Search results for "Climate"
showing 10 items of 4934 documents
Overview paper: New insights into aerosol and climate in the Arctic
2019
Motivated by the need to predict how the Arctic atmosphere will change in a warming world, this article summarizes recent advances made by the research consortium NETCARE (Network on Climate and Aerosols: Addressing Key Uncertainties in Remote Canadian Environments) that contribute to our fundamental understanding of Arctic aerosol particles as they relate to climate forcing. The overall goal of NETCARE research has been to use an interdisciplinary approach encompassing extensive field observations and a range of chemical transport, earth system, and biogeochemical models. Several major findings and advances have emerged from NETCARE since its formation in 2013. (1) Unexpectedly high summer…
Influence of vessel characteristics and atmospheric processes on the gas and particle phase of ship emission plumes: in situ measurements in the Medi…
2020
A total of 252 emission plumes of ships operating in the Mediterranean Sea and around the Arabian Peninsula were investigated using a comprehensive dataset of gas- and submicron-particle-phase properties measured during the 2-month shipborne AQABA (Air Quality and Climate Change in the Arabian Basin) field campaign in summer 2017. The post-measurement identification of the corresponding ship emission events in the measured data included the determination of the plume sources (up to 38 km away) as well as the plume ages (up to 115 min) and was based on commercially available historical records of the Automatic Identification System. The dispersion lifetime of chemically inert C…
Enhancements of the refractory submicron aerosol fraction in the Arctic polar vortex: feature or exception ?
2014
In situ measurements with a four-channel stratospheric condensation particle counter (CPC) were conducted at up to 20 km altitude on board the aircraft M-55 Geophysica from Kiruna, Sweden, in January through March (EUPLEX 2003, RECONCILE 2010) and in December (ESSenCe 2011). During all campaigns air masses from the upper stratosphere and mesosphere were subsiding inside the Arctic winter vortex, thus initializing a transport of refractory aerosol into the lower stratosphere (Θ 3 were generally detected. Up to 8 of these 11 particles per cm3 were found to contain thermo-stable (at 250 °C) residuals with diameters of 10 nm to about 1 μm. Particle mixing ratios (150 mg−1) and fractions of non-…
Recent progress in understanding physical and chemical properties of African and Asian mineral dust
2011
International audience; This paper presents a review of recently acquired knowledge on the physico-chemical properties of mineral dust from Africa and Asia based on data presented and discussed during the Third International Dust Workshop, held in Leipzig (Germany) in September 2008. Various regional field experiments have been conducted in the last few years, mostly close to source regions or after short-range transport. Although significant progress has been made in characterising the regional variability of dust properties close to source regions, in particular the mineralogy of iron and the description of particle shape and mixing state, difficulties remain in estimating the range of va…
On the radiative impact of aerosols on photolysis rates: comparison of simulations and observations in the Lampedusa island during the ChArMEx/ADRIME…
2016
The Mediterranean basin is characterized by large concentrations of aerosols from both natural and anthropogenic sources. These aerosols affect tropospheric photochemistry by modulating the photolytic rates. Three simulations of the atmospheric composition at basin scale have been performed with the CHIMERE chemistry-transport model for the period from 6 June to 15 July 2013 covered by the ADRIMED campaign, a campaign of intense measurements in the western Mediterranean basin. One simulation takes into account the radiative effect of the aerosols on photochemistry, the second one does not, and the third one is designed to quantify the model sensitivity to a bias in the ozone column. These s…
Airborne observations of far-infrared upwelling radiance in the Arctic
2016
Abstract. The first airborne measurements of the Far-InfraRed Radiometer (FIRR) were performed in April 2015 during the panarctic NETCARE campaign. Vertical profiles of spectral upwelling radiance in the range 8–50 μm were measured in clear and cloudy conditions from the surface up to 6 km. The clear-sky profiles highlight the strong dependence of radiative fluxes to the temperature inversion typical of the Arctic. Measurements acquired for total column water vapor from 1.5 to 10.5 mm also underline the sensitivity of the far-infrared greenhouse effect to specific humidity. The cloudy cases show that optically thin ice clouds increase the cooling rate of the atmosphere by a factor up to thr…
Titan's 3-micron spectral region from ISO high-resolution spectroscopy
2006
Abstract The near-infrared spectrum of Titan, Saturn's largest moon and one of the Cassini/Huygens' space mission primary targets, covers the 0.8 to 5 micron region in which it shows several weak CH 4 absorption regions, and in particular one centered near 2.75 micron. Due to the interference of telluric absorption, only part of this window region (2.9–3.1 μm) has previously been observed from the ground [Noll, K.S., Geballe, T.R., Knacke, R., Pendleton, F., Yvonne, J., 1996. Icarus 124, 625–631; Griffith, C.A., Owen, T., Miller, G.A., Geballe, T., 1998. Nature 395, 575–578; Griffith, C.A., Owen, T., Geballe, T.R., Rayner, J., Rannou, P., 2003. Science 300, 628–630; Geballe, T.R., Kim, S.J.…
First results of the Piton de la Fournaise STRAP 2015 experiment: multidisciplinary tracking of a volcanic gas and aerosol plume
2016
Abstract. The STRAP (Synergie Transdisciplinaire pour Répondre aux Aléas liés aux Panaches volcaniques) campaign was conducted in 2015 to investigate the volcanic plumes of Piton de La Fournaise (La Réunion, France). For the first time, measurements at the local (near the vent) and at the regional scales around the island were conducted. The STRAP 2015 campaign has become possible thanks to a strong cross-disciplinary collaboration between volcanologists and meteorologists. The main observations during four eruptive periods (85 days) are summarized. They include the estimates of SO2, CO2 and H2O emissions, the altitude of the plume at the vent and over different areas of La Réunion Island, …
Error propagation from line parameters to spectra simulations. Illustration on high temperature methane.
2010
Astrophysical investigations generally need both complete and accurate spectroscopic databases. Despite continuous efforts in experimental and theoretical spectroscopic investigations, the lack of data in some spectral regions of interest is one of the main limitation of the presently available spectroscopic databases. Unfortunately information about missing data relevant to specific experimental conditions is rarely directly accessible from spectroscopic databases (focusing naturally on available data). Such information relies essentially on theoretical investigations which are equally limited to the present state of the art of modelling. The purpose of the talk is to show how multi-resolu…
Titan's surface and atmosphere from Cassini/VIMS data with updated methane opacity
2013
International audience; We present an analysis of Titan data acquired by the Cassini Visual and Infrared Mapping Spectrometer (VIMS), making use of recent improvements in methane spectroscopic parameters in the region 1.3-5.2 μm. We first analyzed VIMS spectra covering a 8 × 10-km2 area near the Huygens landing site in order to constrain the single scattering albedo (ω0) of the aerosols over all of the VIMS spectral range. Our aerosol model agrees with that derived from Huygens Probe Descent Imager/Spectral Radiometer (DISR) in situ measurements below 1.6 μm. At longer wavelengths, ω0 steadily decreases from 0.92 at 1.6 μm to about 0.70 at 2.5 μm and abruptly drops to about 0.50 near 2.6 μm…