Author: Kaifeng Wu

0000000001299346

AUTHOR

Kaifeng Wu

showing 2 related works from this author

Photo-Induced Cluster-to-Cluster Transformation of [Au37–xAgx(PPh3)13Cl10]3+ into [Au25–yAgy(PPh3)10Cl8]+: Fragmentation of a Trimer of 8-Electron Su…

2021

We present the photoinduced size/structure transformation of [Au37-xAgx(PPh3)13Cl10]3+ (M37) into [Au25-yAgy(PPh3)10Cl8]+ (M25) cluster. Single-crystal X-ray diffraction revealed that M37 has a tri-icosahedron M36 metal core assembled via the fusion of three Au7Ag6 icosahedrons in a cyclic fashion and that the M36 core is further protected by phosphine and chloride ligands. The M37 cluster is found to be highly sensitive toward ambient light, and the M37 → M25 transition is observed with 530 nm irradiation, monitored by time-dependent UV-vis spectroscopy, electrospray ionization mass spectrometry (ESI-MS), and femtosecond transient absorption spectroscopy. Linear-response time-dependent DFT…

Materials science010405 organic chemistryElectrospray ionizationTrimer010402 general chemistry01 natural sciencesDissociation (chemistry)0104 chemical sciencesCrystallographyFragmentation (mass spectrometry)Ultrafast laser spectroscopyCluster (physics)General Materials SciencePhysical and Theoretical ChemistryAbsorption (chemistry)SpectroscopyThe Journal of Physical Chemistry Letters

researchProduct

CCDC 2093430: Experimental Crystal Structure Determination

2022

Related Article: Zhaoxian Qin, Junhui Wang, Sachil Sharma, Sami Malola, Kaifeng Wu, Hannu Häkkinen, Gao Li|2021|J.Phys.Chem.Lett.|12|10920|doi:10.1021/acs.jpclett.1c02863

Space GroupCrystallographyCrystal SystemCrystal Structuredecakis(mu-chloro)-tridecakis(triphenylphosphine)-octadeca-gold-nonadeca-silver tris(hexafluoroantimonate)Cell ParametersExperimental 3D Coordinates

researchProduct

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