeV-per-nucleon Pb-208 primary beam on a natural beryllium target at the GSI Fragment Separator. The beta-decay half-lives of Ta-188, Ta-190, and Ta-192 have been measured, with gamma-ray decays of low-lying states in their respective W daughter nuclei, using heavy-ion beta-gamma correlations and a position-sensitive silicon detector setup. The data provide information on the low-lying excited states in W-188, W-190, and W-192, which highlight a change in nuclear shape at W-190 compared with that of …

Decay studies in the A∼225 Po-Fr region from the DESPEC campaign at GSI in 2021

The HISPEC-DESPEC collaboration aims at investigating the struc-ture of exotic nuclei formed in fragmentation reactions with decay spectroscopymeasurements, as part of the FAIR Phase-0 campaign at GSI. This paper reportson first results of an experiment performed in spring 2021, with a focus on beta-decaystudies in the Po-Fr nuclei in the 220 < A <230 island of octupole deformationexploiting the DESPEC setup. Ion-beta correlations and fast-timing techniques arebeing employed, giving an insight into this difficult-to-reach region. peerReviewed

Microscopic structure of coexisting $0^+$ states in $^{68}$Ni probed via two-neutron transfer

© 2019 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. The structure of low-spin states originating from shape-coexisting configurations in Ni284068 was directly probed via the two-neutron transfer reaction Ni66(t,p)Ni68 in inverse kinematics using a radioactive ion beam on a radioactive target. The direct feeding to the first excited 0+ state was measured for center-of-mass angles 4-16 and amounts to an integral of 4.2(16)% rela…

Shape coexistence in $^{178}$Hg

Lifetime measurements of excited states in 178 Hg have been performed using the 103 Rh ( 78 Kr , p 2 n ) reaction at a beam energy of 354 MeV. The recoil-decay tagging (RDT) technique was applied to select the 178 Hg nuclei and associate the prompt γ rays with the correlated characteristic ground-state α decay. Lifetimes of the four lowest yrast states of 178 Hg have been determined using the recoil distance Doppler-shift (RDDS) method. The experimental data are compared to theoretical predictions with focus on shape coexistence. The results confirm the shift of the deformed prolate structures to higher lying states but also indicate their increasing deformation with decreasing neutron numb…

Isomers and high-spin structures in the N=81 isotones Xe135 and Ba137

The high-spin structures of the N = 81 isotones 135Xe and 137Ba are investigated after multinucleontransfer (MNT) and fusion-evaporation reactions. Both nuclei are populated in (i) 136Xe+238U and (ii) 136Xe+208Pb MNT reactions employing the high-resolution Advanced Gamma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA, (iii), in the 136Xe+198Pt MNT reaction employing the -ray array GAMMASPHERE in combination with the gas detector array Chico, and (iv) via a 11B+130Te fusion-evaporation reaction. The high-spin level schemes of 135Xe and 137Ba are considerably extended to higher energies. The 2058-keV (19=2 ) state in 135Xe is identified as an isomer, completing the systema…

Shape Coexistence in the Neutron-Deficient Even-EvenHg182−188Isotopes Studied via Coulomb Excitation

Coulomb-excitation experiments to study electromagnetic properties of radioactive even-even Hg isotopes were performed with 2.85 MeV/nucleon mercury beams from REX-ISOLDE. Magnitudes and relative signs of the reduced E2 matrix elements that couple the ground state and low-lying excited states in Hg182-188 were extracted. Information on the deformation of the ground and the first excited 0(+) states was deduced using the quadrupole sum rules approach. Results show that the ground state is slightly deformed and of oblate nature, while a larger deformation for the excited 0(+) state was noted in Hg-182; 184. The results are compared to beyond mean field and interacting-boson based models and i…

New ß-decaying state in 214Bi

Lifetime measurements of excited states in neutron-rich Ti53 : Benchmarking effective shell-model interactions

