Search results for "EMT"
showing 10 items of 413 documents
Quasi-isotropic 3-D resolution in two-photon scanning microscopy.
2009
One of the main challenges in three-dimensional microscopy is to overcome the lack of isotropy of the spatial resolution, which results from the axially-elongated shape of the point spread function. Such anisotropy gives rise to images in which significant axially-oriented structures of the sample are not resolved. In this paper we achieve an important improvement in z resolution in two-photon excitation microscopy through spatial modulation of the incident beam. Specifically, we demonstrate that the design and implementation of a simple shaded ring performs quasi-isotropic three-dimensional imaging and that the corresponding loss in luminosity can be easily compensated by most available fe…
Photodetachment of F− by short laser pulses. Comparison between experiments and numerical results
2009
Recently, angle-resolved photoelectron spectra have been measured by exposing negative F− ions to linearly or circularly polarized infrared femtosecond laser fields. We compare the experimental results with numerical calculations carried out in the framework of a Keldysh-type theory modified to account for both the time shape and the spatial inhomogeneity of the pulse. In order to account for the finite duration of the laser pulse, our results have been obtained through calculations of photodetachment probabilities. By using the saddle-point method it is possible to show that the transition amplitude may be written as a coherent sum of terms giving rise to interferences. This circumstance s…
Ultrafast and Energy-Efficient Quenching of Spin Order: Antiferromagnetism Beats Ferromagnetism
2017
By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material - metallic dysprosium - we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much more efficiently manipulated by optical excitation than its ferromagnetic counterpart. We assign the fast and extremely efficient process in the antiferromagnet to an interatomic transfer of angular momentum within the spin system. Our findings do not only reveal this angular momentum transfer channel effective in antiferromagnets and other magnetic structures with non-parallel spin alignment, they also point out a possible route towards energy-efficient …
Time- and energy resolved photoemission electron microscopy-imaging of photoelectron time-of-flight analysis by means of pulsed excitations
2010
Abstract The present work enlightens the developments in time- and energy resolved photoemission electron microscopy over the past few years. We describe basic principles of the technique and demonstrate different applications. An energy- and time-filtering photoemission electron microscopy (PEEM) for real-time spectroscopic imaging can be realized either by a retarding field or hemispherical energy analyzer or by using time-of-flight optics with a delay line detector. The latter method has the advantage of no data loss at all as all randomly incoming particles are measured not only by position but also by time. This is of particular interest for pump–probe experiments in the femtosecond an…
Absolute frequency measurements on the 2S→3S transition of lithium-6,7
2009
The frequencies of the 2S–3S two-photon transition for the stable lithium isotopes were measured by cavity-enhanced Doppler-free laser excitation that was controlled by a femtosecond frequency comb. The resulting values of 815 618 181.57(18) and 815 606 727.59(18) MHz, respectively, for 7Li and 6Li are in agreement with previous measurements but are more accurate by an order of magnitude. There is still a discrepancy of about 11.6 and 10.6 MHz from the latest theoretical values. This is comparable to the uncertainty in the theoretical calculations, while uncertainty in our experimental values is more than a hundred-fold smaller. More accurate theoretical calculation of the transition freque…
Hot electrons and nonlinear optical nanoantennas
2017
The large field enhancement generated at the surface of a resonant plasmonic nanoparticle, or optical antennas, is the key mechanism that eventually led to the development of nonlinear plasmonics [1-2]. While the resonance may boost the nonlinear yield of an adjacent structure or surrounding medium, it was soon realized that optical antennas possess nonlinear coefficients comparable or exceeding those of standard nonlinear optical materials [3]. We discuss here two nonlinear optical processes — incoherent multi-photon luminescence (MPL) and coherent second-harmonic generation (SHG) — emitted from gold rod optical antennas upon local illumination with a tightly focused femtosecond near-infra…
Evidence for metastable photo-induced superconductivity in K3C60
2021
Far and mid infrared optical pulses have been shown to induce non-equilibrium unconventional orders in complex materials, including photo-induced ferroelectricity in quantum paraelectrics, magnetic polarization in antiferromagnets and transient superconducting correlations in the normal state of cuprates and organic conductors. In the case of non-equilibrium superconductivity, femtosecond drives have generally resulted in electronic properties that disappear immediately after excitation, evidencing a state that lacks intrinsic rigidity. Here, we make use of a new optical device to drive metallic K$_3$C$_{60}$ with mid-infrared pulses of tunable duration, ranging between one picosecond and o…
Optical gratings induced by field-free alignment of molecules
2006
We analyze the alignment of molecules generated by a pair of crossed ultra-short pump pulses of different polarizations by a technique based on the induced time-dependent gratings. Parallel polarizations yield an intensity grating, while perpendicular polarizations induce a polarization grating. We show that both configurations can be interpreted at moderate intensity as an alignment induced by a single polarized pump pulse. The advantage of the perpendicular polarizations is to give a signal of alignment that is free from the plasma contribution. Experiments on femtosecond transient gratings with aligned molecules were performed in CO2 at room temperature in a static cell and at 30 K in a …
Optimization of field-free molecular alignment by phase-shaped laser pulses
2007
We theoretically demonstrate the optimization of field-free molecular alignment by phase-shaped femtosecond laser pulses. The effect is assessed in ${\mathrm{O}}_{2}$ at $T=60\phantom{\rule{0.3em}{0ex}}\mathrm{K}$ under realistic conditions of intensity and pulse shaping. The spectral laser phase is sampled through 128 control parameters and a self-learning evolutionary algorithm combined with a nonperturbative regime calculation is used in order to design the specific phase that maximizes the degree of alignment. The postpulse molecular alignment appears significantly enhanced compared to a Fourier-transform-limited pulse of same energy. The analysis of the target state reveals that the so…
Field-free molecular alignment of CO2 mixtures in presence of collisional relaxation
2008
The present work explores the extension of the concept of short-pulse-induced alignment to dissipative environments within quantum mechanical density matrix formalism (Liouville equation) from the weak to the strong field regime. This is illustrated within the example of the CO2 molecule in mixture with Ar and He, at room temperature, for which a steep decrease of the alignment is observed at moderate pressure because of the collisional relaxation. The field-free alignment is measured by a polarization technique where the degree of alignment is monitored in the time domain by measuring the resulting transient birefringence with a probe pulse Raman induced polarization spectroscopy (RIPS) Co…