Search results for "DEGRADATION"

showing 10 items of 1208 documents

Effect of Nanodiamonds on Structure and Durability of Polyethylene Oxide-Based Nanocomposites

2016

Polymer-based nanocomposites containing nanodiamonds (NDs) are attractive multifunctional materials with a growing range of applications. In this work, in the frame of developing completely biocompatible systems, nanocomposites based on polyethylene oxide (PEO) and different amount of NDs have been formulated through melt mixing and fully characterized. In particular, the reinforcement effect of NDs in PEO has been probed through tensile tests, and the rheological response of PEO-based nanocomposites as a function of the nanoparticles amount has been investigated and discussed. The obtained results show that the presence of well-distributed NDs strengthens the mechanical performance of the …

Materials scienceArticle SubjectNanoparticle02 engineering and technology010402 general chemistry01 natural sciencesDurabilityCrystallinitylcsh:Technology (General)Ultimate tensile strengthGeneral Materials ScienceComposite materialPhotodegradationPolyethylene Oxidechemistry.chemical_classificationNanocompositeNanocompositePolymerAdhesion021001 nanoscience & nanotechnologyAccelerated aging0104 chemical sciencesSettore ING-IND/22 - Scienza E Tecnologia Dei Materialichemistrylcsh:T1-995Materials Science (all)0210 nano-technologyNanodiamondJournal of Nanomaterials
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Design of highly efficient porous carbon foam cathode for electro-Fenton degradation of antimicrobial sulfanilamide

2021

Abstract This work investigated, for the first time, the potential of novel biomass derived carbon foam as a suitable and efficient electrocatalytic material (as cathode) for in-situ hydrogen peroxide (H2O2) production and its applicability in electro-Fenton (EF) approach for oxidizing organic pollutants. The carbon foam cathode was prepared by polymerization and carbonization of sucrose at high temperature. The as-prepared carbon foam consists of highly porous and extremely light structure with interconnected spherical cells. It exhibited excellent electrocatalytic properties such as high conductivity, relatively high redox current and several active-sites for producing oxidizing species, …

Materials scienceCarbonizationProcess Chemistry and TechnologyCarbon nanofoam02 engineering and technologyElectrolyte010402 general chemistry021001 nanoscience & nanotechnology01 natural sciencesRedoxCatalysisCathode0104 chemical scienceslaw.inventionchemistry.chemical_compoundchemistryChemical engineeringlawOxidizing agentDegradation (geology)0210 nano-technologyHydrogen peroxideGeneral Environmental ScienceApplied Catalysis B: Environmental
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TiO2/ORMOSIL Thin Films Doped with Phthalocyanine Dyes:  New Photocatalytic Devices Activated by Solar Light

2008

WOS: 000253222200065

Materials scienceChemical substancePhthalocyaninesThin filmsPhotochemistryOrmosillaw.inventionDegradationchemistry.chemical_compoundMagazinelawSol-gel processPhotocatalysisPhysical and Theoretical ChemistryThin filmDopingsol−gel TiO2/organosilica films phthalocyaninesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsGeneral EnergychemistryPhotocatalysisPhthalocyanineTitanium dioxideIrradiationScience technology and societyThe Journal of Physical Chemistry C
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Preparation, characterization and in vitro antimicrobial activity of ampicillin-loaded polyethylcyanoacrylate nanoparticles.

