Search results for "Dynamics"

showing 10 items of 9782 documents

Elucidating the ligand shell structure and dynamics of Au683MBA32 gold nanocluster using molecular dynamics simulations

2017

Synthesising novel gold nanoparticles and -clusters can be often easier than characterising them, and after experimental analysis many options for the possible molecular formula of the cluster may remain as equally valid options. These options may be investigated by quantum computational means, such as density functional theory, but since DFT includes the electronic interactions, this might take time and excessive effort if the amount of options is large. In this thesis a new way of easing the computational task is introduced by a novel method, that combines a guessing algorithm and molecular dynamics simulations. The algorithm produces possible structures by utilising existing structures o…

ligand layerkultananopartikkelivuorovaikutusgold nanoclusterkultananoklusterinanohiukkasetpintarakenteetmolekyylidynamiikkainteractionssurface structuregold nanoparticlemolecular dynamicskulta
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Virtual screening : development of a novel structure-based method

2013

ligandipohjaiset menetelmätmolekyylimekaniikkanegative image-based screeninglääkeainekehitysrakennepohjaiset menetelmätliganditvirtual screeningmolecular dynamicscomputational drug discoverylääkesuunnittelulääkeaihiotlaskennalliset menetelmätmolekyylidynamiikkavirtuaaliseulontabinding free energy
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Complex dynamics, hidden attractors and continuous approximation of a fractional-order hyperchaotic PWC system

2018

In this paper, a continuous approximation to studying a class of PWC systems of fractionalorder is presented. Some known results of set-valued analysis and differential inclusions are utilized. The example of a hyperchaotic PWC system of fractional order is analyzed. It is found that without equilibria, the system has hidden attractors.

likiarvotFOS: Physical sciencesAerospace EngineeringattraktoritOcean EngineeringDynamical Systems (math.DS)hidden chaotic attractor01 natural sciences010305 fluids & plasmasDifferential inclusion0103 physical sciencesAttractorFOS: MathematicsApplied mathematicsOrder (group theory)Mathematics - Dynamical Systemsdynaamiset systeemitElectrical and Electronic Engineering010301 acousticsMathematicskaaosteoriaContinuous approximationmurtoluvutperiodicity of fractional-order systemPWC system of fractional orderApplied MathematicsMechanical EngineeringNonlinear Sciences - Chaotic DynamicsNonlinear Sciences::Chaotic DynamicsComplex dynamicshyperchaosControl and Systems Engineeringcontinuous approximationapproksimointiChaotic Dynamics (nlin.CD)Nonlinear Dynamics
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Pairwise and higher-order measures of brain-heart interactions in children with temporal lobe epilepsy

2022

Abstract Objective. While it is well-known that epilepsy has a clear impact on the activity of both the central nervous system (CNS) and the autonomic nervous system (ANS), its role on the complex interplay between CNS and ANS has not been fully elucidated yet. In this work, pairwise and higher-order predictability measures based on the concepts of Granger Causality (GC) and partial information decomposition (PID) were applied on time series of electroencephalographic (EEG) brain wave amplitude and heart rate variability (HRV) in order to investigate directed brain-heart interactions associated with the occurrence of focal epilepsy. Approach. HRV and the envelopes of δ and α EEG activity re…

linear predictionBiomedical Engineeringheart rate variabilityBrainHeartElectroencephalographyCellular and Molecular NeuroscienceEpilepsy Temporal LobeSeizuresSettore ING-INF/06 - Bioingegneria Elettronica E InformaticaHumansGranger causality (GC)epilepsyEpilepsies PartialChildinformation dynamics
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The electric properties of ionic solutions: a molecular dynamics (preliminary) study

2011

lipid bilayer ionic solutions molecular dynamics non equilibriumlipid bilayer ionic solution molecula drynamics electric fieldSettore FIS/07 - Fisica Applicata(Beni Culturali Ambientali Biol.e Medicin)
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Dynamics of supercooled confined water measured by deep inelastic neutron scattering

