Search results for "Francium"
showing 10 items of 17 documents
The Collinear Resonance Ionization Spectroscopy (CRIS) experimental setup at CERN-ISOLDE
2012
The CRIS setup at CERN-ISOLDE is a laser spectroscopy experiment dedicated to the high-resolution study of the spin, hyperfine structure and isotope shift of radioactive nuclei with low production rates (a few per second). It combines the Doppler-free resolution of the in-flight collinear geometry with the high detection efficiency of resonant ionisation. A recent commissioning campaign has demonstrated a 1% experimental efficiency, and as low as a 0.001% non-resonant ionisation. The current status of the experiment and its recent achievements with beams of francium isotopes are reported. The first identified systematic effects are discussed. publisher: Elsevier articletitle: The Collinear …
Beta-decay measurements of neutron-rich thallium, lead, and bismuth by means of resonant laser ionisation
2004
Abstract Neutron-rich thallium, lead, and bismuth isotopes were investigated at the ISOLDE facility. After mass separation and resonant laser ionisation of the produced activity, new spectroscopic data were obtained for 215,218 Bi and 215 Pb. An attempt to reach heavy thallium had to be abandoned because of a strong francium component in the beam that gave rise to a neutron background through (α,n) reactions on the aluminium walls of the experimental chamber.
Quadrupole moment of Fr 203
2017
The spectroscopic electric quadrupole moment of the neutron-deficient francium isotope 203Fr was measured by using high-resolution collinear resonance ionization spectroscopy (CRIS) at the CERN Isotope Separation On-Line Device (ISOLDE)facility. A remeasurement of the 207Fr quadrupole momentwas also performed, resulting in a departure from the established literature value. A sudden increase in magnitude of the 203Fr quadrupole moment, with respect to the general trend in the region, points to an onset of static deformation at N =116 in the 87Fr isotopic chain. Calculation of the static and total deformation parameters show that the increase in static deformation only cannot account for the o…
CRIS: A new method in isomeric beam production
2013
The Collinear Resonance Ionization Spectroscopy (CRIS) experiment at ISOLDE, CERN, uses laser radiation to stepwise excite and ionize an atomic beam for the purpose of ultra-sensitive detection of rare isotopes, and hyperfine-structure measurements. The technique also offers the ability to purify an ion beam that is heavily contaminated with radioactive isobars, including the ground state of an isotope from its isomer, allowing decay spectroscopy on nuclear isomeric states to be performed. The isomeric ion beam is selected by resonantly exciting one of its hyperfine structure levels, and subsequently ionizing it. This selectively ionized beam is deflected to a decay spectroscopy station (DS…
Laser spectroscopy of francium isotopes at the borders of the region of reflection asymmetry
2014
The magnetic dipole moments and changes in mean-square charge radii of the neutron-rich $^{218m,219,229,231}\text{Fr}$ isotopes were measured with the newly-installed Collinear Resonance Ionization Spectroscopy (CRIS) beam line at ISOLDE, CERN, probing the $7s~^{2}S_{1/2}$ to $8p~^{2}P_{3/2}$ atomic transition. The $\delta\langle r^{2}\rangle^{A,221}$ values for $^{218m,219}\text{Fr}$ and $^{229,231}\text{Fr}$ follow the observed increasing slope of the charge radii beyond $N~=~126$. The charge radii odd-even staggering in this neutron-rich region is discussed, showing that $^{220}\text{Fr}$ has a weakly inverted odd-even staggering while $^{228}\text{Fr}$ has normal staggering. This sugges…
Evaluation of the magnetic moment ofRa213
1991
The hyperfine field at the nucleus of singly ionized radium has been investigated using the relativistic linked-cluster many-body-perturbation-theory procedure, including the effects of distributed charge and magnetization over the nucleus. The total hyperfine field of 1239 T, when combined with the experimentally observed hyperfine constant for $^{213}\mathrm{Ra}^{+}$, yields a nuclear moment of 0.607(12)${\mathrm{\ensuremath{\mu}}}_{\mathit{N}}$, in excellent agreement with the experimentally observed moment of 0.6133(18)${\mathrm{\ensuremath{\mu}}}_{\mathit{N}}$ from Zeeman measurements. Our investigation leads to exchange core-polarization and correlation contributions of 14% and 13%, r…
Nuclear moments and charge radii of neutron-deficient francium isotopes and isomers
2015
Collinear laser fluorescence spectroscopy has been performed on the ground and isomeric states of 204,206Fr in order to determine their spins, nuclear moments, and changes in mean-squared charge radii. A new experimental technique has been developed as part of this work which much enhances the data collection rate while maintaining the high resolution. This has permitted the extension of this study to the two isomeric states in each nucleus. The investigation of nuclear g factors and mean-squared charge radii indicates that the neutron-deficient Fr isotopes lie in a transitional region from spherical towards more collective structures. peerReviewed
Combined high-resolution laser spectroscopy and nuclear decay spectroscopy for the study of the low-lying states inFr206,At202, andBi198
2016
High-resolution laser spectroscopy was performed on $^{206}\mathrm{Fr}$ with the collinear resonance ionization spectroscopy (CRIS) experiment at CERN-ISOLDE. The hyperfine structure and isotope shift of the ground, first isomeric and second isomeric states were measured. The hyperfine components were unambiguously assigned to each nuclear state by means of laser-assisted nuclear decay spectroscopy. The branching ratios in the $\ensuremath{\alpha}$ decay of $^{206}\mathrm{Fr}$ and $^{202}\mathrm{At}$ were also measured for the first time with isomerically purified beams. The extracted hindrance factors allow determination of the spin of the ground, first isomeric, and second isomeric states…
Mass Determination of Francium and Radium Isotopes by a Penning Trap Mass Spectrometer
1992
Abstract A tandem Penning trap mass spectrometer is used for mass measurement of radioactive isotopes produced at the on-line isotope separator ISOLDE/CERN. The mass is determined directly and with high accuracy by measuring the cyclotron frequency of the stored ions. Measurements were performed on 209 210 211 212 221 222Fr and 226 230Ra. A resolving power of 5 × 105 was used and an accuracy of 1·8 × 10−7 has been achieved.
Use of a Continuous Wave Laser and Pockels Cell for Sensitive High-Resolution Collinear Resonance Ionization Spectroscopy
2015
New technical developments have led to a 2 orders of magnitude improvement of the resolution of the collinear resonance ionization spectroscopy (CRIS) experiment at ISOLDE, CERN, without sacrificing the high efficiency of the CRIS technique. Experimental linewidths of 20(1) MHz were obtained on radioactive beams of francium, allowing us for the first time to determine the electric quadrupole moment of the short lived [t1/2=22.0(5) ms]219Fr Qs=−1.21(2) eb, which would not have been possible without the advantages offered by the new method. This method relies on a continuous-wave laser and an external Pockels cell to produce narrow-band light pulses, required to reach the high resolution in t…