Search results for " laser spectroscopy"
showing 10 items of 113 documents
Induced optical absorption and ITS relaxation in LiNbO3
1999
Abstract Electron pulse induced absorption spectra and their decay kinetics have been investigated in LiNbO3 crystals with various Li/Nb ratios rasnging from congruent to stoichiometric composition. It is shown that the absorption spectra, the optical density and the decay kinetics depend on the Li/Nb ratio. The rising front of the induced absorption is too fast to be resolved. The room temperature decay, characterized by the half-lifetime Δt, is faster in the stoichiometric crystal (∼ 750 ns) than in the congrruent crystal (∼ 3.5 μs).
Pulsed electron beam excited transient absorption in SrTiO3
2002
Abstract Transient absorption (TA) spectra and optical density relaxation kinetics in SrTiO3 (STO), STO–Nb and STO–V were studied. The electron polaron free or bound at intrinsic defect is suggested to be responsible for the TA band at ∼1.4 eV observed in STO. The band peaking below 0.75 eV in STO–Nb is proposed to be from Nb4+. The electron center V3+ or electron polaron bound in the vicinity of V4+ is responsible for the absorption band at 1.0 eV in STO–V. The absorption from hole polarons is suggested to be in the range 1.8–2.3 eV. It is shown that TA in pure STO at room temperature decays due to electron–hole polaron recombination.
First application of the Laser Ion Source and Trap (LIST) for on-line experiments at ISOLDE
2012
The Laser Ion Source and Trap (LIST) provides a new mode of operation for the resonance ionization laser ion source (RILIS) at ISOLDE/CERN, reducing the amount of surface-ionized isobaric contaminants by up to four orders of magnitude. After the first successful on-line test at ISOLDE in 2011 the LIST was further improved in terms of efficiency, selectivity, and reliability through several off-line tests at Mainz University and at ISOLDE. In September 2012, the first on-line physics experiments to use the LIST took place at ISOLDE. The measurements of the improved LIST indicate more than a twofold increase in efficiency compared to the LIST of the 2011 run. The suppression of surface-ionize…
First Offline Results from the S3 Low-Energy Branch
2022
International audience; We present the first results obtained from the S3 Low-Energy Branch , the gas cell setup at SPIRAL2-GANIL, which will be installed behind the S3 spectrometer for atomic and nuclear spectroscopy studies of exotic nuclei. The installation is currently being commissioned offline, with the aim to establish optimum conditions for the operation of the radio frequency quadrupole ion guides, mass separation and ion bunching, providing high-efficiency and low-energy spatial spread for the isotopes of interest. Transmission and mass-resolving power measurements are presented for the different components of the S3-LEB setup. In addition, a single-longitudinal-mode, injection-lo…
Quadrupole moments of odd-A 53−63Mn: Onset of collectivity towards N=40
2016
Physics letters / B 760, 387 - 392 (2016). doi:10.1016/j.physletb.2016.07.016
Experimental and theoretical studies of polaron optical properties in KNbO3 perovskite
2004
Time-resolved absorption and luminescence spectra have been measured in KNbO3 perovskite crystals after pulsed band-gap excitation by 200 fs laser pulses and 10 ns electron pulses. Quantum chemical calculations using the large unit cell periodic model support the interpretation of the observed transient absorption bands at 0.8 and 1.1 eV as the self-trapped electron polarons and bound hole polarons, respectively. The activation energy for the 2.2 eV green luminescence quenching is 0.05 eV. We suggest that the short lifetime (,15 ns) of the luminescence at RT is caused by the radiative recombination of nearest electron and hole polarons. q 2003 Elsevier Ltd. All rights reserved.
X‐ray and pulsed electron beam excited luminescence and optical absorption in KTaO 3 crystals
2005
Pulsed electron beam excited time-resolved transient absorption and luminescence have been studied in nominally pure and Li-doped KTaO3 single crystals. It is found that under electron beam excitation in nominally pure KTaO3 the absorption bands peaks at ∼0.8 eV, ∼1.1 eV and 1.7 eV whereas in KTaO3:Li at ∼1.1 eV and ∼1.7 eV. The transient absorption decay varies over the spectrum thus revealing several short-lived centers. The main luminescence peak is centred at ∼2.7 eV in all KTaO3 specimens. Luminescence decay kinetics observed for the two bands slightly differ indicating different kinds of excited states are involved. (© 2005 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim)
Size-And Wavelength-Dependent Two-Photon Absorption Cross-Section of CsPbBr3 Perovskite Quantum Dots
2017
All-inorganic colloidal perovskite quantum dots (QDs) based on cesium, lead, and halide have recently emerged as promising light emitting materials. CsPbBr3 QDs have also been demonstrated as stable two-photon-pumped lasing medium. However, the reported two photon absorption (TPA) cross sections for these QDs differ by an order of magnitude. Here we present an in-depth study of the TPA properties of CsPbBr3 QDs with mean size ranging from 4.6 to 11.4 nm. By using femtosecond transient absorption (TA) spectroscopy we found that TPA cross section is proportional to the linear one photon absorption. The TPA cross section follows a power law dependence on QDs size with exponent 3.3 +- 0.2. The …
Strong Exciton-Coherent Phonon Coupling in Single-Layer MoS2
2020
Broadband transient absorption with sub-20fs temporal resolution, supported by ab-initio calculations, quantitatively provides the strength of exciton-coherent phonon coupling in 1L-MoS2, showing a resonant profile around the C exciton.
Transient absorption of polarons in KNbO3
2002
Abstract Transient absorption spectra have been measured in a number of undoped KNbO 3 crystals following two kinds of electronic excitation: two-photon absorption of 200 fs laser pulses and 10 ns pulsed electron beam. A band peaking at 0.8 eV and broad, poorly resolved absorption in the range 1.3–3.3 eV were observed. Based on similarity to the 1 eV band in LiNbO 3 previously identified as the intrinsic electron polaron (electron self-localized on niobium in the regular lattice site), we suggest that the transient absorption band at 0.8 eV in KNbO 3 is also associated with the intrinsic electron polaron.