Search results for "Coherence"
showing 10 items of 905 documents
Anomalous thermalization of nonlinear wave systems
2010
We report theoretically and experimentally in an optical system a process of anomalous thermalization of one-dimensional nonlinear Hamiltonian waves. It is characterized by an irreversible evolution of the waves towards a specific equilibrium state of a fundamental different nature than the expected thermodynamic equilibrium state. A kinetic approach of the problem reveals that this phenomenon is due to the existence of a local invariant in frequency space. A novel family of equilibrium distributions is discovered, which is found in quantitative agreement with the numerical simulations.
Microscopic description of dissipative dynamics of a level-crossing transition
2011
We analyze the effect of a dissipative bosonic environment on the Landau-Zener-Stuckelberg-Majorana (LZSM) level crossing model by using a microscopic approach to derive the relevant master equation. For an environment at zero temperature and weak dissipation our microscopic approach confirms the independence of the survival probability on the decay rate that has been predicted earlier by the simple phenomenological LZSM model. For strong decay the microscopic approach predicts a notable increase of the survival probability, which signals dynamical decoupling of the initial state. Unlike the phenomenological model our approach makes it possible to study the dependence of the system dynamics…
Reconstruction of time-dependent coefficients: a check of approximation schemes for non-Markovian convolutionless dissipative generators
2010
We propose a procedure to fully reconstruct the time-dependent coefficients of convolutionless non-Markovian dissipative generators via a finite number of experimental measurements. By combining a tomography based approach with a proper data sampling, our proposal allows to relate the time-dependent coefficients governing the dissipative evolution of a quantum system to experimentally accessible quantities. The proposed scheme not only provides a way to retrieve full information about potentially unknown dissipative coefficients but also, most valuably, can be employed as a reliable consistency test for the approximations involved in the theoretical derivation of a given non-Markovian convo…
Emergence of Coherence through Variation of Intermolecular Distances in a Series of Molecular Dimers
2015
Quantum coherences between electronically excited molecules are a signature of entanglement and play an important role for energy transport in molecular assemblies. Here we monitor and analyze for a homologous series of molecular dimers embedded in a solid host the emergence of coherence with decreasing intermolecular distance by single-molecule spectroscopy and quantum chemistry. Coherent signatures appear as an enhancement of the purely electronic transitions in the dimers which is reflected by changes of fluorescence spectra and lifetimes. Effects that destroy the coherence are the coupling to the surroundings and to vibrational excitations. Complementary information is provided by excit…
Catastrophic process of coherence degradation
2018
We predict a catastrophic process of coherence degradation characterized by a virtually unlimited spectral broadening of the waves. This effect is described by self-similar solutions of the kinetic equations inherent to the wave turbulence theory.
Temporal dynamics of incoherent waves in noninstantaneous response nonlinear Kerr media
2012
International audience; We consider the temporal evolution of an incoherent optical wave that propagates in a noninstantaneous response nonlinear medium, such as single mode optical fibers. In contrast with the expected Raman-like spectral redshift due to a delayed nonlinear response, we show that a highly noninstantaneous response leads to a genuine modulational instability of the incoherent optical wave. We derive a Vlasov-like kinetic equation that provides a detailed description of this process of incoherent modulational instability in the temporal domain.
Rogue waves, rational solitons and wave turbulence theory
2011
International audience; Considering a simple one dimensional nonlinear Schrödinger optical model, we study the existence of rogue wave events in the highly incoherent state of the system and compare them with the recently identified hierarchy of rational soliton solutions. We show that rogue waves can emerge in the genuine turbulent regime and that their coherent deterministic description provided by the rational soliton solutions is compatible with an accurate statistical description of the random wave provided by the wave turbulence theory. Furthermore, the simulations reveal that even in the weakly nonlinear regime, the nonlinearity can play a key role in the emergence of an individual r…
Field-free molecular alignment of CO2 mixtures in presence of collisional relaxation
2008
The present work explores the extension of the concept of short-pulse-induced alignment to dissipative environments within quantum mechanical density matrix formalism (Liouville equation) from the weak to the strong field regime. This is illustrated within the example of the CO2 molecule in mixture with Ar and He, at room temperature, for which a steep decrease of the alignment is observed at moderate pressure because of the collisional relaxation. The field-free alignment is measured by a polarization technique where the degree of alignment is monitored in the time domain by measuring the resulting transient birefringence with a probe pulse Raman induced polarization spectroscopy (RIPS) Co…
Real-time optical spectrum analyzers operating with spectrally incoherent broadband continuous-wave light source
2007
On the framework of coherence theory we discuss the averaged temporal intensity output provided by real-time optical Fourier transformers when the spectral line shape of the stationary source is considered. Some numerical examples are given and the deviations from perfectly monochromatic sources are pointed out.
Atomic Coherence Effects in Doppler-Broadened Three-Level Systems with Standing-Wave Drive
2001
We study atomic coherence effects (e.g., electromagnetically induced transparency, EIT, and amplification without inversion, AWI) for a probe travelling-wave (TW) laser field in closed Doppler-broadened three-level systems driven by a standingwave (SW) laser field of moderate intensity (its Rabi frequencies are smaller than the Doppler width of the driven transition). We show that probe windows of transparency occur only for values of the probe to drive field frequency ratio R close to half integer values. For optical transitions and typical values of Doppler broadening for atoms in a vapor cell, we show that for R > 1 a SW drive field is appreciably more efficient than a TW drive in induci…