Level lifetimes of the yrast (5/2(-)) to 13/2(-) states in the neutron-rich nucleus Ti-53, produced in a multinucleon-transfer reaction, have been measured for the first time. The recoil distance Doppler-shift method was employed and lifetimes of the excited states were extracted by a lineshape analysis aided by GEANT4-based Monte-Carlo simulations. The experiment was performed at the Grand Accelerateur National d'Ions Lourds facility in Caen, France, by using the Advanced Gamma Tracking Array for the gamma-ray detection coupled to the large-acceptance variable mode spectrometer for an event-by-event particle identification and the Cologne plunger for deep-inelastic reactions. Reduced trans…

Shape dynamics in neutron-rich Kr isotopes: Coulomb excitation of 92Kr, 94Kr and 96Kr

We report on the study of excited states in 92,94,96Kr populated via projectile Coulomb excitation at safe energies. The radioactive ion beams at energies of 2.85 MeV/u were delivered by the REX-ISOLDE facility at CERN and impinged on self-supporting 194,196Pt targets. The emitted γ -rays were detected by the Miniball detector-array. A detailed description of the experimental techniques used for extracting diagonal and transitional matrix elements and of the theoretical framework is given. The present experiment reveals the moderate evolution of the collective structure in the considered neutron-rich Kr isotopic chain, which is supported by the interacting boson model combined with the self…

Coulomb Excitation of Proton-rich N=80 Isotones at HIE-ISOLDE

Abstract A projectile Coulomb-excitation experiment was performed at the radioactive ion beam facility HIE-ISOLDE at CERN. The radioactive 140Nd and 142Sm ions were post accelerated to the energy of 4.62 MeV/A and impinged on a 1.45 mg/cm2-thin 208Pb target. The γ rays depopulating the Coulomb-excited states were recorded by the HPGe-array MINIBALL. The scattered charged particles were detected by a double-sided silicon strip detector in forward direction. Experimental γ-ray intensities were used for the determination of electromagnetic transition matrix elements. Preliminary results for the reduced transition strength of the B ( M 1 ; 2 3 + → 2 1 + ) = 0.35 ( 19 ) μ N 2 of 140Nd and a firs…

Collective 2$^{+1}$ excitations in$^{206}$Po and$^{208,210}$Rn

In the present study, $B(E2; 2^{+}_{1}\rightarrow 0^{+}_{1})$ values have been measured in the 208,210Rn and 206Po nuclei through Coulomb excitation of re-accelerated radioactive beams in inverse kinematics at CERN-ISOLDE. These nuclei have been proposed to lie in, or at the boundary of the region where the seniority scheme should persist. However, contributions from collective excitations are likely to be present when moving away from the N=126 closed shell. Such an effect is confirmed by the observed increased collectivity of the $2^{+}_{1}\rightarrow 0^{+}_{1}$ transitions. Experimental results have been interpreted with the aid of theoretical studies carried out within the BCS-based QRP…

β-Delayed and isomer spectroscopy of neutron-rich Ta and W isotopes

Decays of neutron-rich A ~ 190 nuclei have been studied following projectile fragmentation of a 208Pb beam on a 9Be target at the GSI Fragment Separator. Gamma-ray decays from previously reported isomeric states in 188Ta, 190W and 192, 193Re were used as internal calibrations for the particle identification analysis, together with the identification of previously unreported isomeric decays in 189Ta and 191W. The current work also identifies β-delayed γ rays following the decay of 188Ta to 188W for the first time. Algora, Alejandro, Alejandro.Algora@ific.uv.es ; Molina Palacios, Francisco Manuel, Francisco.Molina@ific.uv.es; Rubio Barroso, Berta, Berta.Rubio@ific.uv.es

Measurement of lifetimes in Fe-62,Fe-64, Co-61,Co-63, and Mn-59

Lifetimes of the 4(1)(+) states in Fe-62,Fe-64 and the 11/2(1)(-) states in Co-61,Co-63 and Mn-59 were measured at the Grand Accelerateur National d'Ions Lourds (GANIL) facility by using the Advanced Gamma Tracking Array (AGATA) and the large-acceptance variable mode spectrometer (VAMOS++). The states were populated through multinucleon transfer reactions with a U-238 beam impinging on a Ni-64 target, and lifetimes in the picosecond range were measured by using the recoil distance Doppler shift method. The data show an increase of collectivity in the iron isotopes approaching N = 40. The reduction of the subshell gap between the nu 2p(1/2) and nu 1g(9/2) orbitals leads to an increased popul…

