Search results for "Ground State"

showing 10 items of 928 documents

Strongly Red-Emissive Molecular Ruby [Cr(bpmp)2]3+ Surpasses [Ru(bpy)3]2+

2021

Gaining chemical control over the thermodynamics and kinetics of photoexcited states is paramount to an efficient and sustainable utilization of photoactive transition metal complexes in a plethora of technologies. In contrast to energies of charge transfer states described by spatially separated orbitals, the energies of spin-flip states cannot straightforwardly be predicted as Pauli repulsion and the nephelauxetic effect play key roles. Guided by multireference quantum chemical calculations, we report a novel highly luminescent spin-flip emitter with a quantum chemically predicted blue-shifted luminescence. The spin-flip emission band of the chromium complex [Cr(bpmp)2]3+ (bpmp = 2,6-bis(…

Nephelauxetic effectPhotoluminescenceQuenching (fluorescence)ChemistryQuantum yieldGeneral ChemistryPhotochemistryBiochemistryCatalysisColloid and Surface ChemistryAtomic orbitalExcited stateLuminescenceGround stateJournal of the American Chemical Society
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Disentangling decaying isomers and searching for signatures of collective excitations in β decay

2019

6 pags., 3 figs., 1 tab. -- 27th International Nuclear Physics Conference (INPC2019) 29 July - 2 August 2019, Glasgow, UK

Neutron-rich nucleiHistoryIsotope-separator-on-lineGround statePenning trapspektroskopiaBeta decay01 natural sciencesEducationNuclear physics0103 physical sciencesGamma-ray spectroscopy010306 general physicsNuclear ExperimentPhysicsPygmy dipole resonances010308 nuclear & particles physicsGamma rays[PHYS.PHYS.PHYS-GEN-PH]Physics [physics]/Physics [physics]/General Physics [physics.gen-ph]3. Good healthComputer Science ApplicationsQuasiparticleIsomeric stateFísica nuclearydinfysiikkaGamma ray spectrometersCollective excitations
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Role of triaxiality in the ground-state shape of neutron-rich Yb, Hf, W, Os and Pt isotopes

2009

The evolution of the ground-state shape of several isotopes of Yb, Hf, W, Os and Pt along the triaxial landscape is analyzed using the self-consistent Hartree-Fock-Bogoliubov approximation. Two well-reputed interactions (Gogny D1S and Skyrme SLy4) have been used in the study in order to assess to which extent the results are independent of the details of the effective interaction. A large number of even-even nuclei, with neutron numbers from N = 110 up to N = 122, have been considered, covering in this way a vast extension of the nuclear landscape where signatures of oblate-prolate shape transitions have already manifested both theoretically and experimentally.

Nuclear Theory (nucl-th)Nuclear physicsPhysicsNuclear and High Energy PhysicsIsotopeNuclear TheoryNuclear TheoryShape evolutionFOS: Physical sciencesOrder (group theory)NeutronGogny Energy Density FunctionalGround state
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Collectivity in ${}^{\mathrm{196,198}}$Pb isotopes probed in Coulomb-excitation experiments at REX-ISOLDE

2017

The neutron-deficient ${}^{\mathrm{196,198}}$Pb isotopes have been studied in Coulomb-excitation experiments employing the Miniball γ-ray spectrometer and radioactive ion beams from the REX-ISOLDE post-accelerator at CERN. The reduced transition probabilities of the first excited 2+ states in 196Pb and 198Pb nuclei have been measured for the first time. Values of $B(E2)={18.2}_{-4.1}^{+4.8}$ W.u. and $B(E2)={13.1}_{-3.5}^{+4.9}$ W.u., were obtained, respectively. The experiment sheds light on the development of collectivity when moving from the regime governed by the generalised seniority scheme to a region, where intruding structures, associated with different deformed shapes, start to com…

Nuclear and High Energy Physics3106Coulomb excitationREX-ISOLDESHELLHadronElementary particleCoulomb excitation[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]114 Physical sciences01 natural sciencesNuclear physicsSHAPE COEXISTENCE0103 physical sciencesSCATTERINGradioactive ion beamsACCELERATED RADIOACTIVE BEAMS010306 general physicsPhysicsPb isotopesNUCLEI010308 nuclear & particles physicsBaryongamma-ray spectroscopyEXCITED-STATESCoulomb-excitation experimentExcited stateAtomic physicsGround stateNucleongamma transitions and level energiesEnergy (signal processing)
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Mass and half-life measurements of neutron-deficient iodine isotopes

2020

The European physical journal / A 56(5), 143 (2020). doi:10.1140/epja/s10050-020-00153-5

Nuclear and High Energy PhysicsALPHA-DECAYSEPARATORMass spectrometry01 natural sciences530Ionjodi0103 physical sciencesNuclear fusionNeutronddc:530010306 general physicsNuclear ExperimentPhysicsisotoopitIsotope010308 nuclear & particles physicsPERFORMANCESPECTROMETRYQuadrupoleFRS; PROJECTILEAlpha decayAtomic physicsydinfysiikkaGround stateSYSTEM
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Time integral and time differential Mössbauer measurements on [57Co/Mn(bipy)3](PF6)2

1994

The Mossbauer emission spectra of nucleogenic iron(II) complexes with a low spin (LS) ground state show two metastable iron(II) high spin (HS) states at low temperatures. In order to identify these metastable HS states, the compound [57Co/Mn(bipyridine)3](PF6)2 has been studied by time differential Mossbauer emission spectroscopy (TDMES) and optical lifetime measurements of excited electronic states in the corresponding Fe-doped Mn compound. The lifetime of one of the HS states of the nucleogenic iron(II) determined by TDMES has been measured to be the same as the lifetime of the laser-excited iron(II) electronic state.

