Search results for "ARTICLES"
showing 10 items of 9626 documents
Temperature effect on phase state and reactivity controls atmospheric multiphase chemistry and transport of PAHs
2017
Atmospheric refrigerator increases the global transport and health risks of carcinogenic PAHs.
New horizons in microparticle forensics: Actinide imaging and detection of 238Pu and 242mAm in hot particles
2021
Description
The size distribution of primary biological aerosol particles in cloud water on the mountain Kleiner Feldberg/Taunus (FRG)
2000
During the field campaign, FELDEX 95 cloud water samples were collected and the insoluble particles were analysed by single particle analysis in order to determine the content of primary biological aerosol particles (PBAP). It is found that 25% of the total insoluble particles are biological ones. During cloud events with increasing wind velocity, the concentration of biological particles also increases. Anthropogenic influence leads to a higher amount of both total and biological particles. Within the size distribution, the percentage of biological particles decreases with increasing radius.
Aircraft-based observation of meteoric material in lower-stratospheric aerosol particles between 15 and 68° N
2021
We analyse aerosol particle composition measurements from five research missions between 2014 and 2018 to assess the meridional extent of particles containing meteoric material in the upper troposphere and lower stratosphere (UTLS). Measurements from the Jungfraujoch mountaintop site and a low-altitude aircraft mission show that meteoric material is also present within middle- and lower-tropospheric aerosol but within only a very small proportion of particles. For both the UTLS campaigns and the lower- and mid-troposphere observations, the measurements were conducted with single-particle laser ablation mass spectrometers with bipolar-ion detection, which enabled us to measure the chemical c…
Airborne measurements of dust layer properties, particle size distribution and mixing state of Saharan dust during SAMUM 2006
2009
The Saharan Mineral Dust Experiment (SAMUM) was conducted in May/June 2006 in southern Morocco. As part of SAMUM, airborne in situ measurements of the particle size distribution in the diameter range 4 nm < Dp < 100 μm were conducted. The aerosol mixing state was determined below Dp < 2.5 μm. Furthermore, the vertical structure of the dust layers was investigated with a nadir-looking high spectral resolution lidar (HSRL). The desert dust aerosol exhibited two size regimes of different mixing states: below 0.5 μm, the particles had a non-volatile core and a volatile coating; larger particles above 0.5 μm consisted of non-volatile components and contained light absorbing material. In…
Characterization of the inter-annual, seasonal, and diurnal variations of condensation particle concentrations at Neumayer, Antarctica
2011
Continuous condensation particle (CP) observations were conducted from 1984 through 2009 at Neumayer Station under stringent contamination control. During this period, the CP concentration (median 258 cm<sup>−3</sup>) showed no significant long term trend but exhibited a pronounced seasonality characterized by a stepwise increase starting in September and reaching its annual maximum of around 10<sup>3</sup> cm<sup>−3</sup> in March. Minimum values below 10<sup>2</sup> cm<sup>&ndash;3</sup> were observed during June/July. Dedicated time series analyses in the time and frequency domain revealed no significant correlations between…
An evaluation of the estimation of road traffic emission factors from tracer studies
2010
Road traffic emission factors (EFs) are one of the main sources of uncertainties in emission inventories; it is necessary to develop methods to reduce these uncertainties to manage air quality more efficiently. Recently an alternative method has been proposed to estimate the EFs. In that work the emission factors were estimated from a long term tracer study developed in Ho Chi Minh City (HCMC) Vietnam. A passive tracer was continuously emitted from a finite line source placed in one side of an urban street canyon. Simultaneously, the resulting tracer concentrations were monitored at the other side of the street. The results of this experiment were used to calculate the dispersion factors an…
A predictive model for salt nanoparticle formation using heterodimer stability calculations
2021
Acid–base clusters and stable salt formation are critical drivers of new particle formation events in the atmosphere. In this study, we explore salt heterodimer (a cluster of one acid and one base) stability as a function of gas-phase acidity, aqueous-phase acidity, heterodimer proton transference, vapor pressure, dipole moment and polarizability for salts comprised of sulfuric acid, methanesulfonic acid and nitric acid with nine bases. The best predictor of heterodimer stability was found to be gas-phase acidity. We then analyzed the relationship between heterodimer stability and J4×4, the theoretically predicted formation rate of a four-acid, four-base cluster, for sulfuric acid salts ove…
Beating Darwin-Bragg losses in lab-based ultrafast x-ray experiments
2017
The use of low temperature thermal detectors for avoiding Darwin-Bragg losses in lab-based ultrafast experiments has begun. An outline of the background of this new development is offered, showing the relevant history and initiative taken by this work. (C) 2017 Author(s). Funding Agencies|Knut and Alice Wallenberg Foundation; ERC [226136]; Finnish Funding Agency for Technology and Innovation TEKES; Academy of Finland [260880]; NIST Innovations in Measurement Science program; DOE Office of Basic Energy Sciences
Resonance ionization spectroscopy of thorium isotopestowards a laser spectroscopic identification of the low-lying 7.6 eV isomer of 229Th
2011
International audience; In-source resonance ionization spectroscopy was used to identify an efficient and selective three step excitation/ionization scheme of thorium, suitable for titanium:sapphire (Ti:sa) lasers. The measurements were carried out in preparation of laser spectroscopic investigations for an identification of the low-lying 229 m Th isomer predicted at 7.6 ± 0.5 eV above the nuclear ground state. Using a sample of 232 Th, a multitude of optical transitions leading to over 20 previously unknown intermediate states of even parity as well as numerous high-lying odd parity auto-ionizing states were identified. Level energies were determined with an accuracy of 0.06 cm −1 for inte…