Nature of seniority symmetry breaking in the semimagic nucleus $^{94}Ru$

Physical review / C 105(3), L031304 (2022). doi:10.1103/PhysRevC.105.L031304

β-delayedγ-ray spectroscopy of203,204Au and200−202Pt

The beta decay of five heavy, neutron-rich nuclei, Pt-203,Pt-204 and Ir200-202, has been investigated following relativistic cold fragmentation reactions of lead projectiles using the FRS + RISING setup at GSI. This paper reports on the study of the low-lying states in the decay daughter nuclei Au-203,Au-204 and Pt200-202. The characteristic gamma rays for each nucleus have been determined using beta-delayed gamma-ray spectroscopy. Tentative level schemes, relative intensities, and apparent beta feedings are provided. These data are compared with shell-model calculations, which indicate a substantial contribution to the total beta strength from high-energy first-forbidden beta-decay transit…

New β-decaying state in 214Bi

A new β-decaying state in 214Bi has been identified at the ISOLDE Decay Station at the CERN-ISOLDE facility. A preferred Iπ = (8−) assignment was suggested for this state based on the β-decay feeding pattern to levels in 214Po and shell-model calculations. The half-life of the Iπ = (8−) state was deduced to be T1/2 = 9.39(10) min. The deexcitation of the levels populated in 214Po by the β decay of this state was investigated via γ -γ coincidences and a number of new levels and transitions was identified. Shell-model calculations for excited states in 214Bi and 214Po were performed using two different effective interactions: the H208 and the modified Kuo-Herling particle interaction. Both ca…

Coulomb excitation of re-accelerated 208Rn and 206Po beams

In the present study, B( E2; 2(+)-> 0(+) ) values have been measured in the Rn-208 and Po-206 nuclei through Coulomb excitation of re-accelerated radioactive beams in inverse kinematics at CERN-ISOLDE. The resulting B(E2; 2(+)-> 0(+)) in 208Rn is similar to 0.08 e(2)b(2). These nuclei lie in, or at the boundary of the region where seniority scheme should persist. However, contributions from collective excitations may be present when moving away from the N = 126 shell closure. To date, surprisingly little is known of the transition probabilities between the low-spin states in this region.

Evidence for a Smooth Onset of Deformation in the Neutron-Rich Kr Isotopes

The neutron-rich nuclei Kr94,96 were studied via projectile Coulomb excitation at the REX-ISOLDE facility at CERN. Level energies of the first excited 2 + states and their absolute E2 transition strengths to the ground state are determined and discussed in the context of the E(21+) and B(E2;21+→01+) systematics of the krypton chain. Contrary to previously published results no sudden onset of deformation is observed. This experimental result is supported by a new proton-neutron interacting boson model calculation based on the constrained Hartree-Fock-Bogoliubov approach using the microscopic Gogny-D1M energy density functional. © 2012 American Physical Society.

Preliminary results of lifetime measurements in neutron-rich $^{53}$Ti

To study the nuclear structure of neutron-rich titanium isotopes, a lifetime measurement was performed at the Grand Accélérateur National d'Ions Lourds (GANIL) facility in Caen, France. The nucleiwere produced in a multinucleon-transfer reaction by using a 6.76 MeV/u 238U beam. The Advanced Gamma Tracking Array (AGATA) was employed for the γ-ray detection and target-like recoils were identified event-by-event by the large-acceptance variable mode spectrometer (VAMOS++). Preliminary level lifetimes of the (5/2−) to 13/2− states of the yrast band in the neutron-rich nucleus 53Ti were measured for the first time employing the recoil distance Doppler-shift (RDDS) method and the compact plunger …

Testing refined shell-model interactions in thesdshell: Coulomb excitation ofNa26