2017

In this paper, we present the results of deep inelastic neutron scattering (DINS) measurements on supercooled water confined within the pores (average pore diameter ~ 20 Å) of a disordered hydrophilic silica matrix obtained through hydrolysis and polycondensation of the alkoxide precursor Tetra-Methyl-Ortho-Silicate via the sol-gel method. Experiments were performed at two temperatures (250 K and 210 K, i.e., before and after the putative liquid–liquid transition of supercooled confined water) on a “wet” sample with hydration h ~ 40% w/w, which is high enough to have water-filled pores but low enough to avoid water crystallization. A virtually “dry” sample at h ~ 7% was also inve…

liquid-liquid transitionMaterials sciencePhysics and Astronomy (miscellaneous)HydrogenThermodynamicschemistry.chemical_element02 engineering and technologyNeutron scatteringKinetic energy01 natural sciencesInelastic neutron scatteringMomentumchemistry.chemical_compoundsilica xerogelconfined water0103 physical sciences010306 general physicsSupercoolingliquid–liquid transitionSettore FIS/07021001 nanoscience & nanotechnologyconfined water; hydrogen mean kinetic energy; liquid–liquid transition; silica xerogel; Physics and Astronomy (miscellaneous)Settore FIS/07 - Fisica Applicata(Beni Culturali Ambientali Biol.e Medicin)chemistryhydrogen mean kinetic energyAlkoxideWater of crystallization0210 nano-technology
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Experimental evidence for a liquid-liquid crossover in deeply cooled confined water.

2014

International audience; In this work we investigate, by means of elastic neutron scattering, the pressure dependence of mean square displacements (MSD) of hydrogen atoms of deeply cooled water confined in the pores of a three-dimensional disordered SiO 2 xerogel; experiments have been performed at 250 and 210 K from atmospheric pressure to 1200 bar. The " pressure anomaly " of supercooled water (i.e., a mean square displacement increase with increasing pressure) is observed in our sample at both temperatures; however, contrary to previous simulation results and to the experimental trend observed in bulk water, the pressure effect is smaller at lower (210 K) than at higher (250 K) temperatur…

liquid-liquid transitionPhase transitionPACS: 64.70.Ja 64.70.pm 25.40.DnMaterials scienceNeutron diffractionGeneral Physics and AstronomyThermodynamicsNeutron scatteringSettore FIS/03 - Fisica Della MateriaPhase TransitionNuclear magnetic resonanceWater Movementsglass transitionElastic neutron scattering[PHYS.COND]Physics [physics]/Condensed Matter [cond-mat]SupercoolingElastic neutron scattering; calorimetry; glass transition; liquid-liquid transitionAtmospheric pressure[SDV.BBM.BS]Life Sciences [q-bio]/Biochemistry Molecular Biology/Structural Biology [q-bio.BM]Calorimetry Differential ScanningWaterSilicon DioxideSettore FIS/07 - Fisica Applicata(Beni Culturali Ambientali Biol.e Medicin)Cold Temperature[SDV.BBM.BS]Life Sciences [q-bio]/Biochemistry Molecular Biology/Biomolecules [q-bio.BM]Neutron DiffractionModels ChemicalGlass transitioncalorimetryHydrophobic and Hydrophilic InteractionsAmbient pressureBar (unit)HydrogenPhysical review letters
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The boson peak of deeply cooled confined water reveals the existence of a low-temperature liquid-liquid crossover.

2014

International audience; The Boson peak of deeply cooled water confined in the pores of a silica xerogel is studied by inelastic neutron scattering at different hydration levels to separate the contributions from matrix, water on the pore surfaces and "internal" water. Our results reveal that at high hydration level, where the contribution from internal water is dominant, the temperature dependence of the Boson peak intensity shows an inflection point at about 225 K. The complementary use of differential scanning calorimetry to describe the thermodynamics of the system allows identifying the inflection point as the signature of a water liquid-liquid crossover.

