Search results for "COMPOUND"

showing 10 items of 35174 documents

BODIPY atropisomer interconversion, face discrimination, and superstructure appending

2016

International audience; A strategy was developed to append sterically hindered apical pickets on both faces of the BODIPY platform to prevent stacking and aggregation. Ortho-substitution of both the meso-phenyl ring and the boron-bound catechol affords the right directionality to append pickets, achieve face discrimination, featuring two inter-convertible atropisomers, and is reminiscent of the picket-fence strategy in porphyrins.

spectroscopybindingStereochemistryStackingAppend010402 general chemistryRing (chemistry)porphyrins01 natural sciencesbiomolecules[ CHIM ] Chemical SciencesCatalysischemistry.chemical_compounddimersMaterials Chemistryfluorophores[CHIM]Chemical SciencesAtropisomer010405 organic chemistryChemistryMetals and AlloysGeneral Chemistry0104 chemical sciencesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsFace discriminationCeramics and CompositescellsfluorescenceBODIPYprobesSuperstructure (condensed matter)moieties
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Spectroscopic characterization of alkaline earth uranyl carbonates

2005

A series of alkaline uranyl carbonates, M[UO{sub 2}(CO{sub 3}){sub 3}].nH{sub 2}O (M=Mg{sub 2}, Ca{sub 2}, Sr{sub 2}, Ba{sub 2}, Na{sub 2}Ca, and CaMg) was synthesized and characterized by inductively coupled plasma mass spectrometry (ICP-MS) and atomic absorption spectrometry (AAS) after nitric acid digestion, X-ray powder diffraction (XRD), and thermal analysis (TGA/DTA). The molecular structure of these compounds was characterized by extended X-ray absorption fine-structure (EXAFS) spectroscopy and X-ray photoelectron spectroscopy (XPS). Crystalline Ba{sub 2}[UO{sub 2}(CO{sub 3}){sub 3}].6H{sub 2}O was obtained for the first time. The EXAFS analysis showed that this compound consists of …

spectroscopysynthesisAbsorption spectroscopyTRLFSAnalytical chemistryElectron spectroscopyUranyl carbonateuraniumInorganic Chemistrycarbonatechemistry.chemical_compoundXPSMaterials ChemistrystructurePhysical and Theoretical ChemistrySpectroscopyX-ray spectroscopyExtended X-ray absorption fine structureChemistryCondensed Matter PhysicsUranylalkaline earthElectronic Optical and Magnetic MaterialsEXAFSX-ray crystallographyCeramics and CompositesJournal of Solid State Chemistry
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Spectroscopy of short-lived radioactive molecules

2020

Molecular spectroscopy offers opportunities for the exploration of the fundamental laws of nature and the search for new particle physics beyond the standard model1–4. Radioactive molecules—in which one or more of the atoms possesses a radioactive nucleus—can contain heavy and deformed nuclei, offering high sensitivity for investigating parity- and time-reversal-violation effects5,6. Radium monofluoride, RaF, is of particular interest because it is predicted to have an electronic structure appropriate for laser cooling6, thus paving the way for its use in high-precision spectroscopic studies. Furthermore, the effects of symmetry-violating nuclear moments are strongly enhanced5,7–9 in molecu…

spektroskopiacollinearnucl-ex01 natural sciences010305 fluids & plasmasRadiumchemistry.chemical_compoundIonizationExperimental nuclear physicsNuclear ExperimentPhysicsMultidisciplinaryLarge Hadron ColliderStable isotope rationew physics[PHYS.HTHE]Physics [physics]/High Energy Physics - Theory [hep-th]hep-thmolekyylithep-phradiumelectron: electric momentNuclear Physics - Theoryradioactivitymany-body problemElectronic structure of atoms and moleculesAtomic physicsydinfysiikkaParticle Physics - Theoryexceptionalnucl-th[PHYS.NUCL]Physics [physics]/Nuclear Theory [nucl-th]MonofluorideResearchInstitutes_Networks_Beacons/photon_science_institutechemistry.chemical_elementnucleus: structure functionElectronic structure[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]Photon Science InstituteArticle0103 physical sciencesionizationMoleculeNuclear Physics - Experiment010306 general physicsSpectroscopyenhancementParticle Physics - Phenomenologystabilitysensitivitylaserchemistry[PHYS.HPHE]Physics [physics]/High Energy Physics - Phenomenology [hep-ph]Exotic atoms and moleculesnucleus: deformation
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Overexpression of SAMDC1 gene in Arabidopsis thaliana increases expression of defense-related genes as well as resistance to Pseudomonas syringae and…