Background: Shell-model calculations crucially depend on the residual interaction used to approximate the nucleon-nucleon interaction. Recent improvements to the empirical universal $sd$ interaction (USD) describing nuclei within the $sd$ shell yielded two new interactions---USDA and USDB---causing changes in the theoretical description of these nuclei.Purpose: Transition matrix elements between excited states provide an excellent probe to examine the underlying shell structure. These observables provide a stringent test for the newly derived interactions. The nucleus $^{26}\mathrm{Na}$ with 7 valence neutrons and 3 valence protons outside the doubly-magic ${}^{16}\mathrm{O}$ core is used a…

Erratum: Evidence for a Smooth Onset of Deformation in the Neutron-Rich Kr Isotopes [Phys. Rev. Lett.108, 062701 (2012)]

Lifetime measurements in Ti52,54 to study shell evolution toward N=32

Lifetimes of the excited states in the neutron-rich Ti-52,Ti-54 nuclei, produced in a multinucleon-transfer reaction, were measured by employing the Cologne plunger device and the recoil-distance D ...

Coulomb Excitation of Neutron-Rich Zn Isotopes: First Observation of the21+State inZn80

Neutron-rich, radioactive Zn isotopes were investigated at the Radioactive Ion Beam facility REX-ISOLDE (CERN) using low-energy Coulomb excitation. The energy of the 2(1)+ state in 78Zn could be firmly established and for the first time the 2+ --> 0(1)+ transition in 80Zn was observed at 1492(1) keV. B(E2,2(1)+ --> 0(1)+) values were extracted for (74,76,78,80)Zn and compared to large scale shell model calculations. With only two protons outside the Z=28 proton core, 80Zn is the lightest N=50 isotone for which spectroscopic information has been obtained to date. Two sets of advanced shell model calculations reproduce the observed B(E2) systematics. The results for N=50 isotones indicate a g…

In-beam γ-ray spectroscopy of 94Ag

A recoil-beta-tagging experiment has been per formed to study the excited T = 0 and T = 1 states in the odd–odd N = Z nucleus 94Ag, populated via the 40Ca(58Ni,1p3n)94Ag reaction. The experiment was con ducted using the MARA recoil separator and JUROGAM3 array at the Accelerator Laboratory of the University of Jyväskylä. Through correlating fast, high-energy beta decays at the MARA focal plane with prompt γ rays emitted at the reaction target, a number of transitions between excited states in 94Ag have been identified. The timing characteris tics of these transitions confirm that they fall within decay sequences that feed the short-lived T = 1 ground state of 94Ag. The transitions are propo…

Restoring the valence-shell stabilization in Nd 140

A projectile Coulomb-excitation experiment was performed at the radioactive-ion beam facility HIE-ISOLDE at CERN to obtain E2 and M1 transition matrix elements of Nd-140 using the multistep Coulomb-excitation code GOSIA. The absolute M1 strengths, B(M1; 2(2)(-) -> 2(1)(+)) = 0.033(8)mu(2)(N), B(M1 ; 2(3)(+) -> 2(1)(+)) = 0.26(-0.10)(+0.11)mu(2)(N), and B(M1; 2(4)+ -> 2(1)(+)) <0.04 mu(2)(N) identify the 2(3)(+) state as the main fragment of the one-quadrupole-phonon proton-neutron mixed-symmetry state of Nd-140. The degree of F-spin mixing in Nd-140 was quantified with the determination of the mixing matrix element VF-mix <7(-7)(-13) keV. Peer reviewed

Multipleβ−decaying states in194Re: Shape evolution in neutron-rich osmium isotopes

decays from heavy, neutron-rich nuclei with A∼190 have been investigated following their production via the relativistic projectile fragmentation of an E/A=1 GeV 208Pb primary beam on a ∼2.5 g/cm2 9Be target. The reaction products were separated and identified using the GSI FRagment Separator (FRS) and stopped in the RISING active stopper. γ decays were observed and correlated with these secondary ions on an event-by-event basis such that γ-ray transitions following from both internal (isomeric) and β decays were recorded. A number of discrete, β-delayed γ-ray transitions associated with β decays from 194Re to excited states in 194Os have been observed, including previously reported decays …

