Search results for "Absorption"
showing 10 items of 2701 documents
Phototransition of Na(3p3/2) into high Rydberg states and the ionization continuum
2005
A model potential method is used to investigate photoabsorption from the Na(3p3/2) state. Absorption cross sections into higher Rydberg states and photoionization cross sections are presented as an analytical function of photo electron energy. Einstein coefficients for spontaneous emissions 3p3/2 ← ns1/2, nd5/2, nd3/2 are tabulated for n up to 50. The Einstein coefficients and low-energy ionization cross sections are believed to be accurate to better than 2–3%, above 1 eV the error may increase to 4–6%.
MultiChannel Multiple Scattering Theory for XAFS. Application to L2,3 Edges of Ca
2005
We present a multichannel extension of the multiple scattering method for x-ray absorption fine structure (XAFS) spectroscopy that allows to take account of atomic multiplet-like electron correlation effects in condensed systems, on the basis of ab initio electron structure calculations. The formalism is outlined and an application to near-edge XAFS at the L2,3 edges of Ca metal is presented. In this system, the experimentally observed branching ratio deviates strongly from that obtained from the standard (one-electron) approach to XAFS. This is due to that fact that one-electron theory neglects the multiplet coupling between the photo-electron and the 2p core-hole. Within the multi-channel…
Interpretation of unexpected behavior of infrared absorption spectra ofScF3beyond the quasiharmonic approximation
2016
Scandium fluoride (${\mathrm{ScF}}_{3}$), having cubic ${\mathrm{ReO}}_{3}$-type structure, has attracted much scientific attention due to its rather strong negative thermal expansion (NTE) in the broad temperature range from 10 to 1100 K. Here we use the results of diffraction and extended x-ray absorption fine-structure (EXAFS) spectroscopy to interpret the influence of NTE on the temperature dependence of infrared absorption spectra of ${\mathrm{ScF}}_{3}$. Original infrared absorption and EXAFS experiments in a large temperature range are presented and interpreted using ab initio lattice dynamics simulations within and beyond quasiharmonic approximations. We demonstrate that ab initio e…
Resonant scattering in macromolecular structure research. Applications in molecular biology and material science
1983
Abstract This report concerns the X-ray resonance scattering work carried out using the instrument X15 which receives synchrotron radiation from the storage ring DORIS. X15 covers a wavelength range from 0.6 to 3.3 A. It therefore accesses resonance scattering at the K-absorption edges of the elements with Z = 20 (Ca) to Z = 42 (Mo) and at the L 3 -absorption edges from Z = 50 (Sn) to all heavier atoms. The instrument consists of a double monochromator with a vertical offset of the beam by 1.22 m and a camera of 10 m length. A multiwire proportional chamber (from A. Gabriel) at the end of the evacuated beam line detects the scattered X-ray photons on its area 200 mm × 200 mm. The distances …
Intensity Invariance of Strong-Field Two-Photon Absorption
2010
We demonstrate experimentally and theoretically the intensity-invariant scaling formula of coherent control of two-photon absorption as a function of pulse-shape parameters of ultrafast laser field in the strong-interaction regime.
Total absorption spectroscopy study of the β decay of Br86 and Rb91
2017
The beta decays of 86Br and 91Rb have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the IGISOL facility in Jyvaskyla and further purified using the JYFLTRAP. 86Br and 91Rb are considered high priority contributors to the decay heat in reactors. In addition 91Rb was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam et al. assuming that this decay was well known from high-resolution measurements. Our results shows that both decays were suffering from the Pandemonium effect and that the results of Rudstam et al. should be renormalized.
TAGS measurements of $^{100}$Nb ground and isomeric states and $^{140}$Cs for neutrino physics with the new DTAS detector
2016
V. Guadilla et al. -- 4 pags., 6 figs. -- Open Access funded by Creative Commons Atribution Licence 4.0
IGR J17451-3022: a dipping and eclipsing low mass X-ray binary
2016
In this paper, we report on the available X-ray data collected by INTEGRAL, Swift, and XMM-Newton during the first outburst of the INTEGRAL transient IGR J17451-3022, discovered in 2014 August. The monitoring observations provided by the JEM-X instruments on-board INTEGRAL and the Swift/XRT showed that the event lasted for about 9 months and that the emission of the source remained soft for the entire period. The source emission is dominated by a thermal component (kT~1.2 keV), most likely produced by an accretion disk. The XMM-Newton observation carried out during the outburst revealed the presence of multiple absorption features in the soft X-ray emission that could be associated to the p…
The nature of the extreme X-ray variability in the NLS1 1H 0707-495
2021
We examine archival XMM-Newton data on the extremely variable narrow-line Seyfert 1 (NLS1) active galactic nucleus (AGN) 1H 0707-495. We construct fractional excess variance (Fvar) spectra for each epoch, including the recent 2019 observation taken simultaneously with eROSITA. We explore both intrinsic and environmental absorption origins for the variability in different epochs, and examine the effect of the photoionised emission lines from outflowing gas. In particular, we show that the unusual soft variability first detected by eROSITA in 2019 is due to a combination of an obscuration event and strong suppression of the variance at 1 keV by photoionised emission, which makes the variance …
Chandra X-ray spectroscopy of a clear dip in GX 13+1
2014
The source GX 13+1 is a persistent, bright Galactic X-ray binary hosting an accreting neutron star. It shows highly ionized absorption features, with a blueshift of $\sim$ 400 km s$^{-1}$ and an outflow-mass rate similar to the accretion rate. Many other X-ray sources exhibit warm absorption features, and they all show periodic dipping behavior at the same time. Recently, a dipping periodicity has also been determined for GX 13+1 using long-term X-ray folded light-curves, leading to a clear identification of one of such periodic dips in an archival Chandra observation. We give the first spectral characterization of the periodic dip of GX 13+1 found in this archival Chandra observation perfo…