2014

It has been previously described that elevation of endogenous spermine levels in Arabidopsis could be achieved by transgenic overexpression of S-Adenosylmethionine decarboxylase (SAMDC) or Spermine synthase (SPMS). In both cases, spermine accumulation had an impact on the plant transcriptome, with up-regulation of a set of genes enriched in functional categories involved in defense-related processes against both biotic and abiotic stresses. In this work, the response of SAMDC1-overexpressing plants against bacterial and oomycete pathogens has been tested. The expression of several pathogen defense-related genes was induced in these plants as well as in wild type plants exposed to an exogeno…

sperminepolyaminesSperminePlant ScienceSAMDClcsh:Plant cultureMicrobiologychemistry.chemical_compoundbiotic stressJasmonateArabidopsisBotanyPseudomonas syringaePolyaminesArabidopsis thalianalcsh:SB1-1110Original Research ArticleJasmonateHyaloperonospora arabidopsidisbiologystress response and stress tolerancefungifood and beveragesBiotic stressbiology.organism_classificationjasmonatechemistrySpermine synthasebiology.proteinSpermineFrontiers in Plant Science
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Design Scheme of New Tetragonal Heusler Compounds for Spin-Transfer Torque Applications and its Experimental Realization

2012

Band Jahn-Teller type structural instabilities of cubic Mn(2)YZ Heusler compounds causing tetragonal distortions can be predicted by ab initio band-structure calculations. This allows for identification of new Heusler materials with tunable magnetic and structural properties that can satisfy the demands for spintronic applications, such as in spin-transfer torque-based devices.

spintronics010302 applied physicsMaterials scienceCondensed matter physicsSpintronicsMechanical EngineeringAb initioSpin-transfer torqueNanotechnology02 engineering and technology021001 nanoscience & nanotechnology01 natural sciencesCommunicationsspin-transfer torquesCondensed Matter::Materials ScienceTetragonal crystal systemMechanics of Materials0103 physical sciencesTorqueCondensed Matter::Strongly Correlated ElectronsGeneral Materials Sciencemagnetic properties0210 nano-technologyHeusler compoundsRealization (systems)Advanced Materials
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DESIGN OF SF3B1 SUBUNIT MODULATORS OF THE SF3B SPLICEOSOME COMPLEX

2022

The subject of this dissertation is the search for new therapeutic strategies for pancreatic cancer and aims to implement a Drug Discovery process for the rational design and synthesis of molecules active in the modulation of pathways related to the regulation of pre-mRNA splicing process. This research project is the result of a joint PhD between the University of Palermo, Italy, and the Department of Medical Oncology, VU University Medical Center, Amsterdam, The Netherlands. It integrates complementary skills in pharmaceutical chemistry and translational cancer research with a special focus on the rational design of new anticancer compounds potentially active on SF3B1 (Splicing Factor 3B …

splicing4]thiadiazole compoundsdrug resistancehuman equilibrative nucleoside transporter-13mesotheliomaSF3B1gemcitabinepancreatic ductal adenocarcinoma1-b][1SF3B1 splicing imidazo[21-b][134]thiadiazole compounds pancreatic ductal adenocarcinoma gemcitabine human equilibrative nucleoside transporter-1 drug resistance mesotheliomaimidazo[2
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The effects of antimicrobial sprays and mouthrinses on supragingival plaque regrowth: a comparative study.

2006

BACKGROUND: Due to the side effects of chlorhexidine digluconate (CHX) mouthrinsing, a spray has been proposed as an alternative method of CHX delivery to the oral cavity. The aim of this study was to investigate the plaque inhibitory effects of CHX, cetylpyridinium chloride (CPC), and triclosan (TRN) delivered by sprays and mouthrinses. METHODS: The study was an observer-masked, randomized cross-over design balanced for carryover effects, involving 15 healthy volunteers in a 4-day plaque regrowth model. Products being tested (0.2% CHX, 0.12% CHX, 0.05% CPC, and 0.03% TRN) were used both as sprays and mouthrinses. A saline solution served as a negative control. On day 1, subjects received p…