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around Z=82 and the neutron midshell at N=104. Purpose: Evidence for shape coexistence has been inferred from α-decay measurements, laser spectroscopy, and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of Rn202 and Rn…

Search for Isovector Valence-Shell Excitations in 140 Nd and 142 Sm via Coulomb excitation reactions of radioactive ion beams

Projectile Coulomb excitation experiments were performed at HIE-ISOLDE at CERN with the radioactive ion beams of 140Nd and 142Sm. Ions with an energy of 4:62 MeV/A were impinging on a 1.45 mg/cm2 thick 208Pb target. The γ-rays depopulating the Coulomb-excited states were recorded by the HPGe-array MINIBALL and scattered particles were detected by a double-sided silicon strip detector. Experimental intensities were used for the determination of electromagnetic transition matrix elements. A preliminary result of the B(M1; 2+3 → 2+1) of 140Nd and an upper limit for the case of 142Sm are revealing the main fragments of the proton-neutron mixed-symmetry 2+1;ms states.

High-spin structures in Xe132 and Xe133 and evidence for isomers along the N=79 isotones

Author(s): Vogt, A; Siciliano, M; Birkenbach, B; Reiter, P; Hadynska-Klȩk, K; Wheldon, C; Valiente-Dobon, JJ; Teruya, E; Yoshinaga, N; Arnswald, K; Bazzacco, D; Blazhev, A; Bracco, A; Bruyneel, B; Chakrawarthy, RS; Chapman, R; Cline, D; Corradi, L; Crespi, FCL; Cromaz, M; De Angelis, G; Eberth, J; Fallon, P; Farnea, E; Fioretto, E; Fransen, C; Freeman, SJ; Fu, B; Gadea, A; Gelletly, W; Giaz, A; Gorgen, A; Gottardo, A; Hayes, AB; Hess, H; Hetzenegger, R; Hirsch, R; Hua, H; John, PR; Jolie, J; Jungclaus, A; Karayonchev, V; Kaya, L; Korten, W; Lee, IY; Leoni, S; Liang, X; Lunardi, S; MacChiavelli, AO; Menegazzo, R; Mengoni, D; Michelagnoli, C; Mijatovic, T; Montagnoli, G; Montanari, D; Muller-…

Corrigendum to: “Shape dynamics in neutron-rich Kr isotopes: Coulomb excitation of 92Kr, 94Kr and 96Kr” [Nucl. Phys. A 899 (2013) 1–28]

Isospin symmetry in thesdshell: Transition strengths in the neutron-deficientsdshell nucleusAr33

Reduced transition strengths of the deexciting transitions from the first two excited states in 33Ar were measured in a relativistic Coulomb excitation experiment at the GSI Helmholtz center. The radioactive ion beam was produced by fragmentation of a primary 36Ar beam on a 9Be target followed by the selection of the reaction product of interest via the GSI Fragment Separator. The 33Ar beam hit a secondary 197Au target with an energy of approximately 145 MeV/nucleon. An array of high-purity germanium cluster detectors and large-volume BaF2 scintillator detectors were employed for γ -ray spectroscopy at the secondary target position. The Lund-York-Cologne Calorimeter was used to track the ou…

Determination of the B(E3, 0+ → 3−)-excitation strength in octupole-correlated nuclei near A ≈224 by the means of Coulomb excitation at REX-ISOLDE

The IS475 collaboration conducted Coulomb-excitation experiments with postaccelerated radioactive 220Rn and 224Ra beams at the REX-ISOLDE facility. The beam particles (Ebeam ≈ 2.83 MeV/u) were Coulomb excited using 60Ni, 114Cd, and 120Sn scattering targets. De-excitation γ-rays were detected employing the Miniball array and scattered particles were detected in a silicon detector. Exploiting the Coulomb-excitation code GOSIA for each nucleus several matrix elements could be obtained from the measured γ-ray yields. The extracted 3−||Ê3||0+ matrix element allows for the conclusion that, while 220Rn represents an octupole vibrational system, 224Ra has already substantial octupole correlations i…

