Author: Hongfeng Wang

0000000001307144

AUTHOR

Hongfeng Wang

A hybrid magnet with coexistence of ferromagnetism and photoinduced Fe(iii) spin-crossover

International audience; The insertion of a [Fe(sal2-trien)]+ complex cation into a 2D oxalate network results in a hybrid magnet with coexistence of magnetic ordering and photoinduced spin-crossover (LIESST effect) in compound [FeIII(sal2-trien)][MnIICrIII(ox)3]*(CH2Cl2) (1). A complete photomagnetic characterization together with a detailed structural analysis of the low-spin (LS) and high-spin (HS) structures of 1 is presented in order to understand such unusual behavior. This very rare and unexpected property in a FeIII spin-crossover complex, has been attributed to the strong distortion exhibited by the metastable HS state. Furthermore, 1 has shown that, in contrast to what has been pre…

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Stimuli responsive hybrid magnets : tuning the photoinduced spin-crossover in Fe(III) complexes inserted into layered magnets

The insertion of a [Fe(sal_2 trien)]^+ complex cation into a 2D oxalate network in the presence of different solvents results in a family of hybrid magnets with coexistence of magnetic ordering and photoinduced spin crossover (LIESST effect) in compounds [Fe^{III}(sal_2 trien)][Mn^{II}Cr^{III}(ox)_3]·CHCl_3 (1·CHCl_{3}) [Fe^{III}(sal_{2} trien)][Mn^{II}Cr^{III}(ox)_{3}]·CHBr_{3} (1·CHBr_{3}) and [Fe^{III}(sal_{2} trien)][Mn^{II}Cr^{III}(ox)_{3}]·CH_{2}Br_{2} (1·CH_{2}Br_{2}). The three compounds crystallize in a 2D honeycomb anionic layer formed by Mn^{II} and Cr^{III} ions linked through oxalate ligands and a layer of [Fe(sal_{2} trien)]^{+} complexes and solvent molecules (CHCl_{3} CHBr_{…

research product

CCDC 929206: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

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CCDC 929201: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

research product

CCDC 929203: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

research product

CCDC 929204: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

research product

CCDC 929205: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

research product

CCDC 929202: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

research product

CCDC 929207: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

research product

CCDC 929208: Experimental Crystal Structure Determination

Related Article: Miguel Clemente-León, Eugenio Coronado, Maurici López-Jordà, João C. Waerenborgh, Cédric Desplanches, Hongfeng Wang, Jean-François Létard, Andreas Hauser , and Antoine Tissot|2013|J.Am.Chem.Soc.|135|8655|doi:10.1021/ja402674x

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