spray/therapeutic useAdultMalemedicine.medical_treatmentDental PlaqueMouthwashesDentistryCetylpyridiniumCetylpyridiniumSodium ChlorideCetylpyridinium chlorideDental plaqueOral hygienetriclosan/therapeutic use.chemistry.chemical_compoundSettore MED/28 - Malattie OdontostomatologichemedicineHumansSingle-Blind MethodColoring AgentsSalinedental plaque/prevention and controlAerosolsObserver VariationCross-Over Studiesmouthrinse/therapeutic usebusiness.industryChlorhexidineChlorhexidineDental ProphylaxisReproducibility of Resultsmedicine.diseaseOral HygieneCrossover studyTriclosanTriclosanchlorhexidine/ therapeutic usechemistryCetylpyridinium chloride/therapeutic useAnti-Infective Agents LocalPeriodonticsFemalebusinessmedicine.drugJournal of periodontology
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Absence of Adverse Effects of Tiotropium/Olodaterol Compared with the Monocomponents on Long-Term Heart Rate and Blood Pressure in Patients with Mode…

2020

Stefan Andreas,1,2 Lorcan McGarvey,3 Ulrich Bothner,4 Matthias Trampisch,4 Alberto de la Hoz,4 Matjaz Fležar,5 Roland Buhl,6 Peter Alter7 1Department of Cardiology and Pneumology, University Medical Center Göttingen, Göttingen, Germany; 2LungClinic Immenhausen, Immenhausen, Germany, Member of the German Center for Lung Research (DZL); 3Queen’s University Belfast, Belfast, UK; 4Boehringer Ingelheim International GmbH, Ingelheim am Rhein, Germany; 5Klinika Golnik, Golnik, Slovenia; 6Pulmonary Department, Johannes Gutenberg University Mainz, Mainz, Germany; 7Department of Medicine, Pulmonary and Critical Care Medicine, Philipps University of Marburg (UMR); Member o…

srčna frekvencamedicine.medical_specialtymedicine.drug_classDiastoleBlood PressureInternational Journal of Chronic Obstructive Pulmonary Diseasechronic obstructive -- drug therapychronic obstructive pulmonary disease03 medical and health scienceschemistry.chemical_compoundPulmonary Disease Chronic Obstructive0302 clinical medicinetiotropiumDouble-Blind MethodHeart RateInternal medicineBronchodilatorForced Expiratory VolumeHeart ratePost-hoc analysisheart ratemedicineHumans030212 general & internal medicineTiotropium BromideAdverse effectudc:616.2pulmonary diseasekrvni tlaktOriginal ResearchtiotropijCOPDbusiness.industryolodaterolkronična obstruktivna pljučna bolezen -- terapija z zdraviliOlodaterolblood pressureGeneral Medicinemedicine.diseasehumanities3. Good healthBenzoxazinesBronchodilator AgentsBlood pressureTreatment Outcome030228 respiratory systemchemistryCardiologybusinessInternational Journal of Chronic Obstructive Pulmonary Disease
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Efficient regio- and stereoselective access to novel fluorinated ?-aminocyclohexanecarboxylates

2013

A regio- and stereoselective method has been developed for the synthesis of novel fluorinated 2-aminocyclohexanecarboxylic acid derivatives with the fluorine attached to position 4 of the ring. The synthesis starts from either cis- or trans-β-aminocyclohex-4-enecarboxylic acids and involves regio- and stereoselective transformation of the ring C–C double bond through iodooxazine formation and hydroxylation, followed by hydroxy–fluorine or oxo–fluorine exchange.

stereoselective reactionDouble bondStereochemistrychemistry.chemical_elementaminohapotRing (chemistry)Full Research PaperhydroxylationHydroxylationlcsh:QD241-441chemistry.chemical_compoundlcsh:Organic chemistryepoxidationlcsh:Scienceta116chemistry.chemical_classificationamino acidsOrganic ChemistryfluorinationAmino acidChemistrychemistryFluorineStereoselectivitylcsh:QBeilstein Journal of Organic Chemistry
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Steroidal supramolecular metallogels

2020

The review deals with an expanding number of steroidal compounds that are capable of forming a metallogel providing a multitude of novel materials rich in their properties. The future of steroidal metallogels holds a myriad of potential applications as new intelligent materials. Detection of potentially harmful compounds without expensive instrumentation, entrapment of environmentally hazardous substances, and sensitive and selective nanomaterials represent only a few of these potential applications. This article reviews the design, synthesis, characterization, and applications of steroidal metallogels. peerReviewed

steroidal metallogelsMaterials sciencesteroidal compoundssupramolekulaarinen kemiaSupramolecular chemistryNanotechnologyGeneral ChemistryInstrumentation (computer programming)metallogelsChemical Society Reviews
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