Local suppression of collectivity in the N=80 isotones at the Z=58 subshell closure

Background: Recent data on N=80 isotones have suggested that the proton π(1g7/2) subshell closure at Z=58 has an impact on the properties of low-lying collective states. Purpose: Knowledge of the B(E2;2+1→0+1) value of 140Nd is needed in order to test this conjecture. Method: The unstable, neutron-rich nucleus 140Nd was investigated via projectile Coulomb excitation at the REX-ISOLDE facility with the MINIBALL spectrometer. Results: The B(E2) value of 33(2) W.u. expands the N=80 systematics beyond the Z=58 subshell closure. Conclusions: The measurement demonstrates that the reduced collectivity of 138Ce is a local effect possibly due to the Z=58 subshell closure and requests refined theoret…

Evidence of octupole-phonons at high spin in 207Pb

A lifetime measurement of the 19/2 state in Pb has been performed using the Recoil Distance Doppler-Shift (RDDS) method. The nuclei of interest were produced in multi-nucleon transfer reactions induced by a Pb beam impinging on a Mo enriched target. The beam-like nuclei were detected and identified in terms of their atomic mass number in the VAMOS++ spectrometer while the prompt γ rays were detected by the AGATA tracking array. The measured large reduced transition probability B(E3,19/2→13/2)=40(8) W.u. is the first indication of the octupole phonon at high spin in Pb. An analysis in terms of a particle-octupole-vibration coupling model indicates that the measured B(E3) value in Pb is compa…

Half-Life Systematics across theN=126Shell Closure: Role of First-Forbidden Transitions in theβDecay of Heavy Neutron-Rich Nuclei

This Letter reports on a systematic study of β-decay half-lives of neutron-rich nuclei around doubly magic Pb208. The lifetimes of the 126-neutron shell isotone Pt204 and the neighboring Ir200-202, Pt203, Au204 are presented together with other 19 half-lives measured during the "stopped beam" campaign of the rare isotope investigations at GSI collaboration. The results constrain the main nuclear theories used in calculations of r-process nucleosynthesis. Predictions based on a statistical macroscopic description of the first-forbidden β strength reveal significant deviations for most of the nuclei with N<126. In contrast, theories including a fully microscopic treatment of allowed and first…

Testing refined shell-model interactions in the sd shell: Coulomb excitation of 26Na

Background: Shell-model calculations crucially depend on the residual interaction used to approximate the nucleon-nucleon interaction. Recent improvements to the empirical universal sd interaction (USD) describing nuclei within the sd shell yielded two new interactions—USDA and USDB—causing changes in the theoretical description of these nuclei. Purpose: Transitionmatrix elements between excited states provide an excellent probe to examine the underlying shell structure. These observables provide a stringent test for the newly derived interactions. The nucleus 26Na with 7 valence neutrons and 3 valence protons outside the doubly-magic 16O core is used as a test case. Method: A radioactive b…

The Miniball spectrometer

The Miniball germanium detector array has been operational at the REX (Radioactive ion beam EXperiment) post accelerator at the Isotope Separator On-Line facility ISOLDE at CERN since 2001. During the last decade, a series of successful Coulomb excitation and transfer reaction studies have been performed with this array, utilizing the unique and high-quality radioactive ion beams which are available at ISOLDE. In this article, an overview is given of the technical details of the full Miniball setup, including a description of the γ-ray and particle detectors, beam monitoring devices and methods to deal with beam contamination. The specific timing properties of the REX-ISOLDE facility are hi…

β-decay study of150Er,152Yb, and156Yb: Candidates for a monoenergetic neutrino beam facility

The beta decays of ^{150}Er, ^{152}Yb, and ^{156}Yb nuclei are investigated using the total absorption spectroscopy technique. These nuclei can be considered possible candidates for forming the beam of a monoenergetic neutrino beam facility based on the electron capture (EC) decay of radioactive nuclei. Our measurements confirm that for the cases studied, the EC decay proceeds mainly to a single state in the daughter nucleus.