Nuclear and High Energy PhysicsAstrophysics::High Energy Astrophysical PhenomenaAnalytical chemistryComputer Science::Computational GeometryCondensed Matter PhysicsAtomic and Molecular Physics and OpticsBipyridinechemistry.chemical_compoundchemistryNucleogenicMetastabilityMössbauer spectroscopyCondensed Matter::Strongly Correlated ElectronsEmission spectrumPhysical and Theoretical ChemistryGround stateSpectroscopySpin (physics)Hyperfine Interactions
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Lifetime measurements in99Sr and100Zr

1989

The lifetime of the first excited state in99Sr has been determined by the delayed γ-γ coincidence method. The value of t/2=0.58(9) ns corresponds to a deformation parameter s=0.38(4). The deduced value confirms the previously proposed ν[411]3/2 Nilsson assignment for the99Sr ground state. In addition, lifetime values for the 2+ (t1/2=0.40(8) ns) and 0+ (t1/2=5.36(23) ns) states in100Zr are obtained, which deviate from older measurements and indicate a larger deformation of s=0.39(4).

Nuclear and High Energy PhysicsChemistryExcited stateValue (computer science)Nuclear fusionDeformation (meteorology)Atomic physicsGround stateCoincidenceZeitschrift f�r Physik A Atomic Nuclei
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How to measure nuclear ground-state properties in simple systems such as 11Li or U91+?

2008

Abstract Atomic spectroscopy yields key information on properties of ground and isomeric states via a determination of the hyperfine structure and isotope shift. In order to deduce precise nuclear moments and charge radii, the electromagnetic fields produced by the electrons at the site of the nucleus must be known with high accuracy. This is presently possible only for simple systems with very few electrons. This contribution describes two scenarios for such experiments: the determination of the charge radius of the neutron-rich isotopes 8,9Li and of the halo nucleus 11Li at the on-line isotope separators at GSI and TRIUMF and the Highly charged Ion TRAP (HITRAP) facility which is under co…

Nuclear and High Energy PhysicsChemistryNuclear TheoryHighly charged ionHalo nucleusElectronAtomic spectroscopyIonNuclear physicsCharge radiusPhysics::Atomic PhysicsAtomic physicsNuclear ExperimentGround stateInstrumentationHyperfine structureNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Towards on-line production of N=Z94Ag at IGISOL

2008

Abstract A future study of the ground state and low-lying isomeric states of 94 Ag and 96 Ag at the Ion Guide Isotope Separator On-Line (IGISOL) facility, University of Jyvaskyla, requires the development of a low-energy beam of neutron-deficient silver. In order to attain the highest possible extraction efficiencies the coupling of a hot cavity graphite catcher device to the IGISOL mass-separator is planned. A heavy-ion fusion-evaporation reaction will produce the silver recoils which will be captured in the graphite catcher. Resonant laser ionization techniques will be applied to efficiently and selectively ionize the evaporated silver atoms. A simulation program has been written to study…

Nuclear and High Energy PhysicsChemistrySeparator (oil production)LaserIonlaw.inventionNuclear physicslawIonizationPhysics::Atomic and Molecular ClustersThermal emittancePhysics::Atomic PhysicsGraphiteAtomic physicsNuclear ExperimentGround stateInstrumentationBeam (structure)Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Properties of the ground-state baryons in chiral perturbation theory

2010

15th High Energy Physics International Conference on Quantum Chromodynamics. Montpellier (FRANCE). JUN 28-JUL 02, 2010

Nuclear and High Energy PhysicsChiral perturbation theoryNuclear TheoryHigh Energy Physics::LatticeNuclear TheoryLattice field theoryExtrapolationFOS: Physical sciencesAstrophysics::Cosmology and Extragalactic AstrophysicsHigh Energy Physics - ExperimentNuclear Theory (nucl-th)High Energy Physics - Experiment (hep-ex)Theoretical physicsHigh Energy Physics - Phenomenology (hep-ph)High Energy Physics - LatticeChiral perturbation theoryNuclear Experiment (nucl-ex)Nuclear ExperimentNuclear ExperimentPhysicsHigh Energy Physics - Lattice (hep-lat)High Energy Physics::PhenomenologyHyperonLattice QCDAtomic and Molecular Physics and OpticsBaryonHigh Energy Physics - PhenomenologyCoupling (physics)Baryon structureGround stateNuclear Physics B - Proceedings Supplements
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