liquid-liquid transition[SDV.BBM.BS] Life Sciences [q-bio]/Biochemistry Molecular Biology/Structural Biology [q-bio.BM]CrossovereducationGeneral Physics and Astronomyinelastic neutron scatteringInelastic neutron scatteringSettore FIS/03 - Fisica Della MateriaMatrix (geology)Differential scanning calorimetryPhysical and Theoretical ChemistryPhysics::Atmospheric and Oceanic PhysicsCondensed matter physicsCalorimetry Differential Scanning[SDV.BBM.BS]Life Sciences [q-bio]/Biochemistry Molecular Biology/Structural Biology [q-bio.BM]ChemistrySolvationwater anomalieWaterSilicon DioxideSettore FIS/07 - Fisica Applicata(Beni Culturali Ambientali Biol.e Medicin)Cold Temperaturewater anomalies; differential scanning calorimetry; inelastic neutron scattering; liquid-liquid transitionInflection pointChemical physicsThermodynamicsBoson peakdifferential scanning calorimetryGelsPorosityIntensity (heat transfer)
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Recent changes in chironomid communities and hypolimnetic oxygen conditions relate to organic carbon in subarctic ecotonal lakes

2018

A key question in aquatic elemental cycling is related to the influence of bottom water oxygen conditions in regulating the burial and release of carbon under climate warming. In this study, we used head capsules of Chironomidae larvae to assess community and diversity change between the past (estimated as Pre-Industrial Period) and present and to reconstruct changes in hypolimnetic oxygen conditions from 30 subarctic ecotonal lakes (northeastern Lapland) using the top-bottom paleolimnological approach applying surface sediment (topmost 0-2 cm) and reference (4-5 cm) samples. Subsequently, we tested the findings against dissolved organic carbon (DOC) concentration of the sites. We found tha…

liuennut orgaaninen hiili010504 meteorology & atmospheric sciencesClimateCALIBRATION MODEL010501 environmental sciencesDOC01 natural sciencesPaleolimnologyFreshwater ecosystemFRESH-WATER ECOSYSTEMSDissolved organic carbonGREENHOUSE-GASWaste Management and DisposalTEMPERATUREhappikatoTotal organic carbonCLIMATE-CHANGEpaleolimnologyPollutionSubarctic climateAdaptation PhysiologicalpaleolimnologiaOceanographyBenthic zonedissolved oxygenHypolimnionEnvironmental MonitoringEnvironmental EngineeringClimate Changeta1171ChironomidaeBottom waterRECONSTRUCTIONSSUBFOSSIL CHIRONOMIDSEnvironmental ChemistryAnimals14. Life underwatersurviaissääsket1172 Environmental sciences0105 earth and related environmental sciencesMIDGES DIPTERA15. Life on landNUTRIENT DYNAMICSCarbontop-bottom approachOxygenLakesLapland13. Climate actionEnvironmental scienceta1181subarktinen vyöhykeSOUTHERN FINLANDScience of the Total Environment
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Possible Contribution of T-pattern Detection and Analysis to the Study of the Behavioral Correlates of Afferent Inhibition.

2020

A pivotal tenet in modern behavioral sciences is that the study of behavior, in its most intimate structure, necessarily deals with time and, for this reason, behavioral dynamics are not intuitively perceivable and/or detectable (Eibl-Eibesfeldt, 1970). In reality, the possibility to describe a given behavior in terms of its structural/temporal features makes available new and detailed information otherwise unavailable. The aim of the present paper is to discuss the possible application of T-pattern detection and analysis, i.e., a multivariate approach specifically developed to describe the temporal structure of behavior, to the study of an important and still scantly investigated issue, na…

long-latency afferent inhibitionGeneral Neurosciencemedicine.medical_treatmentT-pattern analysiNeurophysiologyT-pattern analysisSettore BIO/09 - Fisiologia030227 psychiatrylcsh:RC321-571Transcranial magnetic stimulationshort-latency afferent inhibition03 medical and health sciencesPattern detectionafferent inhibition0302 clinical medicineEditorialAfferentBehavioral dynamicstranscranial magnetic stimulationmedicineTPAPsychologyNeurosciencelcsh:Neurosciences. Biological psychiatry. Neuropsychiatry030217 neurology & neurosurgeryBrain sciences
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