97/37 Rb 60 : The Cornerstone of the Region of Deformation around A∼100

Excited states of the neutron-rich nuclei 97,99Rb were populated for the first time using the multistep Coulomb excitation of radioactive beams. Comparisons of the results with particle-rotor model calculations provide clear identification for the ground-state rotational band of 97Rb as being built on the πg9/2 [431] 3/2+ Nilsson-model configuration. The ground-state excitation spectra of the Rb isotopes show a marked distinction between single-particle-like structures below N=60 and rotational bands above. The present study defines the limits of the deformed region around A∼100 and indicates that the deformation of 97Rb is essentially the same as that observed well inside the deformed regi…

Enhanced Quadrupole and Octupole Strength in Doubly Magic Sn132

The first 2+ and 3- states of the doubly magic nucleus Sn132 are populated via safe Coulomb excitation employing the recently commissioned HIE-ISOLDE accelerator at CERN in conjunction with the highly efficient MINIBALL array. The Sn132 ions are accelerated to an energy of 5.49 MeV/nucleon and impinged on a Pb206 target. Deexciting γ rays from the low-lying excited states of the target and the projectile are recorded in coincidence with scattered particles. The reduced transition strengths are determined for the transitions 0g.s.+→21+, 0g.s.+→31-, and 21+→31- in Sn132. The results on these states provide crucial information on cross-shell configurations which are determined within large-sca…

Studies of pear-shaped nuclei using accelerated radioactive beams

There is strong circumstantial evidence that certain heavy, unstable atomic nuclei are ‘octupole deformed’, that is, distorted into a pear shape. This contrasts with the more prevalent rugby-ball shape of nuclei with reflection-symmetric, quadrupole deformations. The elusive octupole deformed nuclei are of importance for nuclear structure theory, and also in searches for physics beyond the standard model; any measurable electric-dipole moment (a signature of the latter) is expected to be amplified in such nuclei. Here we determine electric octupole transition strengths (a direct measure of octupole correlations) for short-lived isotopes of radon and radium. Coulomb excitation experiments we…

Fast-timing Measurement in \(^{96}\)Pd: Improved Accuracy for the Lifetime of the \(4_1^{+}\) State

Direct lifetime measurements via γ–γ coincidences using the FATIMA fast-timing LaBr3(Ce) array were performed for the excited states below previously reported isomers. In the N = 50 semi-magic 96Pd nucleus, lifetimes below the I π = 8+ seniority isomer were addressed as a benchmark for further analysis. The results for the I π = 2+ and 4 + states confirm the published values. Increased accuracy for the lifetime value was achieved for the 4 + state. peerReviewed

Superallowed Gamow-Teller decay of the doubly magic nucleus $^{100}$Sn

Expérience au GSI; The shell structure of atomic nuclei is associated with 'magic numbers' and originates in the nearly independent motion of neutrons and protons in a mean potential generated by all nucleons. During b1-decay, a proton transforms into a neutron in a previously not fully occupied orbital, emitting a positron-neutrino pair with either parallel or antiparallel spins, in a Gamow-Teller or Fermi transition, respectively. The transition probability, or strength, of a Gamow-Teller transition depends sensitively on the underlying shell structure and is usually distributed among many states in the neighbouring nucleus. Here we report measurements of the half-life and decay energy fo…

Collectivity in ${}^{\mathrm{196,198}}$Pb isotopes probed in Coulomb-excitation experiments at REX-ISOLDE

The neutron-deficient ${}^{\mathrm{196,198}}$Pb isotopes have been studied in Coulomb-excitation experiments employing the Miniball γ-ray spectrometer and radioactive ion beams from the REX-ISOLDE post-accelerator at CERN. The reduced transition probabilities of the first excited 2+ states in 196Pb and 198Pb nuclei have been measured for the first time. Values of $B(E2)={18.2}_{-4.1}^{+4.8}$ W.u. and $B(E2)={13.1}_{-3.5}^{+4.9}$ W.u., were obtained, respectively. The experiment sheds light on the development of collectivity when moving from the regime governed by the generalised seniority scheme to a region, where intruding structures, associated with different deformed shapes, start to com…

