6533b7ddfe1ef96bd1274aa6

RESEARCH PRODUCT

Orientation of Polar Molecules by Laser Induced Adiabatic Passage

Stéphane GuérinLeonid P. YatsenkoHans-rudolf JauslinOlivier FaucherBruno Lavorel

subject

[PHYS.PHYS.PHYS-OPTICS] Physics [physics]/Physics [physics]/Optics [physics.optics]Physics[ PHYS.PHYS.PHYS-OPTICS ] Physics [physics]/Physics [physics]/Optics [physics.optics]Linear polarizationChemical polarityGeneral Physics and AstronomyDouble-well potentialLaserlaw.inventionlawOrientation (geometry)HarmonicAtomic physicsMolecular alignmentAdiabatic processComputer Science::Databases

description

International audience; We show that two overlapping linearly polarized laser pulses of frequencies ω and its second harmonic 2ω can strongly orient linear polar molecules, by adiabatic passage along dressed states. The resulting robust orientation can be interpreted as a laser-induced localization in the effective double well potential created by the fields, which induces a preliminary molecular alignment. The direction of the orientation can be selected by the relative phase of the fields.

https://hal.archives-ouvertes.fr/hal-00398111