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RESEARCH PRODUCT

Isotope shifts of neutron-deficient gold isotopes with 193?A?190

H. KremmlingJ. StreibH.-j. KlugeH. W. SchaafR. B. MooreK. Wallmeroth

subject

PhysicsNuclear and High Energy PhysicsIsotopeResonance fluorescenceKinetic isotope effectAnalytical chemistryResonanceNeutronIsotopes of goldSpectroscopyMolecular electronic transition

description

The isotope shift between197Au (stable) and the radioactive Au isotopes190Au,191Au,192Au and193Au were determined by resonance fluorescence spectroscopy in the 6s2S1/2–6p2P1/2.λ=267.6nm line. The unstable Au isotopes were produced at the ISOLDE mass separator at CERN. The nuclei were investigated semi on-line in a resonance vessel, heated to 1,400°C. The results areδν190,197=−11.12(39) GHz,δν191,197=−9.67(12) GHz,δν192,197=−8.32(15) GHz,δν193,197=−6.29(11) GHz, corresponding to a change of the mean-square charge radius byδ〈r2〉190,197 =0.261(12) fm2,δ〈r2〉191,197=0.227(5) fm2,δ〈r2〉192,197=0.195(5) fm2,δ〈r2〉193,197 =0.148(4) fm2.

https://doi.org/10.1007/bf01432427