Search results for "Atom"
showing 10 items of 31559 documents
Comparative theoretical study of the Ag–MgO (100) and (110) interfaces
1999
We have calculated the atomic and electronic structures of Ag–MgO(100) and (110) interfaces using a periodic (slab) model and an ab initio Hartree–Fock approach with a posteriori electron correlation corrections. The electronic structure information includes interatomic bond populations, effective charges, and multipole moments of ions. This information is analyzed in conjunction with the interface binding energy and the equilibrium distances for both interfaces for various coverages. There are significant differences between partly covered surfaces and surfaces with several layers of metal, and these can be understood in terms of electrostatics and the electron density changes. For complet…
CCDC 1859264: Experimental Crystal Structure Determination
2020
Related Article: Fernando Machado dos Santos, Meiry Edivirges Alvarenga, Ana Karoline Silva Mendanha Valdo, Renato Rabelo, Danielle Cangussu de Castro Gomes, Ângelo de Fátima, Thiago Vinicius Costa Lara, Cleiton Moreira da Silva, Thiago Teixeira Tasso, João Honorato Araujo Neto, Alzir Azevedo Batista, Alejandro Pedro Ayala, Javier Alcides Ellena, Vinicius Ferraz Guimarães, Cecília Maria Alves Oliveira, Lidya Cardozo da Silva, Boniek Gontijo Vaz, Felipe Terra Martins|2020|Chem.Commun.|56|15024|doi:10.1039/D0CC07043B
Vacancy-like Dressed States in Topological Waveguide QED
2020
We identify a class of dressed atom-photon states formingat the same energy of the atom at any coupling strength. As a hallmark, their photonic component is an eigenstate of the bare photonic bath with a vacancy in place of the atom. The picture accommodates waveguide-QED phenomena where atoms behave as perfect mirrors, connecting in particular dressed bound states (BS) in the continuum or BIC with geometrically-confined photonic modes. When applied to photonic lattices, the framework provides a general criterion to predict dressed BS in lattices with topological properties by putting them in one-to-one correspondence with photonic BS. New classes of dressed BS are thus predicted in the pho…
Work fluctuations in bosonic Josephson junctions
2016
We calculate the first two moments and full probability distribution of the work performed on a system of bosonic particles in a two-mode Bose-Hubbard Hamiltonian when the self-interaction term is varied instantaneously or with a finite-time ramp. In the instantaneous case, we show how the irreversible work scales differently depending on whether the system is driven to the Josephson or Fock regime of the bosonic Josephson junction. In the finite-time case, we use optimal control techniques to substantially decrease the irreversible work to negligible values. Our analysis can be implemented in present-day experiments with ultracold atoms and we show how to relate the work statistics to that…
Aggregation of [Ln(12)(III)] clusters by the dianion of 3-formylsalicylic acid. Synthesis, crystal structures, magnetic and luminescence properties
2019
Three isostrucutral dodecanuclear clusters with the general formula [Ln(12)(fsa)(12)(mu f(3)-OH)(12)(DMF)(12)]center dot nDMF (fsa(2-) is the dianion of 3-formylsalicylic acid; Ln = Eu 1, Gd 2, Dy 3) have been obtained from the reaction of fromylsalicyclic acid (H(2)fsa), tetrabutylammonium hydroxide and Ln(NO3)(3)center dot 6H(2)O in methanol/DMF. Their structure consists of four vertex-sharing heterocubanes. Each heterocubane unit is assembled from four Ln(III) ions, three mu(3)-OH groups and one mu(3)-oxygen atom arising from the fsa(2-) carboxylato group. The photophysical properties of the europium derivative investigated at both 300 and 80 K sustain a relative intense emission obtaine…
Quantum-state transfer in staggered coupled-cavity arrays
2015
We consider a coupled-cavity array, where each cavity interacts with an atom under the rotating-wave approximation. For a staggered pattern of inter-cavity couplings, a pair of field normal modes each bi-localized at the two array ends arise. A rich structure of dynamical regimes can hence be addressed depending on which resonance condition between the atom and field modes is set. We show that this can be harnessed to carry out high-fidelity quantum-state transfer (QST) of photonic, atomic or polaritonic states. Moreover, by partitioning the array into coupled modules of smaller length, the QST time can be substantially shortened without significantly affecting the fidelity.
Atom-field dressed states in slow-light waveguide QED
2015
We discuss the properties of atom-photon bound states in waveguide QED systems consisting of single or multiple atoms coupled strongly to a finite-bandwidth photonic channel. Such bound states are formed by an atom and a localized photonic excitation and represent the continuum analog of the familiar dressed states in single-mode cavity QED. Here we present a detailed analysis of the linear and nonlinear spectral features associated with single- and multi-photon dressed states and show how the formation of bound states affects the waveguide-mediated dipole-dipole interactions between separated atoms. Our results provide a both qualitative and quantitative description of the essential strong…
Más allá de los dinosaurios: nuevas perspectivas para el patrimonio paleontológico de La Rioja
2018
El patrimonio paleontológico en nuestro país ha sido objeto de discusión entre científicos y legisladores desde su controvertida consideración dentro del patrimonio histórico en la Ley 16/1985, de 25 de junio, del Patrimonio Histórico Español. Así, tanto el patrimonio inmueble (yacimientos) como el mueble (ejemplares ex situ alojados en museos, colecciones y exposiciones locales) se gestionaron durante años bajo esta norma hasta su inclusión, en el año 2007, en la nueva Ley 42/2007, de 13 de diciembre, de Patrimonio Natural y Biodiversidad. Fil: García Ortiz de Landaluce, Esperanza. Universidad de la Rioja; España Fil: Díaz Martínez, Ignacio. Consejo Nacional de Investigaciones Científicas …
Dynamical learning of a photonics quantum-state engineering process
2021
Abstract. Experimental engineering of high-dimensional quantum states is a crucial task for several quantum information protocols. However, a high degree of precision in the characterization of the noisy experimental apparatus is required to apply existing quantum-state engineering protocols. This is often lacking in practical scenarios, affecting the quality of the engineered states. We implement, experimentally, an automated adaptive optimization protocol to engineer photonic orbital angular momentum (OAM) states. The protocol, given a target output state, performs an online estimation of the quality of the currently produced states, relying on output measurement statistics, and determine…
Energy transfer in LH2 of Rhodospirillum Molischianum, studied by subpicosecond spectroscopy and configuration interaction exciton calculations.
2001
Two color transient absorption measurements were performed on a LH2 complex from Rhodospirillum molischianum by using several excitation wavelengths (790, 800, 810, and 830 nm) and probing in the spectral region from 790 to 870 nm at room temperature. The observed energy transfer time of ∼1.0 ps from B800 to B850 at room temperature is longer than the corresponding rates in Rhodopseudomonas acidophila and Rhodobacter sphaeroides. We observed variations (0.9-1.2 ps) of B800-850 energy transfer times at different B800 excitation wavelengths, the fastest time (0.9 ps) was obtained with 800 nm excitation. At 830 nm excitation the energy transfer to the B850 ring takes place within 0.5 ps. The m…