Templatgesteuerte Photoreaktion von C60auf Calcit

6533b854fe1ef96bd12afc6d

RESEARCH PRODUCT

Templatgesteuerte Photoreaktion von C60auf Calcit

Angelika Kühnle André Gourdon Markus Kittelmann Ralf Bechstein Philipp Rahe Philipp Rahe Robert Lindner

subject

General Medicine

description

Wir zeigen die photochemisch induzierte Reaktion von C60 auf dem Nichtleiter Calcit, die mit Nichtkontakt-Rasterkraftmikroskopie untersucht wurde. Die Bildung kovalenter Bindungen wird durch die Verringerung intermolekularer Abstande offensichtlich. Diese Interpretation wird zusatzlich durch UV/Vis- und Massenspektren an dicken Filmen gestutzt. Die Bestrahlung von C60 fuhrt zu wohlgeordneten, kovalent verknupften Domanen. Daruber hinaus wird die Orientierung der Domanen durch die Gitterdimensionen des Calcitsubstrats vorgegeben. Die Gitterfehlanpassung gezielt zu nutzen, um bewusst die Richtung der Reaktion zu beeinflussen, ist ein neuer Ansatz, um Reaktionen auf Oberflachen maszuschneidern. Hier stellen wir eine Strategie vor, die es ermoglicht, orientierte, kovalente Netzwerke auf Nichtleitern zu generieren.

year	journal	country	edition	language
2014-04-01	Angewandte Chemie

https://doi.org/10.1002/ange.201309128

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