Search results for "Ferro"

Mechanism for ultrafast electric-field driven skyrmion nucleation

2021

We show how a Dzyaloshinskii-Moriya interaction can be generated in an ultrathin metal film from a femtosecond pulse in electric field. This interaction does not require structural inversion-symmetry breaking, and its amplitude can be tuned depending on the amplitude of the field. We perform first-principles calculations to estimate the strength of the field-induced magnetoelectric coupling for ferromagnetic Fe, Co, and Ni, and antiferromagnetic Mn, as well as FePt and MnPt alloys. Last, using atomistic simulations, we demonstrate how an isolated antiferromagnetic skyrmion can be coherently nucleated from the collinear background by an ultrashort pulse in electric field on a hundred-femtose…

Epitaxial Films of Relaxor Ferroelectric PbMg1/3Nb2/3O3in Strong Electric Fields

2005

Epitaxial thin films of perovskite relaxor ferroelectric PbMg 1/3 Nb 2/3 O 3 were grown on MgO (001) substrates by pulsed laser deposition using La 0.5 Sr 0.5 CoO 3 bottom electrode layers. Dielectric response of the films was experimentally studied as a function of temperature and frequency in a broad range of amplitudes of ac electric field (to 10 MV/m) and magnitudes of dc electric field (to 50 MV/m). At small fields, a glass-like behavior was observed. With increasing magnitude of the dc field, an onset of a polar state was detected. The orientation of the polar clusters along the direction of the field and fluctuations of the direction of their dipole moments were suggested to determin…

Spontaneous Magnetization in Heterometallic NiFe-MOF-74 Microporous Magnets by Controlled Iron Doping

2017

We report the direct synthesis of mixed-metal NiFe-MOF-74 solids that display combination of porosity with ferrimagnetic ordering. Compared to the undoped Ni phase, controlled doping with Fe enables to modify intra and interchain magnetic interactions for the onset of spontaneous magnetization at temperatures fixed by the doping level. Synthesis of porous magnets remains somewhat elusive due to the difficulties in isolating foreseeable metal-organic architectures that combine small bridging linkers, for strong magnetic coupling, with polyaromatic connectors responsible for porosity. In turn, we demonstrate that metal doping is better fitted to modify the magnetism of Metal-Organic Framework…

Theoretical investigation of the platinum substrate influence on BaTiO 3 thin film polarisation

2019

Density functional theory calculations are performed to study the out-of-plane polarisation in BaTiO3 (BTO) thin films epitaxially grown on platinum. Prior to any polarisation calculation, the stability of the Pt(001)/BaTiO3(001) structure is thoroughly discussed. In particular, the nature of the Pt/BTO and BTO/vacuum interfaces is characterised. The growth of BTO is shown to start with a TiO2 layer while the nature of the surface termination does not broadly modify the stability. Therefore both upper terminations are considered when describing the ferroelectric behaviour in Pt/BTO interfaces. The geometric and electronic effects of the substrate on the polarisation are investigated. To iso…

An Ising ferromagnet with an antiferromagnetic surface layer: A simple model for magnetic surface reconstruction

1985

Simple cubic Ising lattices are studied by Monte Carlo simulation, using a thin film geometry (usually 40 atomic layers thick), with nearest neighbour ferromagnetic exchange J in the bulk and nearest neighbour antiferromagnetic interaction Js between surface spins. Applying a technique of preferential sampling in the surface layers, we investigate the ordering for a variety of values of JsJ and for various temperatures. For JsAF < Js < − 0.25J (where JsAF ≈ − 2.01J) ferromagnetic ordering occurs at a higher temperature than the antiferromagnetic surface ordering, while for − 0.25J < Js no antiferromagnetic long range order is possible. For Js < JsAF the surface transition occurs at a higher…

A neutron scattering study of the magnetic properties of PrSn3

1988

The intermetallic compound PrSn3 has been studied by elastic and inelastic neutron scattering. The paramagnetic phase shows overdamped crystal field excitations and an anisotropic distribution of the diffuse magnetic intensity. The dispersion relation of the excitations of the antiferromagnetic phase has been determined. The results are analyzed in terms of an anisotropic exchange coupling.

Influence of Structure Ordering, Defects and External Conditions on Properties of Ferroelectric Perovskites

2000

Results of comprehensive studies of the (A’A“)(B’B”)O3-ferroelectric perovskites are reported. Examined compositions include Pb1-xLax(Zr0.65Ti0.35)1-x/4O3(PLZT), PbSc0.5Nb0.5O3(PSN), PbSc0.5Ta0.5O3(PST), and PMNT, PSNT and PLuNT pseudo-binary systems exhibiting pronounced dielectric, electrooptical, and electromechanical properties. Degree of ordering in the materials has been varied by chemical composition (modification, isomorphic ion substitution), by variation of technology (hot-pressing, specific thermal treatment, thin films), and by irradiation of different kind and intensity (γ-rays, electrons, neutrons).

Dielectric relaxation of space charges and polarons in ferroelectric perovskites

2001

Abstract In all ferroelectric perovskites, intentionally introduced or “unwanted” point defects do play a role in the dielectric spectra and in the conductivity. Above room temperature, space charge relaxation at the electrodes interfaces are observed. This can be of interest in the context of the nowadays applications of ferroelectric thin films. At liquid helium temperatures much more localised dielectric relaxation occurs. Special emphasis will be brought on SrTiO3 which has received renewed interest at the beginning of the nineties and for which a wealth of reliable experimental data are available. Considering that a gradual freezing of polarized objects is occurring at low temperatures…

Magnetic Skyrmions: Current-Induced Skyrmion Generation through Morphological Thermal Transitions in Chiral Ferromagnetic Heterostructures (Adv. Mate…

2018

Electronic, structural, and magnetic properties of the half-metallic ferromagnetic quaternary Heusler compounds CoFeMnZ(Z=Al, Ga, Si, Ge)

2011

The quaternary intermetallic Heusler compounds CoFeMn$Z$ ($Z=\text{Al}$, Ga, Si, or Ge) with $1:1:1:1$ stoichiometry were predicted to exhibit half-metallic ferromagnetism by ab initio electronic structure calculations. The compounds were synthesized using an arc-melting technique and the crystal structures were analyzed using x-ray powder diffraction. The electronic properties were investigated using hard x-ray photoelectron spectroscopy. The low-temperature magnetic moments, as determined from magnetization measurements, follow the Slater-Pauling rule, confirming the proposed high spin polarizations. All compounds have high Curie temperatures, allowing for applications at room temperature…