Search results for "Helium"
showing 10 items of 1689 documents
Helium Behavior in Oxide Nuclear Fuels: First Principles Modeling
2010
UO2 and (U,Pu)O2 solid solutions (the so-called MOX) nowadays are used as commercial nuclear fuels in many countries. One of the safety issues during the storage of these fuels is related to their self-irradiation that produces and accumulates point defects and helium therein. We present density functional theory (DFT) calculations for UO2, PuO2 and MOX containing He atoms in octahedral interstitial positions. In particular, we calculated basic MOX properties and He incorporation energies as functions of Pu concentration within the spin-polarized, generalized gradient approximation (GGA) DFT calculations. We also included the on-site electron correlation corrections using the Hubbard model …
Status report of the Jyvaskyla ion guide isotope separator on-line facility
1997
The ion guide isotope separator facility IGISOL of the University of Jyvaskyla has been moved to the new K-130 heavy ion cyclotron laboratory. The totally reconstructed facility is described in detail. The primary beams and targets, helium pumping, separator beam line construction and separator beam diagnostics are discussed. The spectroscopy stations are introduced with illustrative examples from the research program, including beta-delayed proton and neutron spectroscopy, gamma-ray spectroscopy with and without arrays, conversion electron spectroscopy, collinear laser spectroscopy and nuclear level lifetime spectroscopy.
Cryogenic helium as stopping medium for high-energy ions
2008
We have investigated the survival and transport efficiency of Ra-219 ions emitted by a Ra-223 source in high-density cryogenic helium gas, with ionisation of the gas induced by a proton beam. The combined efficiency of ion survival and transport by an applied electric field was measured as a function of ionisation rate density for electric fields up to 160 V/cm and for three temperature and density combinations: 77 K, 0.18 mg/cm(3), 10 K, 0.18 mg/cm(3) and 10 K, 0.54 mg/cm(3). At low beam intensity or high electric field, an efficiency of 30%, is obtained, confirming earlier results. A sharp drop in efficiency is observed at a "threshold" ionisation rate density which increases with the squ…
High-precision measurement of the electron spin g factor of trapped atomic nitrogen in the endohedral fullerene N@C60
2018
Abstract The electronic g factor carries highly useful information about the electronic structure of a paramagnetic species, such as spin-orbit coupling and dia- or paramagnetic (de-)shielding due to local fields of surrounding electron pairs. However, in many cases, a near “spin-only” case is observed, in particular for light elements, necessitating accurate and precise measurement of the g factors. Such measurement is typically impeded by a “chicken and egg situation”: internal or external reference standards are used for relative comparison of electron paramagnetic resonance (EPR) Larmor frequencies. However, the g factor of the standard itself usually is subject to a significant uncerta…
RILIS-ionized mercury and tellurium beams at ISOLDE CERN
2017
This paper presents the results of ionization scheme development for application at the ISOLDE Resonance Ionization Laser Ion Source (RILIS). Two new ionization schemes for mercury are presented: a three-step three-resonance ionization scheme, ionizing via an excitation to a Rydberg level and a three-step two-resonance ionization scheme, with a non-resonant final step to the ionization continuum that corresponded to a factor of four higher ionization efficiency. The efficiency of the optimal mercury ionization scheme was measured, together with the efficiency of a new three-step three resonance ionization scheme for tellurium. The efficiencies of the mercury and tellurium ionization schemes…
Energy spectrum of cosmic protons and helium nuclei by a hybrid measurement at 4300 m a.s.l.
2014
The energy spectrum of cosmic Hydrogen and Helium nuclei has been measured, below the so-called "knee", by using a hybrid experiment with a wide field-of-view Cherenkov telescope and the Resistive Plate Chamber (RPC) array of the ARGO-YBJ experiment at 4300 m above sea level. The Hydrogen and Helium nuclei have been well separated from other cosmic ray components by using a multi-parameter technique. A highly uniform energy resolution of about 25% is achieved throughout the whole energy range (100 TeV - 700 TeV). The observed energy spectrum is compatible with a single power law with index gamma=-2.63+/-0.06.
TRITIUM RELEASE CHARACTERISTICS OF NEUTRON-IRRADIATED REFERENCE BERYLLIUM PEBBLES FOR THE HELIUM COOLED PEBBLE BED (HCPB) BLANKET
2011
In this paper, we present results on tritium release from the beryllium pebbles irradiated for 294 full power days from 17 April 2003 to November 2004 to the neutron fluence of 1.5-2 × 1025 m-2 (E>...
Thin film growth into the ion track structures in polyimide by atomic layer deposition
2017
Abstract High-aspect ratio porous structures with controllable pore diameters and without a stiff substrate can be fabricated using the ion track technique. Atomic layer deposition is an ideal technique for depositing thin films and functional surfaces on complicated 3D structures due to the high conformality of the films. In this work, we studied Al2O3 and TiO2 films grown by ALD on pristine polyimide (Kapton HN) membranes as well as polyimide membranes etched in sodium hypochlorite (NaOCl) and boric acid (BO3) solution by means of RBS, PIXE, SEM-EDX and helium ion microcopy (HIM). The focus was on the first ALD growth cycles. The areal density of Al2O3 film in the 400 cycle sample was det…
On the Secondary Discharge of an Atmospheric-Pressure Pulsed DBD in He with Impurities
2008
The secondary discharge was induced at the end of a slow-falling voltage flank, when a semisine monopolar pulse voltage excites the dielectric-barrier discharge. Formation and properties of the secondary discharge with respect to different dielectric materials such as glass, ceramic, and polyethylene theraphtalate were studied. The tunable diode laser absorption spectrometry (at 777.194 nm) was used to analyze the time-space distribution of the density of the atomic oxygen in metastable state (35S2 rarr 35P3) in addition to both discharge voltage and discharge current versus time. The secondary discharge is always formed, and its amplitude, as well as the amplitude of the main discharge, de…
Thermo-mechanical testing of Li-ceramic for the helium cooled pebble bed (HCPB) breeding blanket
2004
The helium cooled pebble bed (HCPB) Test blanket module (TBM) for the DEMO Reactor foresees the utilization of lithiate ceramics as breeder in form of pebble beds. The pebbles are organized in several layers alternatively stacked among couples of cooling plates (CP). ENEA has launched an experimental programme for the out-of-pile thermo-mechanical testing of mock-ups simulating a portion of the HCPB-TBM. The programme foresees the fabrication and testing of different mock-ups, to be tested in the HE-FUS3 facility at ENEA Brasimone. The paper describes the HELICHETTA III campaign carried-out in 2003. In particular, the test section layout, the pebble filling procedure, the experimental set-u…