0000000001314405

AUTHOR

Víctor A. De La Peña O’shea

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Hydroxamate Titanium–Organic Frameworks and the Effect of Siderophore-Type Linkers over Their Photocatalytic Activity

2019

The chemistry of metal–organic frameworks (MOFs) relies on the controlled linking of organic molecules and inorganic secondary building units to assemble an unlimited number of reticular frameworks. However, the design of porous solids with chemical stability still remains limited to carboxylate or azolate groups. There is a timely opportunity to develop new synthetic platforms that make use of unexplored metal binding groups to produce metal–linker joints with hydrolytic stability. Living organisms use siderophores (iron carriers in Greek) to effectively assimilate iron in soluble form. These compounds make use of hard oxo donors as hydroxamate or catecholate groups to coordinate metal Lew…

SiderophoreQuímica organometàl·licachemistry.chemical_elementGeneral ChemistryTitani010402 general chemistry01 natural sciencesBiochemistryCombinatorial chemistryCatalysis0104 chemical sciencesCatalysisMetalchemistry.chemical_compoundColloid and Surface Chemistrychemistryvisual_artvisual_art.visual_art_mediumPhotocatalysisChemical stabilityLewis acids and basesCarboxylateTitaniumJournal of the American Chemical Society
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CCDC 1884457: Experimental Crystal Structure Determination

2019

Related Article: Natalia M. Padial, Javier Castells-Gil, Neyvis Almora-Barrios, Mariam Barawi, Ivan da Silva, Víctor A. de la Peña O’Shea and Carlos Martí-Gastaldo|2019|J.Am.Chem.Soc.|141|13124|doi:10.1021/jacs.9b04915

Space GroupCrystallographyCrystal SystemCrystal StructureCell Parameterscatena-(tris(mu-N1N4-dioxybenzene-14-dicarboxamide)-di-titanium dimethylformamide solvate)Experimental 3D Coordinates
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