6533b827fe1ef96bd1285ba5

RESEARCH PRODUCT

Crystal structure of (3E)-5-nitro-3-(2-phenylhydrazinylidene)-1H-indol-2(3H)-one

Renan Lira De FariasAdailton J. BortoluzziJecika Maciel VelasquesVanessa Carratu GerviniAdriano Bof De Oliveira

subject

0301 basic medicinecrystal structureStereochemistryin silico evaluationtwo-dimensional hydrogen-bonded networkCrystal structureReductaseisatin–hydrazone derivative010403 inorganic & nuclear chemistryRing (chemistry)01 natural sciencesCrystal03 medical and health scienceschemistry.chemical_compoundHirshfeld surface calculationGeneral Materials ScienceCrystallographybiologyHydrogen bondActive siteGeneral ChemistryCondensed Matter Physics0104 chemical sciences030104 developmental biologychemistryQD901-999biology.proteinNitroisatin-hydrazone derivativeDerivative (chemistry)

description

The reaction between 5-nitroisatin and phenylhydrazine in acidic ethanol yields the title compound, C14H10N4O3, whose molecular structure deviates slightly from a planar geometry (r.m.s. deviation = 0.065 Å for the mean plane through all non-H atoms). An intramolecular N—H...O hydrogen bond is present, forming a ring of graph-set motifS(6). In the crystal, molecules are linked by N—H...O and C—H...O hydrogen-bonding interactions into a two-dimensional network along (120), and rings of graph-set motifR22(8),R22(26) andR44(32) are observed. Additionally, a Hirshfeld surface analysis suggests that the molecules are stacked along [100] through C=O...Cginteractions and indicates that the most important contributions for the crystal structure are O...H (28.5%) and H...H (26.7%) interactions. Anin silicoevaluation of the title compound with the DHFR enzyme (dihydrofolate reductase) was performed. The isatin–hydrazone derivative and the active site of the selected enzyme show N—H...O(ASP29), N—H...O(ILE96) andCg...Cg(PHE33) interactions.

10.1107/s2056989016020375http://scripts.iucr.org/cgi-bin/paper?S2056989016020375