Search results for "Far infrared"

Far infrared absorption by acoustic phonons in titanium dioxide nanopowders

2006

We report spectral features of far infrared electromagnetic radiation absorption in anatase TiO2 nanopowders which we attribute to absorption by acoustic phonon modes of nanoparticles. The frequency of peak excess absorption above the background level corresponds to the predicted frequency of the dipolar acoustic phonon from continuum elastic theory. The intensity of the absorption cannot be accounted for in a continuum elastic dielectric description of the nanoparticle material. Quantum mechanical scale dependent effects must be considered. The absorption cross section is estimated from a simple mechanical phenomenological model. The results are in plausible agreement with the absorption b…

Affordable, ultra-broadband coherent detection of terahertz pulses via CMOS-compatible solid-state devices

2017

We demonstrate the first fully solid-state technique for the coherent detection of ultra-broadband THz pulses (0.1-10 THz), relying on the electric-field-induced second-harmonic generation attained in integrated CMOS-compatible devices.

Spectral and morphological analysis of the remnant of Supernova 1987A with ALMA and ATCA

2014

We present a comprehensive spectral and morphological analysis of the remnant of Supernova (SN) 1987A with the Australia Telescope Compact Array (ATCA) and the Atacama Large Millimeter/submillimeter Array (ALMA). The non-thermal and thermal components of the radio emission are investigated in images from 94 to 672 GHz ($\lambda$ 3.2 mm to 450 $\mu$m), with the assistance of a high-resolution 44 GHz synchrotron template from the ATCA, and a dust template from ALMA observations at 672 GHz. An analysis of the emission distribution over the equatorial ring in images from 44 to 345 GHz highlights a gradual decrease of the east-to-west asymmetry ratio with frequency. We attribute this to the shor…

First analysis of the ν3+ν5 combination band of SF6 observed at Doppler-limited resolution and effective model for the ν3+ν5-ν5 hot band

2018

Abstract Sulfur hexafluoride is a greenhouse gas with a long lifetime in the atmosphere and an important tracer for air mass circulation atmospheric models. The IR spectrum of this heavy species, however, features many hot bands at room temperature (at which only 30% of the molecules lie in the ground vibrational state), especially those originating from the lowest, v 6 and v 5 = 1 vibrational states. Using a cryogenic long path cell with variable optical path length and temperatures regulated between 168 and 163 K, coupled to Synchrotron Radiation and a high resolution interferometer, Doppler-limited spectra of the very weak ν 3 + ν 5 band near 1450 cm−1 have been recorded. Low temperature…

Synchrotron-based Fourier transform spectra of the ν23 and ν24 IR bands of hexamethylenetetramine C6N4H12

2015

Abstract Hexamethylenetetramine (HMT), C6N4H12 is a spherical top with nine IR-active modes. Because of its relevance for astrophysics, we recorded the absorption spectra in the full range of its fundamental bands. In total, we detected eight fundamental bands and recently published the rotational analysis of the four most intense bands ( ν 19 , ν 20 , ν 21 , ν 22 ) located in the 1000–1500 cm−1 range as a support for astronomical searches (Pirali et al., 2014). While the CH stretch modes are unresolved broad features, in this article we report the analysis of the two remaining fundamental bands exhibiting rotationally resolved structures: ν 23 –GS and ν 24 –GS located at about 820 cm−1 and…

Four-Color Infrared Bolometer System for One-Meter Telescope

1978

As a part of the collaborative program between the University of Palermo and the Center for Astrophysics (HCO/SAO) a far infrared photometer has been designed, fabricated and tested by the Univsity of Palermo to be used as a focal plane instrument on the Center of Astrophysics/University of Arizona balloon-borne 102 cm telescope (Fazio et a1. 1974).

INVESTIGATION OF FAR-INFRARED SMITH-PURCELL RADIATION AT THE 3.41 MEV ELECTRON INJECTOR LINAC OF THE MAINZ MICROTRON MAMI

2006

Models, predictions, and experimental measurements of far-infrared NH3-laser dynamics and comparisons with the Lorenz-Haken model

1995

Dynamics of the intensity and optical field amplitude of a coherently pumped far-infrared NH3-laser are measured and characterized. The experimental findings in certain parameter ranges closely follow the dynamics of the Lorenz model and its generalization for laser systems. Similarities and some specific differences are found in geometrical or statistical characterizations of the attractors. The experimental results are also consistent with the results of a model of optically pumped three-level lasers which takes into account the presence of a multiplicity of velocity groups as well as three-level coherence effects. For a certain region in parameter space, this far more complex model with …

INSTABILITIES IN DOPPLER BROADENED OPTICALLY PUMPED FAR-INFRARED LASERS

1988

Recently Weiss and Brock observed Lorenz-type chaos in the 81.5μm emission from an optically-pumped 14NH3 laser1. The theoretical interpretation of the experimental results is an open question, however. In fact, the Lorenz-Haken model refers to incoherently pumped lasers with homogeneously-broadened two-level active media2. Models based on (at least) a three-level system are needed to describe optically-pumped lasers, whose dynamics is known to reduce to that of the Lorez-Haken model under certain limiting conditions3. But these conditions are not met in the 14NH3 laser, and indeed theoretical predictions of a model for this laser, which considered a homogeneously-broadened three-level acti…

Solid-state-biased coherent detection of ultra-broadband terahertz pulses

2017

Significant progress in nonlinear and ultrafast optics has recently opened new and exciting opportunities for terahertz (THz) science and technology, which require the development of reliable THz sources, detectors, and supporting devices. In this work, we demonstrate the first solid-state technique for the coherent detection of ultra-broadband THz pulses (0.1-10 THz), relying on the electric-field-induced second-harmonic generation in a thin layer of ultraviolet fused silica. The proposed CMOS-compatible devices, which can be realized with standard microfabrication techniques, allow us to perform ultra-broadband detection with a high dynamic range by employing probe laser powers and bias v…