0000000001303756
AUTHOR
Xiaoyi Duan
Spin Crossover in a Series of Non-Hofmann-Type Fe(II) Coordination Polymers Based on [Hg(SeCN)3]− or [Hg(SeCN)4]2– Building Blocks
Self-assembly of [Hg(SeCN)4]2- tetrahedral building blocks, iron(II) ions, and a series of bis-monodentate pyridyl-type bridging ligands has afforded the new heterobimetallic HgII-FeII coordination polymers {Fe[Hg(SeCN)3]2(4,4'-bipy)2}n (1), {Fe[Hg(SeCN)4](tvp)}n (2), {Fe[Hg(SeCN)3]2(4,4'-azpy)2}n (3), {Fe[Hg(SeCN)4](4,4'-azpy)(MeOH)}n (4), {Fe[Hg(SeCN)4](3,3'-bipy)}n (5) and {Fe[Hg(SeCN)4](3,3'-azpy)}n (6) (4,4-bipy = 4,4'-bipyridine, tvp = trans-1,2-bis(4-pyridyl)ethylene, 4,4'-azpy = 4,4'-azobispyridine, 3,3-bipy = 3,3'-bipyridine, 3,3'-azpy = 3,3'-azobispyridine). Single-crystal X-ray analyses show that compounds 1 and 3 display a two-dimensional robust sheet structure made up of infini…
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