0000000001173456

AUTHOR

J. Peter Toennies

showing 2 related works from this author

Magic numbers, excitation levels, and other properties of small neutral 4He clusters (Nor = 50).

2006

The ground-state energies and the radial and pair distribution functions of neutral 4He clusters are systematically calculated by the diffusion Monte Carlo method in steps of one 4He atom from 3 to 50 atoms. In addition the chemical potential and the low-lying excitation levels of each cluster are determined with high precision. These calculations reveal that the "magic numbers" observed in experimental 4He cluster size distributions, measured for free jet gas expansions by nondestructive matter-wave diffraction, are not caused by enhanced stabilities. Instead they are explained in terms of an enhanced growth due to sharp peaks in the equilibrium concentrations in the early part of the expa…

Distribution functionChemistryExcited stateAtomMonte Carlo methodCluster (physics)General Physics and AstronomyDiffusion Monte CarloPhysical and Theoretical ChemistryAtomic physicsDiffusion (business)ExcitationThe Journal of chemical physics
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Magic numbers, excitation levels, and other properties of small neutral math clusters (N < 50)

2006

The ground-state energies and the radial and pair distribution functions of neutral math clusters are systematically calculated by the diffusion Monte Carlo method in steps of one math atom from 3 to 50 atoms. In addition the chemical potential and the low-lying excitation levels of each cluster are determined with high precision. These calculations reveal that the “magic numbers” observed in experimental math cluster size distributions, measured for free jet gas expansions by nondestructive matter-wave diffraction, are not caused by enhanced stabilities. Instead they are explained in terms of an enhanced growth due to sharp peaks in the equilibrium concentrations in the early part of the e…

DiffusionHelium neutral atoms ; Atomic clusters ; Ground states ; Excited states ; Chemical potential ; Diffusion ; Monte Carlo methods ; Molecular configurationsHelium neutral atomsAtomic clustersExcited statesMonte Carlo methods:FÍSICA::Química física [UNESCO]Chemical potentialMolecular configurationsGround statesUNESCO::FÍSICA::Química física
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