Isotopic distributions of thermal-neutron-induced fission fragments of near-symmetric fission of Pu239,241 determined using calorimetric low-temperat…

2021

Isotopic distributions were measured for the light fragment group in the transition region from asymmetric to symmetric fission for thermal neutron induced fission of $^{239}\mathrm{Pu}$ and $^{241}\mathrm{Pu}$ using the novel technology of calorimetric low temperature detectors in combination with the passive absorber method. Nuclear charge distributions were determined for 24 masses in the range $A=89$ to $A=112$ for $^{241}\mathrm{Pu}({n}_{\mathrm{th}},f)$ for the first time with the LOHENGRIN mass spectrometer. Moving from asymmetric to symmetric fission, known data were supplemented for masses from $A=110$ to $A=112$ for $^{241}\mathrm{Pu}({n}_{\mathrm{th}},f)$ and from $A=109$ to $A=1…