Search results for "Doppler broadening"
showing 10 items of 66 documents
Possible Precision Far—Infrared Spectroscopy on Trapped Ions
1990
One of the necessary conditions for very high resolution spectroscopy is the existence of long-living energy levels between which transitions can be induced by tunable electromagnetic radiation. Moreover the observation time of the particles under investigation should be sufficiently long, and perturbing effects like Doppler broadening and collisions should be very small. All this leads to the technique of trapped ion spectroscopy which offers all the required conditions. It uses the confinement of charged particles to a very small volume in space under ultrahigh vacuum conditions either by application of a r.f. voltage and a small additional d.c. bias to an arrangement of three electrodes …
Supercontinuum generation in silicon waveguides based on optical wave-breaking
2014
We theoretically find the third order dispersion that optimizes the spectral broadening induced by optical wave-breaking. It produces supercontinuum spectra spanning beyond 2=3 of an octave in a silicon waveguide pumping at 1550 nm.
Second harmonic generation and beam cleaning in optically poled multimode graded-index fibers
2017
Recent experimental results have confirmed that nonlinear effects in multimode graded-index (MM-GRIN) fibers lead to a wealth of observable spatiotemporal effects. In spite of the large number of modes supported by the fiber, by increasing the input power the transverse profile evolves in a clean bell-shaped beam [1, 2]. Next, the input laser line experiences a strong spectral broadening and Geometric Parametric Instability (GPl) peaks are observed [3].
Spectral broadening of the Soret band in myoglobin: an interpretation by the full spectrum of low-frequency modes from a normal modes analysis.
2005
In this work the temperature dependence of the Soret band line shape in carbon-monoxy myoglobin is re-analyzed by using both the full correlator approach in the time domain and the frequency domain approach. The new analyses exploit the full density of vibrational states of carbon-monoxy myoglobin available from normal modes analysis, and avoid the artificial division of the entire set of vibrational modes coupled to the Soret transition into "high-frequency" and "low-frequency" subsets; the frequency domain analysis, however, makes use of the so-called short-times approximation, while the time domain one avoids it. Time domain and frequency domain analyses give very similar results, thus s…
Differences between Bond Lengths in Biogenic and Geological Calcite
2010
8 pages; International audience; We used high-resolution neutron powder diffraction to accurately measure the atomic positions and bond lengths in biogenic and geological calcite. A special procedure for data analysis was developed in order to take into account the considerable amounts of magnesium present in all the investigated samples. As a result, in biogenic calcite we found some atomic bonds to have significantly different lengths as compared to those in geological calcite, after the contribution of magnesium is accounted for. The maximum effect (elongation up to 0.7%) was found for the C−O bonds. We also analyzed changes in frequencies and spectral widths of normal vibrations of carb…
Performance of the Advanced GAmma Tracking Array at GANIL
2020
The performance of the Advanced GAmma Tracking Array (AGATA) at GANIL is discussed, on the basis of the analysis of source and in-beam data taken with up to 30 segmented crystals. Data processing is described in detail. The performance of individual detectors are shown. The efficiency of the individual detectors as well as the efficiency after $\gamma$-ray tracking are discussed. Recent developments of $\gamma$-ray tracking are also presented. The experimentally achieved peak-to-total is compared with simulations showing the impact of back-scattered $\gamma$ rays on the peak-to-total in a $\gamma$-ray tracking array. An estimate of the achieved position resolution using the Doppler broadeni…
Positron annihilation study of spin-crossover in [Fe x Zn1−x (ptz)6](BF4)2 single crystals
1994
Positron lifetime measurements were carried out on [Fe x Zn1−x (ptz)6](BF4)2 single crystals in the temperature range of 72–300 K. Complementary Doppler broadening spectra were also recorded at room temperature. The probability of the formation of o-Ps (lifetime 500–1400 ps) was between 10–30%. Both the spin density and the lattice parameters of the sample affected the lifetime of o-Ps through the ortho-para conversion and the pick-off annihilation, respectively. The positron annihilation technique proved to be a sensitive detector of the spin-crossover5T2 ↔1A1 and of the concomitant phase transformation.
Atomic spectroscopy studies of short-lived isotopes and nuclear isomer separation with the ISOLDE RILIS
2002
The Resonance Ionization Laser Ion Source (RILIS) at the ISOLDE on-line isotope separator is based on the selective excitation of atomic transitions by tunable laser radiation. Ion beams of isotopes of 20 elements have been produced using the RILIS setup. Together with the mass separator and a particle detection system it represents a tool for high-sensitive laser spectroscopy of short-lived isotopes. By applying narrow-bandwidth lasers for the RILIS one can study isotope shifts (IS) and hyperfine structure (HFS) of atomic optical transitions. Such measurements are capable of providing data on nuclear charge radii, spins and magnetic moments of exotic nuclides far from stability. Although t…
First demonstration of Doppler-free 2-photon in-source laser spectroscopy at the ISOLDE-RILIS
2020
Abstract Collinear Doppler-free 2-photon resonance ionization has been applied inside a hot cavity laser ion source environment at CERN-ISOLDE. An injection-seeded Ti:sapphire ring laser was used to generate light pulses with a Fourier-limited linewidth for high-resolution spectroscopy. Using a molybdenum foil as a reflective surface positioned at the end of the target transfer line, rubidium was successfully ionized inside the hot cavity. The results are presented alongside previously obtained data from measurements performed at the RISIKO mass separator at Mainz University, where collinear and perpendicular ionization geometries were tested inside an RFQ ion guide. This work is a pre-curs…
Doppler-broadening of gamma rays following muon capture: search for scalar coupling
2002
Abstract A precision measurement of the 277 keV γ ray produced by capturing muons in gaseous oxygen was performed using high-resolution HPGe detectors. The Doppler-broadened shape of this line is sensitive to the possible admixture into muon capture of genuine scalar interaction. This experiment complements, in the muon sector, in principle, similar ones undertaken recently in nuclear β decay. Using a procedure discussed in earlier papers, a fit to the experimental line-shape allowed us to obtain for the recoil–gamma correlation coefficient the value of a 1 2 =0.096±0.041 (95% CL). The available evaluations of the contributing nuclear matrix elements, performed in the impulse approximation …