Search results for "Attosecond"
showing 10 items of 22 documents
Attosecond Soft-X-Ray Spectroscopy in a Transition Metal Dichalcogenide
2019
Information about the real-time response of carriers to optical fields is paramount to advance information processing or to understand the bottlenecks of light-matter interaction and energy harvesting. Transition-metal dichalcogenide (TMDC) compounds are an emerging class of materials with attractive structural and electronic properties that can be thinned to the 2D limit and TiS 2 is a paradigmatic example for a semi-metallic TMDC, since its electron mobility ranges between that of a metal and a semiconductor.
Tailored pump-probe transient spectroscopy with time-dependent density-functional theory: controlling absorption spectra
2016
Recent advances in laser technology allow us to follow electronic motion at its natural time-scale with ultra-fast time resolution, leading the way towards attosecond physics experiments of extreme precision. In this work, we assess the use of tailored pumps in order to enhance (or reduce) some given features of the probe absorption (for example, absorption in the visible range of otherwise transparent samples). This type of manipulation of the system response could be helpful for its full characterization, since it would allow us to visualize transitions that are dark when using unshaped pulses. In order to investigate these possibilities, we perform first a theoretical analysis of the non…
Use of three detuned lasers to generate isolated attosecond pulses
2010
The dynamics of a one-dimensional atom driven by three-laser fields is investigated. The total electric field is made up of a fundamental laser field of intensity W cm−2 and wavelength λ = 820 nm and two weak lasers with larger wavelengths. The intensity of the two weak fields is with k = 0.25. The frequencies of the weak fields are and , with and . The three lasers have a Gaussian envelope of 72 fs FWHM. It is shown, by numerical computation and using the semiclassical theory of high-harmonic generation, that the atom interacting with this combined field is able to emit an isolated attosecond burst of radiation.
Simulating pump-probe photo-electron and absorption spectroscopy on the attosecond time-scale with time-dependent density-functional theory
2013
Molecular absorption and photoelectron spectra can be efficiently predicted with real-time time-dependent density functional theory. We show herein how these techniques can be easily extended to study time-resolved pump-probe experiments, in which a system response (absorption or electron emission) to a probe pulse is measured in an excited state. This simulation tool helps with the interpretation of fast-evolving attosecond time-resolved spectroscopic experiments, in which electronic motion must be followed at its natural timescale. We show how the extra degrees of freedom (pump-pulse duration, intensity, frequency, and time delay), which are absent in a conventional steady-state experimen…
Generation of isolated attosecond pulses using unipolar and laser fields
2009
A new scheme to generate isolated attosecond pulses is presented that involves the use of a laser field and of a unipolar field. The laser field has a pulse of intensity I = 1.5×1014 W cm−2 and wavelength λ = 820 nm. The unipolar pulse is an asymmetric pulse consisting of a sharp peak, lasting approximately half a laser period, i.e. nearly 1.4 fs, followed by a long and shallow tail. We show that on combining these two fields, it is possible to generate isolated attosecond pulses as short as 1/10 of a laser period, i.e. approximately 270 as. Moreover, it is argued that this scheme is robust either against small variations of the laser envelope, or against small changes in the delay between …
Time- and energy resolved photoemission electron microscopy-imaging of photoelectron time-of-flight analysis by means of pulsed excitations
2010
Abstract The present work enlightens the developments in time- and energy resolved photoemission electron microscopy over the past few years. We describe basic principles of the technique and demonstrate different applications. An energy- and time-filtering photoemission electron microscopy (PEEM) for real-time spectroscopic imaging can be realized either by a retarding field or hemispherical energy analyzer or by using time-of-flight optics with a delay line detector. The latter method has the advantage of no data loss at all as all randomly incoming particles are measured not only by position but also by time. This is of particular interest for pump–probe experiments in the femtosecond an…
Bremsstrahlung from a repulsive potential: attosecond pulse generation
2008
The collision of an electron against a repulsive potential in the presence of a laser field is investigated. It is found that a sufficiently strong laser field forces the electron to remain in the neighbourhood of the repulsive potential causing bremsstrahlung. By appropriately filtering the emitted signal, an electron in the presence of a repulsive potential is capable of generating attosecond pulses.
Modelling the effect of nuclear motion on the attosecond time-resolved photoelectron spectra of ethylene
2014
arXiv:1403.5408
Attosecond soft-X-ray spectroscopy of a transition metal dichalcogenide material
2019
We use attosecond soft X-ray pulses between 284 eV to 543 eV for orbital-selective and real-time probing of the opto-electronic response of semi metallic TiS2.