6533b82ffe1ef96bd1295354

RESEARCH PRODUCT

Non-equilibrium surface diffusion in the O/W(110) system

I. VattulainenJ. MerikoskiT. Ala-nissilaS. C. Ying

subject

Condensed Matter (cond-mat)FOS: Physical sciencesCondensed Matter

description

In this Letter, we present results of an extensive Monte Carlo study of the O/W(110) system under non-equilibrium conditions. We study the mean square displacements and long wavelength density fluctuations of adatoms. From these quantities, we define effective and time-dependent values for the collective and tracer diffusion mobilities. These mobilities reduce to the usual diffusion constants when equilibrium is reached. We discuss our results in view of existing experimental measurements of effective diffusion barriers, and the difficulties associated with interpreting non-equilibrium data.

https://dx.doi.org/10.48550/arxiv.cond-mat/9606184