Relativistic Coulomb excitation of Kr 88

International audience; To investigate the systematics of mixed-symmetry states in N=52 isotones, a relativistic Coulomb excitation experiment was performed during the PreSPEC campaign at the GSI Helmholtzzentrum für Schwerionenforschung to determine E2 transition strengths to 2+ states of the radioactive nucleus $^{88}$Kr. Absolute transition rates could be measured towards the first and third 2+ states. For the latter a mixed-symmetry character is suggested on the basis of the indication for a strong M1 transition to the fully symmetric 21+ state, extending the knowledge of the N=52 isotones below Z=40. A comparison with the proton-neutron interacting boson model and shell-model predictio…

Electromagnetic properties of low-lying states in neutron-deficient Hg isotopes: Coulomb excitation of Hg-182, Hg-184, Hg-186 and Hg-188

The neutron-deficient mercury isotopes serve as a classical example of shape coexistence, whereby at low energy near-degenerate nuclear states characterized by different shapes appear. The electromagnetic structure of even-mass 182-188 Hg isotopes was studied using safe-energy Coulomb excitation of neutron-deficient mercury beams delivered by the REX-ISOLDE facility at CERN. The population of $ 0^{+}_{1,2}$01,2+, $ 2^{+}_{1,2}$21,2+and $ 4^{+}_{1}$41+states was observed in all nuclei under study. Reduced E2 matrix elements coupling populated yrast and non-yrast states were extracted, including their relative signs. These are a sensitive probe of shape coexistence and may be used to validate…

High-spin structure of Xe134

A. Vogt et al. ; 12 págs.; 9 figs.; 1 tab.

Do nuclei go pear-shaped? Coulomb excitation of 220Rn and 224Ra at REX-ISOLDE (CERN)

Artículo escrito por muchos autores, sólo se referencian el primero, los autores que firman como Universidad Autónoma de Madrid y el grupo de colaboración en el caso de que aparezca en el artículo

Coulomb excitation of Na-29,Na-30: Mapping the borders of the island of inversion

Seidlitz, M., et all ; 10 pags. ; 9 figs. ; 1 tab. ; PACS number(s): 21.60.Cs, 23.20.Js, 25.70.De, 29.38.Gj

High-spin structure in the transitional nucleus Xe131 : Competitive neutron and proton alignment in the vicinity of the N=82 shell closure

The transitional nucleus 131Xe is investigated after multinucleon transfer (MNT) in the 136Xe+208Pb and 136Xe+238U reactions employing the high-resolution Advanced GAmma Tracking Array (AGATA) coupled to the magnetic spectrometer PRISMA at the Laboratori Nazionali di Legnaro, Italy and as an elusive reaction product in the fusion-evaporation reaction 124Sn(11B,p3n) 131Xe employing the HORUS γ-ray array coupled to a double-sided silicon strip detector (DSSSD) at the University of Cologne, Germany. The level scheme of 131Xe is extended to 5 MeV. A pronounced backbending is observed at ~ω ≈ 0.4 MeV along the negative-parity one-quasiparticle νh11/2(α = −1/2) band. The results are compared to t…

Spins and electromagnetic moments of Cd101–109

The neutron-deficient cadmium isotopes have been measured by high-resolution laser spectroscopy at CERN-ISOLDE. The electromagnetic moments of $^{101}\mathrm{Cd}$ have been determined for the first time and the quadrupole-moment precision of $^{103}\mathrm{Cd}$ has been vastly improved. The results on the sequence of $5/{2}^{+}$ ground states in $^{101--109}\mathrm{Cd}$ are tentatively discussed in the context of simple structure in complex nuclei as similarities are found with the $11/{2}^{\ensuremath{-}}$ states in the neutron-rich cases. Comparison with shell-model calculations reveals a prominent role of the two holes in the $Z=50$ core.