6533b872fe1ef96bd12d380e
RESEARCH PRODUCT
Recent developments in resonance ionization mass spectrometry for ultra-trace analysis of actinide elements
Tobias ReichNina KneipSebastian RaederKlaus WendtDominik StuderNorbert Trautmannsubject
Chemistry010401 analytical chemistryRadiochemistryActinideMass spectrometry01 natural sciences0104 chemical sciences0103 physical sciencesResonance ionizationTrace analysisPhysics::Atomic PhysicsPhysical and Theoretical Chemistry010306 general physicsUltra tracedescription
Abstract Resonance ionization mass spectrometry is an efficient tool to detect minute amounts of long-lived radio-isotopes in environmental samples. Applying resonant excitation and ionization with pulsed laser radiation within a hot cavity atomizer enables the sensitive detection and precise quantification of long-lived actinide isotopes. Due to the inherently element selective ionization process, this method ensures ultimate suppression of contaminations from other elements and molecules. The characterization of in-source resonance ionization of the actinide elements U, Th, Np, and Am using a compact quadrupole mass spectrometer (QMS) setup are discussed.
year | journal | country | edition | language |
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2019-06-01 | Radiochimica Acta |