Search results for " Polarization"
showing 10 items of 668 documents
Accurate Prediction of Hyperfine Coupling Tensors for Main Group Elements Using a Unitary Group Based Rigorously Spin-Adapted Coupled-Cluster Theory
2019
We present the development of a perturbative triples correction scheme for the previously reported unitary group based spin-adapted combinatoric open-shell coupled-cluster (CC) singles and doubles (COS-CCSD) approach and report on the applications of the newly developed method, termed "COS-CCSD(T)", to the calculation of hyperfine coupling (HFC) tensors for radicals consisting of hydrogen, second- and third-row elements. The COS-CCSD(T) method involves a single noniterative step with [Formula: see text] scaling of the computational cost for the calculation of triples corrections to the energy. The key feature of this development is the use of spatial semicanonical orbitals generated from st…
Measurement of the quadrupole moment of Re185 and Re187 from the hyperfine structure of muonic X rays
2020
The hyperfine splitting of the 5g→4f transitions in muonic Re185,187 has been measured using high resolution high purity germanium detectors and compared to state-of-the-art atomic theoretical predictions. The spectroscopic quadrupole moment has been extracted using modern fitting procedures and compared to the values available in literature obtained from muonic x rays of natural rhenium. The extracted values of the nuclear spectroscopic quadrupole moment are 2.07(5) b and 1.94(5) b, respectively for Re185 and Re187.
Modulational instability in resonant optical fiber with higher-order dispersion effect
2010
International audience; The modulational instability (MI) of an electromagnetic wave in a resonant optical fiber with a two-level system is investigated. In the normal dispersion regime, we find the occurrence of nonconventional MI sidebands which are induced by the two-level resonant atoms. We also observe that the MI gain spectra are suppressed by the higher-order dispersion effect in the anomalous dispersion regime.
Spinovo rozlisena time-of-flight k-reozlisena fotoemissia Ir-- Kompletny fotoemissny experiment.
2017
Ultramicroscopy 183, 19 - 29 (2017). doi:10.1016/j.ultramic.2017.06.025
Complete hyperfine Paschen-Back regime at relatively small magnetic fields realized in potassium nano-cell
2015
A one-dimensional nano-metric-thin cell (NC) filled with potassium metal has been built and used to study optical atomic transitions in external magnetic fields. These studies benefit from the remarkable features of the NC allowing one to use $\lambda/2$- and $\lambda$-methods for effective investigations of individual transitions of the K D_1 line. The methods are based on strong narrowing of the absorption spectrum of the atomic column of thickness L equal to $\lambda/2$ and to $\lambda$(with $\lambda = 770\un{nm}$ being the resonant laser radiation wavelength). In particular, for a $\pi$-polarized radiation excitation the $\lambda$-method allows us to resolve eight atomic transitions (in…
Imaging magnetic scalar potentials by laser-induced fluorescence from bright and dark atoms
2014
We present a spectroscopic method for mapping two-dimensional distributions of magnetic field strengths (magnetic scalar potential lines) using charge-coupled device (CCD) recordings of the fluorescence patterns emitted by spin-polarized Cs vapour in a buffer gas exposed to inhomogeneous magnetic fields. The method relies on the position-selective destruction of spin polarization by magnetic resonances induced by multi-component oscillating magnetic fields, such that magnetic potential lines can be directly detected by the CCD camera. We also present a generic algebraic model allowing for the calculation of the fluorescence patterns and find excellent agreement with the experimental observa…
Angular momentum alignment-to-orientation conversion in the ground state of Rb atoms at room temperature
2020
We investigated experimentally and theoretically angular momentum alignment-to-orientation conversion created by the joint interaction of laser radiation and an external magnetic field with atomic rubidium at room temperature. In particular we were interested in alignment-to-orientation conversion in atomic ground state. Experimentally the laser frequency was fixed to the hyperfine transitions of $D_1$ line of rubidium. We used a theoretical model for signal simulations that takes into account all neighboring hyperfine levels, the mixing of magnetic sublevels in an external magnetic field, the coherence properties of the exciting laser radiation, and the Doppler effect. The experiments were…
Coherent vector pi-pulse in optical amplifiers
2007
We obtain an exact vector solitary solution for the amplification of an optical pulse with a time width short compared with both population and polarization decay time. This dissipative soliton results from the balance between the gain from inverted resonant two-level atoms and the linear loss of the host material. We suppose that the excited state of the active centers is degenerate on the projection of the angular moment. Numerical simulations demonstrate the stability of these vector dissipative solitons in the presence of both linear birefringence and group velocity dispersion of the host material.
Polarization shaping for unidirectional rotational motion of molecules.
2015
Control of the orientation of the angular momentum of linear molecules is demonstrated by means of laser polarization shaping. For this purpose, we combine two orthogonally polarized and partially time-overlapped femtosecond laser pulses so as to produce a spinning linear polarization which in turn induces unidirectional rotation of N2 molecules. The evolution of the rotational response is probed by a third laser beam that can be either linearly or circularly polarized. The physical observable is the frequency shift imparted to the probe beam as a manifestation of the angular Doppler effect. Our experimental results are confirmed by theoretical computations, which allow one to gain a deep p…
Harmonic generation from nanorings driven by a two-color laser field
2014
We study the high harmonic generation and the polarization of the harmonics emitted by a nanoring driven by two laser fields of angular frequency ?1 and ?2, with ?2?=?2?1, and ?1 resonant between the ground and the first excited state. We show that by varying parameters, such as laser intensity, photon energy and the delay between the two laser pulses, we can control the number of harmonics and the polarization of the radiation. In particular we show that with this choice of two-laser photon frequency rate we obtain more harmonics with respect to other configurations. We also calculated the average absorbed energy and the average angular momentum acquired by the electron as a function of th…