Search results for "Clusters"
showing 10 items of 1274 documents
Linear-scaling self-consistent field theory based molecular dynamics: application to C60buckyballs colliding with graphite
2018
In this work, we investigate the collision of a C fullerene with graphite using large-scale molecular dynamics simulations, where the interatomic forces are computed ‘on-the-fly’ by means of self-c...
Compton scattering off nucleons near threshold
2008
The energy dependence of the magnetic polarizability β has been evaluated by use of the delta resonance in the s- and u-channel of the Compton scattering amplitude. It was the idea to extract the influence of higher order terms (higher than ω2, ω = |k| being the photon energy) in the analysis of the polarizability. The static paramagnetic polarizability βPara(0) has been substituted by an energy dependent βδPara(k) and the result is compared with experimental data.
Time-dependent density-functional theory of strong-field ionization of atoms by soft x rays
2014
Under the terms of the Creative Commons Attribution License 3.0 (CC-BY).-- et al.
New Insight into the Cluster Structure of $^9$Be by Reactions with Deuteron Beam
2018
International audience; Angular distributions of protons, deuterons, tritons, and alpha particles emitted in the reaction 2H+9Be at Elab=19.5, 25, and 35 MeV were measured to study the structure of 9Be, especially to shed light on the internal clusters and possible cluster transfer of 5He. The experiments were performed at sufficiently high energies to ensure suppression of compound nucleus contribution. Thus, the direct reaction mechanism should be mainly responsible for the measured five-nucleon transfer cross section. The analysis suggests a significant contribution of simultaneous five-nucleon transfer in the reaction channel 9Be (d,4He) 7Li.
STABILITY AND SPECTRA OF SMALL 3He-4He CLUSTERS
2005
Diffusion Monte Carlo calculations have been systematically performed to analyze the stability of small mixed 3 He -4 He clusters, as well as their excitation spectra. The picture that emerges is that of systems with strong shell effects whose binding and excitation energies are essentially determined by the monopole properties of an effective Hamiltonian.
Hyperfine transitions in the first overtone mode of hydrogen deuteride
2020
Beyond the metrology and computational challenges associated with molecular hydrogen, key data are expected to assess the physics of simple molecular systems, and even the new physics beyond the standard model. To assist the deciphering of Doppler-free spectra obtained at very high accuracy ($\ensuremath{\sim}{10}^{\ensuremath{-}9})$, we report on hyperfine transitions of HD in the lowest vibrational levels of the ground electronic state. Using the spin-rotation, nuclear spin-spin, and quadrupolar hyperfine couplings determined by means of high-level quantum-chemical calculations, the hyperfine energy levels and the associated line intensity have been obtained by using tensorial momentum al…
Rotational echoes as a tool for investigating ultrafast collisional dynamics of molecules
2019
We show that recently discovered rotational echoes of molecules provide an efficient tool for studying collisional molecular dynamics in high-pressure gases. Our study demonstrates that rotational echoes enable the observation of extremely fast collisional dissipation, at timescales of the order of a few picoseconds, and possibly shorter. The decay of the rotational alignment echoes in ${\mathrm{CO}}_{2}$ gas and ${\mathrm{CO}}_{2}\text{\ensuremath{-}}\mathrm{He}$ mixture up to 50 bar was studied experimentally, delivering collision rates that are in good agreement with the theoretical expectations. The suggested measurement protocol may be used in other high-density media, and potentially …
Ultrafast hybrid plasmonics
2008
Abstract We review our recent studies of electromagnetic coupling and associated temporal dynamics of molecular excitations with plasmonic resonances supported by either localized or extended planar geometries. We focus on coherent interactions between plasmon resonances and molecular excitations, which are experimentally challenging due to the very short (∼10–100 fs) coherence times of plasmons. Recent experimental results and theoretical analysis for observing and controlling coherences between molecular excitations and plasmonic polarizations are shown. Advances will explore new directions in ultrafast coherent control of molecular excited states and energy dissipation processes, as well…
Piecewise static Hamiltonian for an atom in strong laser field
2009
We show that it is possible to use a piecewise constant Hamiltonian to describe the main features of the dynamics of an atom interacting with a laser field. In particular we show that using this approximation we are able to give a good description of the ionization signal, of the HHG spectra and of the attosecond pulses generated by the radiating electron. Finally, we give an explicit formula to evaluate the ionization rate in the time dependent laser field. This formula, which is a generalization of the Landau formula for the ionization rate of an atom in a static electric field, fairly well reproduces the numerical ionization rates for a broad range of laser frequency and intensity. The m…
The Gaia-ESO Survey: Catalogue of Hα emission stars
2015
We discuss the properties of Hα emission stars across the sample of 22035 spectra from the Gaia-ESO Survey internal data release, observed with the GIRAFFE instrument and largely belonging to stars in young open clusters. Automated fits using two independent Gaussian profiles and a third component that accounts for the nebular emission allow us to discern distinct morphological types of Hα line profiles with the introduction of a simplified classification scheme. All in all, we find 3765 stars with intrinsic emission and sort their spectra into eight distinct morphological categories: single-component emission, emission blend, sharp emission peaks, double emission, P-Cygni, inverted P-Cygni…