Search results for "CORRELATE"
showing 10 items of 1259 documents
Optical Control of Entangled States in Quantum Wells
2012
We present theory and calculations for coherent high-fidelity quantum control of many-particle states in semiconductor quantum wells. We show that coupling a two-electron double quantum dot to a terahertz optical source enables targeted excitations that are one to two orders of magnitude faster and significantly more accurate than those obtained with electric gates. The optical fields subject to physical constraints are obtained through quantum optimal control theory that we apply in conjunction with the numerically exact solution of the time-dependent Schrodinger equation. Our ability to coherently control arbitrary two-electron states, and to maximize the entanglement, opens up further pe…
Signatures of enhanced superconducting phase coherence through MID-IR excitation in optimally doped Y-Bi2212
2018
Optimally doped cuprate superconductors are characterized by the presence of superconducting fluctuations in a relatively large temperature region above the critical transition temperature. We reveal here that the effect of thermal disorder, which decreases the condensate phase coherence at equilibrium, can be dynamically contrasted by photoexcitation with ultrashort mid-infrared pulses. In particular, our findings reveal that light pulses with photon energy comparable to the amplitude of the superconducting gap and polarized in plane along the copper-copper direction [110] can dynamically enhance the optical response which is associated to the onset of superconductivity. We propose that th…
Density of electron states in a rectangular lattice under uniaxial stress
2008
The closed analytical expression for the electron density of states function in a rectangular lattice is derived in an elementary way in terms of complete elliptic integrals of the first kind. The lattice can be treated as a deformed square lattice under uniform uniaxial stress (or strain). In contrast to hydrostatic case the uniaxial pressure, say along axis y, modifies a length of the y-bonds while the x-bonds remain intact. It also alters the corresponding tight-binding transfer integral gamma_2 between two y-nearest-neighbours leaving unchanged the gamma_1 for x-nn interactions. Due to stress-induced lowering symmetry of this simple model one can get an insight into the decoupling of it…
Spin-Coupling Topology in the Copper Hexamer Compounds A$_2$Cu$_3$O(SO$_4$)$_3$ (A=Na, K)
2020
The compounds A$_2$Cu$_3$O(SO$_4$)$_3$ (A=Na, K) are characterized by copper hexamers which are weakly coupled to realize antiferromagnetic order below TN=3 K. They constitute novel quantum spin systems with S=1 triplet ground-states. We investigated the energy-level splittings of the copper hexamers by inelastic neutron scattering experiments covering the entire range of the magnetic excitation spectra. The observed transitions are governed by very unusual selection rules which we ascribe to the underlying spin-coupling topology. This is rationalized by model calculations which allow an unambiguous interpretation of the magnetic excitations concerning both the peak assignments and the natu…
Semi-local density functional for the exchange-correlation energy of electrons in two dimensions
2010
We present a practical and accurate density functional for the exchange-correlation energy of electrons in two dimensions. The exchange part is based on a recent two-dimensional generalized-gradient approximation derived by considering the limits of small and large density gradients. The fully local correlation part is constructed following the Colle-Salvetti scheme and a Gaussian approximation for the pair density. The combination of these expressions is shown to provide an efficient density functional to calculate the total energies of two-dimensional electron systems such as semiconductor quantum dots. Excellent performance of the functional with respect to numerically exact reference da…
A different look at the spin state of Co$^{3+}$ ions in CoO$_{5}$ pyramidal coordination
2003
Using soft-x-ray absorption spectroscopy at the Co-$L_{2,3}$ and O-$K$ edges, we demonstrate that the Co$^{3+}$ ions with the CoO$_{5}$ pyramidal coordination in the layered Sr$_2$CoO$_3$Cl compound are unambiguously in the high spin state. Our result questions the reliability of the spin state assignments made so far for the recently synthesized layered cobalt perovskites, and calls for a re-examination of the modeling for the complex and fascinating properties of these new materials.
Current driven insulator-to-metal transition without Mott breakdown in Ca$_2$RuO$_4$
2023
The electrical control of a material's conductivity is at the heart of modern electronics. Conventionally, this control is achieved by tuning the density of mobile charge carriers. A completely different approach is possible in Mott insulators such as Ca$_2$RuO$_4$, where an insulator-to-metal transition (IMT) can be induced by a weak electric field or current. This phenomenon has numerous potential applications in, e.g., neuromorphic computing. While the driving force of the IMT is poorly understood, it has been thought to be a breakdown of the Mott state. Using in operando angle-resolved photoemission spectroscopy, we show that this is not the case: The current-driven conductive phase ari…
Magnetic-field-induced reentrance of Fermi-liquid behavior and spin-lattice relaxation rates in YbCu_{5-x}Au_x
2009
A strong departure from Landau-Fermi liquid (LFL) behavior have been recently revealed in observed anomalies in both the magnetic susceptibility $\chi$ and the muon and $\rm ^{63}Cu$ nuclear spin-lattice relaxation rates $1/T_1$ of ${\rm {YbCu_{5-x}Au_x}}$ ($x=0.6$). We show that the above anomalies along with magnetic-field-induced reentrance of LFL properties are indeed determined by the scaling behavior of the quasiparticle effective mass. We obtain the scaling behavior theoretically utilizing our approach based on fermion condensation quantum phase transition (FCQPT) notion. Our theoretical analysis of experimental data on the base of FCQPT approach permits not only to explain above two…
Combined investigation of collective amplitude and phase modes in a quasi-one-dimensional charge-density-wave system over a wide spectral range
2023
We investigate experimentally both the amplitude and phase channels of the collective modes in the quasi-1D charge-density-wave (CDW) system, K0.3MoO3, by combining (i) optical impulsive-Raman pump-probe and (ii) terahertz time-domain spectroscopy (THz-TDS), with high resolution and a detailed analysis of the full complex-valued spectra in both cases. This allows an unequivocal assignment of the observed bands to CDW modes across the THz range up to 9 THz. We revise and extend a time-dependent Ginzburg-Landau model to account for the observed temperature dependence of the modes, where the combination of both amplitude and phase modes allows one to robustly determine the bare-phonon and elec…
Strain dependence of antiferromagnetic interface coupling in La0.7Sr0.3MnO3/SrRuO3 superlattices
2014
We have investigated the magnetic response of La0.7Sr0.3MnO3/SrRuO3 superlattices to biaxial in-plane strain applied in-situ. Superlattices grown on piezoelectric substrates of 0.72PbMg1/3Nb2/3O3-0.28PbTiO3(001) (PMN-PT) show strong antiferromagnetic coupling of the two ferromagnetic components. The coupling field of mu0HAF = 2.8 T is found to decrease by deltaHAF/delta epsilon ~ -520 mT %-1 under reversible biaxial strain mu0HAF at 80 K in a [La0.7Sr0.3MnO3(22)/SrRuO3(55)]15 superlattice. This reveals a significant strain effect on interfacial coupling. The applied in-plane compression enhances the ferromagnetic order in the manganite layers which are under as-grown tensile strain. It is t…