1998

In this paper, the experimental conditions for preparing ampicillin-loaded polyethylcyanoacrylate (PECA) nanoparticles are described. The effects of drug concentration and surfactant type in the polymerization medium on the particle size distribution and loading capacity were studied. The results of these studies show that only the type of surfactant has an impact on the nanoparticle dimensions. The release rate of ampicillin from PECA nanoparticles at pH 7.4 (extracellular value pH) performed either with and without esterases, show that the drug release is considerably increased in the presence of these exzymes. The results of drug release study at pH 1.1 (simulated gastric juice) are very…

Materials scienceChemistry PharmaceuticalBiophysicsNanoparticleBioengineeringBiocompatible MaterialsMicrobial Sensitivity TestsPenicillinsPoloxamerBiomaterialsSurface-Active AgentsPulmonary surfactantDrug StabilityExtracellularOrganic chemistryCyanoacrylatesDrug CarriersChromatographyBiomaterialBiodegradationAntimicrobialIn vitroPolymerizationMechanics of MaterialsDelayed-Action PreparationsCeramics and CompositesAmpicillinBiomaterials
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Cytotoxicity of Metal and Semiconductor Nanoparticles Indicated by Cellular Micromotility

2009

In the growing field of nanotechnology, there is an urgent need to sensitively determine the toxicity of nanoparticles since many technical and medical applications are based on controlled exposure to particles, that is, as contrast agents or for drug delivery. Before the in vivo implementation, in vitro cell experiments are required to achieve a detailed knowledge of toxicity and biodegradation as a function of the nanoparticles' physical and chemical properties. In this study, we show that the micromotility of animal cells as monitored by electrical cell-substrate impedance analysis (ECIS) is highly suitable to quantify in vitro cytotoxicity of semiconductor quantum dots and gold nanorods…

Materials scienceContrast MediaMetal NanoparticlesGeneral Physics and AstronomyNanoparticleNanotechnologyDrug Delivery SystemsIn vivoQuantum DotsMicroscopyElectric ImpedanceAnimalsHumansNanotechnologyGeneral Materials ScienceCytotoxicityFluorescent DyesGeneral EngineeringIn vitroBiodegradation EnvironmentalSemiconductorsMetalsQuantum dotDrug deliveryNanoparticlesNanorodGoldACS Nano
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Halloysite nanotubes/pluronic nanocomposites for waterlogged archeological wood: thermal stability and X-ray microtomography

2020

Filling a polymer with halloysite nanotubes is considered a promising strategy to generate nanocomposites with tailored physicochemical properties. We have focused our attention on pluronic block copolymer/halloysite nanocomposites prepared by melt blending. The effect of composition on thermal stability and polymer crystallinity was investigated by thermogravimetry and differential scanning calorimetry. Electron microscopy was used to monitor the nanoparticle distribution in the polymeric matrix. The pluronic thermal stability is reduced by the clay nanoparticles. Concerning the polymer crystallinity, it is slightly decreased even if the melting temperature is lowered by halloysite. Furthe…

Materials scienceCrystallization of polymersNanoparticleengineering.materialHalloysiteNanocompositesDifferential scanning calorimetryThermal stabilityPhysical and Theoretical Chemistrychemistry.chemical_classificationNanocompositeNanocompositeHalloysite; Nanocomposites; Nanotube; Pluronic; Restoration; Thermal degradation; Waterlogged wood; X-ray microtomography;HalloysitePluronicPolymerCondensed Matter PhysicsArchaeologyNanotubeThermogravimetrychemistryX-ray microtomographyRestorationThermal degradationengineeringSettore L-ANT/10 - Metodologie della Ricerca ArcheologicaWaterlogged woodJournal of Thermal Analysis and Calorimetry
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Preparation of Sm-loaded brookite TiO2 photocatalysts

2011

Abstract Pure and Sm-loaded brookite nanoparticles and thin films were prepared using TiCl4 as precursor of TiO2. The samples were characterized by X-ray diffraction (XRD), specific surface area (SSA) determination, diffuse reflectance spectroscopy (DRS) and photoluminescence (PL) measurements. The photocatalytic activity of the powders was investigated by employing the photodegradation of 4-nitrophenol in a liquid–solid system whilst the photoreactivity of the films was tested by evaluating the rate of degradation of 2-propanol in a gas–solid system. Loading with Sm resulted in a significant improvement of the photoreactivity of brookite and the beneficial effect was attributed to an incre…

