Search results for "Borole"
showing 10 items of 24 documents
CCDC 956378: Experimental Crystal Structure Determination
2013
Related Article: Adrian Y. Houghton, Virve A. Karttunen, Warren E. Piers, Heikki M. Tuononen|2014|Chem.Commun.|50|1295|doi:10.1039/C3CC48796B
CCDC 1010911: Experimental Crystal Structure Determination
2014
Related Article: Adrian Y. Houghton, Juha Hurmalainen, Akseli Mansikkamäki, Warren E. Piers, Heikki M. Tuononen|2014|Nature Chemistry|6|983|doi:10.1038/nchem.2063
CCDC 1998837: Experimental Crystal Structure Determination
2020
Related Article: Dorota Wieczorek, Ewa Kaczorowska, Marta Wiśniewska, Izabela D. Madura, Magdalena Leśniak, Jacek Lipok, Agnieszka Adamczyk-Woźniak|2020|Molecules|25|5999|doi:10.3390/molecules25245999
CCDC 777075: Experimental Crystal Structure Determination
2011
Related Article: Cheng Fan, L.G.Mercier, W.E.Piers, H.M.Tuononen, M.Parvez|2010|J.Am.Chem.Soc.|132|9604|doi:10.1021/ja105075h
CCDC 956382: Experimental Crystal Structure Determination
2013
Related Article: Adrian Y. Houghton, Virve A. Karttunen, Warren E. Piers, Heikki M. Tuononen|2014|Chem.Commun.|50|1295|doi:10.1039/C3CC48796B
CCDC 1937169: Experimental Crystal Structure Determination
2019
Related Article: Matthew M. Morgan, Maryam Nazari, Thomas Pickl, J. Mikko Rautiainen, Heikki M. Tuononen, Warren E. Piers, Gregory C. Welch, Benjamin S. Gelfand|2019|Chem.Commun.|55|11095|doi:10.1039/C9CC05103A
CCDC 1937170: Experimental Crystal Structure Determination
2019
Related Article: Matthew M. Morgan, Maryam Nazari, Thomas Pickl, J. Mikko Rautiainen, Heikki M. Tuononen, Warren E. Piers, Gregory C. Welch, Benjamin S. Gelfand|2019|Chem.Commun.|55|11095|doi:10.1039/C9CC05103A
CCDC 655686: Experimental Crystal Structure Determination
2008
Related Article: H.V.Ly, H.M.Tuononen, M.Parvez, R.Roesler|2008|Angew.Chem.,Int.Ed.|47|361|doi:10.1002/anie.200703556
CCDC 1029678: Experimental Crystal Structure Determination
2015
Related Article: Agnieszka Adamczyk-Woźniak, Krzysztof Ejsmont, Błażej Gierczyk, Ewa Kaczorowska, Alicja Matuszewska, Grzegorz Schroeder, Andrzej Sporzyński, Bartosz Zarychta|2015|J.Organomet.Chem.|788|36|doi:10.1016/j.jorganchem.2015.04.026
Mechanistic Studies on the Metal-Free Activation of Dihydrogen by Antiaromatic Pentarylboroles
2013
The perfluoro- and perprotiopentaphenylboroles 1 and 2 react with dihydrogen to effect H–H bond cleavage and formation of boracyclopentene products. The mechanism of this reaction has been studied experimentally through evaluation of the kinetic properties of the slower reaction between 2 and H2. The reaction is first-order in both [borole] and [H2] with activation parameters of ΔH⧧ = 34(8) kJ/mol and ΔS⧧ = −146(25) J mol–1 K–1. A minimal kinetic isotope effect of 1.10(5) was observed, suggesting an asynchronous geometry for H–H cleavage in the rate-limiting transition state. To explain the stereochemistry of the observed products, a ring-opening/ring-closing mechanism is proposed and suppo…