Author: Guo-zhang Huang

0000000001217849

AUTHOR

Guo-zhang Huang

Isolation of a perfectly linear uranium(II) metallocene

Reduction of the uranium(III) metallocene [(eta(5)-(C5Pr5)-Pr-i)(2)UI] (1) with potassium graphite produces the "second-generation" uranocene [(eta(5)-(C5Pr5)-Pr-i)(2)U] (2), which contains uranium in the formal divalent oxidation state. The geometry of 2 is that of a perfectly linear bis(cyclopentadienyl) sandwich complex, with the ground-state valence electron configuration of uranium(II) revealed by electronic spectroscopy and density functional theory to be 5f(3) 6d(1). Appreciable covalent contributions to the metal-ligand bonds were determined from a computational study of 2, including participation from the uranium 5f and 6d orbitals. Whereas three unpaired electrons in 2 occupy orbi…

research product

CCDC 1955099: Experimental Crystal Structure Determination

Related Article: Richard Layfield, Fu-Sheng Guo, Nikolaus Tsoureas, Guo-Zhang Huang, Ming-Liang Tong, Akseli Mansikkamäki|2020|Angew.Chem.,Int.Ed.|59|2299|doi:10.1002/anie.201912663

research product

CSD 1953092: Experimental Crystal Structure Determination

Related Article: Richard Layfield, Fu-Sheng Guo, Nikolaus Tsoureas, Guo-Zhang Huang, Ming-Liang Tong, Akseli Mansikkamäki|2020|Angew.Chem.,Int.Ed.|59|2299|doi:10.1002/anie.201912663

research product

CSD 1953094: Experimental Crystal Structure Determination

Related Article: Richard Layfield, Fu-Sheng Guo, Nikolaus Tsoureas, Guo-Zhang Huang, Ming-Liang Tong, Akseli Mansikkamäki|2020|Angew.Chem.,Int.Ed.|59|2299|doi:10.1002/anie.201912663

research product

CSD 1953093: Experimental Crystal Structure Determination

Related Article: Richard Layfield, Fu-Sheng Guo, Nikolaus Tsoureas, Guo-Zhang Huang, Ming-Liang Tong, Akseli Mansikkamäki|2020|Angew.Chem.,Int.Ed.|59|2299|doi:10.1002/anie.201912663

research product

PEPhysical Sciences and Engineering
- PE2Fundamental Constituents of Matter
  - PE2_1Theory of fundamental interactions
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- PE1Mathematics
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LSLife Sciences
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SHSocial Sciences and Humanities
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