Materials scienceDiffuse reflectance infrared fourier transformLoaded brookite2Mineralogychemistry.chemical_elementNanoparticleCatalysisSpecific surface areaBrookiteTiOTiO2PhotocatalysisPhotodegradationPhotocatalysis TiO2 Brookite Loaded brookiteBrookiteGeneral ChemistryBrookite; Loaded brookite; Photocatalysis; TiO; 2;Samariumchemistryvisual_artX-ray crystallographyvisual_art.visual_art_mediumPhotocatalysisSettore CHIM/07 - Fondamenti Chimici Delle TecnologieNuclear chemistry
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Absolute crystallinity and photocatalytic activity of brookite TiO2 samples

2017

Abstract This study reports a method to determine the absolute crystallinity of partly crystalline brookite TiO2 photocatalysts. A natural, a commercial and various home-prepared brookite powders were characterized by X-ray diffraction analysis, Raman spectroscopy, scanning electron microscopy, UV–vis diffuse reflectance spectroscopy and nitrogen adsorption measurements. The absolute crystallinity was calculated from the ratio between the full width at half maximum intensity of the (121) X-ray diffraction peaks of the brookite samples and the (111) peak of CaF2 as internal standard. The photocatalytic activity of the powders was tested employing the photodegradation of 4-nitrophenol as well…

Materials scienceDiffuse reflectance infrared fourier transformScanning electron microscopeInorganic chemistry02 engineering and technology010402 general chemistry01 natural sciencesCatalysisCrystallinitysymbols.namesakePhotocatalysiBrookitePhotodegradationCrystallinityGeneral Environmental ScienceBrookiteProcess Chemistry and Technology021001 nanoscience & nanotechnology0104 chemical sciencesFull width at half maximumSettore ING-IND/22 - Scienza E Tecnologia Dei Materialivisual_artPhotocatalysisvisual_art.visual_art_mediumsymbolsCalcinationSettore CHIM/07 - Fondamenti Chimici Delle Tecnologie0210 nano-technologyRaman spectroscopyNuclear chemistry
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Enhanced Solar Light Photocatalytic Activity of Ag Doped TiO2–Ag3PO4 Composites

2020

Composites comprised of Ag3PO4 and bare TiO2 (TiO2@Ag3PO4) or silver doped TiO2 (Ag@TiO2&ndash

Materials scienceDiffuse reflectance infrared fourier transformheterojunction4–nitrophenol degradationScanning electron microscope3General Chemical Engineering42Sol-gel synthesisInfrared spectroscopyAg@TiO2–Ag3PO4 heterojunctionPOArticlelcsh:Chemistrysolar photocatalysissol–gel synthesisSpecific surface areaGeneral Materials ScienceComposite materialFourier transform infrared spectroscopyPrecipitation (chemistry)4-nitrophenol degradationAg@TiODoping4-nitrophenol degradation; Ag@TiO; 2; -Ag; 3; PO; 4; heterojunction; Sol-gel synthesis; Solar photocatalysis-Aglcsh:QD1-999Solar photocatalysisPhotocatalysisAg@TiO<sub>2</sub>–Ag<sub>3</sub>PO<sub>4</sub> heterojunctionNanomaterials
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Ester-Ester Exchange Reactions of Aliphatic Polyesters

1979

Abstract The kinetics of ester-ester exchange reactions of poly(ethylene adipate) and poly(trimethylene adipate) at 312°C and in the absence of a solvent and catalysts has been reported previously. Independent investigations of the thermal degradation reactions of these polyesters under high vacuum have shown that pyrolysis already starts above 270°C. An ester-ester exchange mechanism via a reversible thermal degradation reaction is proposed.

Materials scienceEthyleneKineticsGeneral EngineeringCatalysisSolventPolyesterchemistry.chemical_compoundchemistryAdipatePolymer chemistryOrganic chemistryDegradation (geology)PyrolysisJournal of Macromolecular Science: Part A - Chemistry
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