Search results for "Enantioresolution"

showing 3 items of 3 documents

Modelling the enantioresolution capability of cellulose tris(3,5-dichlorophenylcarbamate) stationary phase in reversed phase conditions for neutral a…

2018

[EN] To the best of our knowledge, the prediction of the enantioresolution ability of polysaccharides-based stationary phases in liquid chromatography for structurally unrelated compounds has not been previously reported. In this study, structural information of neutral and basic compounds is used to model their enantioresolution levels obtained from an immobilised cellulose tris(3,5-dichlorophenylcarbamate) stationary phase in reversed phase conditions. Thirty-four structurally unrelated chiral drugs and pesticides, from seven families, are studied. Categorical enantioresolution levels (RsC, 0 = no baseline enantioresolution and 1 = baseline enantioresolution) are established from the expe…

Models MolecularTrisPhenylcarbamatesEnantioresolution modelling01 natural sciencesBiochemistryAnalytical Chemistrychemistry.chemical_compoundMolecular descriptorPhase (matter)Tris(35-dichlorophenylcarbamate)MoleculeLeast-Squares AnalysisPesticidesCelluloseCelluloseChromatography High Pressure LiquidReversed phase liquid chromatographyEnantioseparationsChromatography Reverse-PhasePrincipal Component AnalysisChromatography010405 organic chemistry010401 analytical chemistryOrganic ChemistryDiscriminant partial least squaresDiscriminant AnalysisStereoisomerismGeneral MedicineReversed-phase chromatography0104 chemical scienceschemistryStationary phaseAsymmetric carbonStationary phaseJournal of Chromatography A
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Optimization of a LC method for the enantioseparation of a non-competitive glutamate receptor antagonist, by experimental design methodology

2006

Abstract The aim of this work was to obtain the direct optical resolution of a new glutamate receptor antagonist (( p -chloro)1-aryl-6,7,-dimethoxy-1,2,3,4-tetrahydroisoquinoline, PS3), by liquid chromatography on Chiralcel ® OD column. A response surface methodology (RSM) was employed to optimize the enantiomeric separation of the racemate with the lowest number of experiments; in particular, a face-centred design (FCD) was applied to evaluate the influence of critical parameters on the experimental response. Furthermore, in order to find the best compromise between several responses, a multicriteria decision-making approach, the Derringer's desirability function, was successful to simulta…

Resolution (mass spectrometry)Clinical BiochemistryAnalytical chemistryPharmaceutical ScienceChiral liquid chromatography Enantioresolution Chiralcel® OD Tetrahydroisoquinoline derivative Face-centred design Desirability functionHigh-performance liquid chromatographyAnalytical Chemistrychemistry.chemical_compoundTetrahydroisoquinolinesDrug DiscoveryGlutamate receptor antagonistResponse surface methodologySpectroscopyChiral liquid chromatographyChromatographyMolecular StructureAntagonistChiralcel® ODStereoisomerismTetrahydroisoquinoline derivativeDesirability functionFace-centred designHexanechemistryModels ChemicalDesirability functionEnantiomerEnantioresolutionExcitatory Amino Acid AntagonistsChromatography Liquid
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Comparative modelling study on enantioresolution of structurally unrelated compounds with amylose-based chiral stationary phases in reversed phase li…

2020

[EN] Polysaccharide-based chiral stationary phases (CSPs) are the most used chiral selectors in HPLC. These CSPs can be used in normal, polar organic and aqueous-organic mobile phases. However, normal and polar organic mobile phases are not adequate for chiral separation of polar compounds, for the analysis of aqueous samples and for MS detection. In these situations, reversed phase conditions, without the usual non-volatile additives incompatible with MS detection, are preferable. Moreover, in most of the reported chiral chromatographic methods, retention is too large for routine work. In this paper, the chiral separation of 53 structurally unrelated compounds is studied using three commer…

Resolution (mass spectrometry)Reversed phase liquid hromatography010402 general chemistryMass spectrometry01 natural sciencesBiochemistryHigh-performance liquid chromatographyAmylose-based chiral stationary phasesMass SpectrometryAnalytical Chemistrychemistry.chemical_compoundAmylosePhase (matter)Least-Squares AnalysisAcetonitrileEnantioresolution modelling and descriptionChromatography High Pressure LiquidChromatography Reverse-PhaseAqueous solutionChromatography010401 analytical chemistryOrganic ChemistryDiscriminant partial least squaresStereoisomerismGeneral MedicineReversed-phase chromatography0104 chemical sciencesModels ChemicalchemistryFeature selectionRegression AnalysisAmyloseJournal of Chromatography A
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