Search results for "IONIZATION"

Resonance lonization mass spectroscopy with a pulsed thermal atomic beam

1987

Resonance ionization mass spectroscopy (RIMS) and pulsed-laser induced desorption (PLID) have been combined for ultrasensitive detection and spectroscopy of very small samples of refractive elements. The method has been tested and applied to laser spectroscopy of 5×109 atoms (1.5 pg) of195Au (T1/2= 183d) implanted at the ISOLDE online mass separator with 60 keV into graphite. A pulsed thermal atomic beam was formed by laser desorption with a 10 ns Nd∶Yag laser pulse. Subsequently the atoms were photoionized in a three-colour, three-step resonant excitation to an autoionizing state. The selectivity was enhanced by a time-of-flight measurement of the photo ions. In resonance, one ion was dete…

2019

The atomic spectrum of neutral promethium has been studied extensively by laser resonance ionization spectroscopy. We report on more than 1000 atomic transitions in the blue and near infrared spectral ranges, most of them between high excited energy levels. As Rydberg convergences could not be assigned unambiguously in the dense spectrum at high excitation energies, the first ionization potential (IP) was determined via field ionization of weakly bound states within a static electric field. By applying the saddle-point model, a value of ${\mathrm{IP}}_{(\mathrm{Pm})}=45\phantom{\rule{0.16em}{0ex}}020.8(3)\phantom{\rule{4pt}{0ex}}{\mathrm{cm}}^{\ensuremath{-}1} [5.58188(4)\phantom{\rule{0.16…

Femtoscopy with identified charged pions in proton-lead collisions at sNN=5.02 TeV with ATLAS

2017

Bose-Einstein correlations between identified charged pions are measured for $p$+Pb collisions at $\sqrt{s_{\mathrm{NN}}}=5.02$ TeV using data recorded by the ATLAS detector at the LHC corresponding to a total integrated luminosity of $28$ $\mathrm{nb}^{-1}$. Pions are identified using ionization energy loss measured in the pixel detector. Two-particle correlation functions and the extracted source radii are presented as a function of collision centrality as well as the average transverse momentum ($k_{\mathrm{T}}$) and rapidity ($y^{\star}_{\pi\pi}$) of the pair. Pairs are selected with a rapidity $-2 < y^{\star}_{\pi\pi} < 1$ and with an average transverse momentum $0.1 < k_{\mathrm{T}} <…

Resonant ionization spectroscopy of autoionizing Rydberg states in cobalt and redetermination of its ionization potential

2017

Multi-step resonance ionization spectroscopy of cobalt has been performed using a hot-cavity laser ion source and three Ti:Sapphire lasers. The photoionization spectra revealed members of five new autoionizing Rydberg series that originate from three different lower levels of 3d74s5s h4F9/2, 3d74s4d f4G11/2, and 3d74s4d f4H13/2 and converge to the first four excited states of singly ionized Co. The analyses of the Rydberg series yield 63564.689 �� 0.036 cm-1 as the first ionization potential of Co, which is an order of magnitude more accurate than the previous estimation. Using a three-step resonance ionization scheme that employs an autoinizing Rydberg state in the last transition, we obta…

Strong-field physics in the molecular frame

2019

XXI International Conference on Ultrafast Phenomena 2018, UP 2018, Hamburg, Germany, 15 Jul 2018 - 20 Jul 2018; The European physical journal / Web of Conferences 205, 07002 (2019). doi:10.1051/epjconf/201920507002

Spectroscopy of Very Hot Plasma in Non-flaring Parts of a Solar Limb Active Region: Spatial and Temporal Properties

2017

In this work we investigate the thermal structure of an off-limb active region (AR) in various non-flaring areas, as it provides key information on the way these structures are heated. In particular, we concentrate on the very hot component (&gt;3 MK) as it is a crucial element to distinguish between different heating mechanisms. We present an analysis using Fe and Ca emission lines from both the Solar Ultraviolet Measurement of Emitted Radiation (SUMER) on board the Solar and Heliospheric Observatory (SOHO) and the EUV Imaging Spectrometer (EIS) on board Hinode. A data set covering all ionization stages from Fe X to Fe XIX has been used for the thermal analysis (both differential emission …

Ionization potential of Al6 and Al7 as a function of temperature

1999

The temperature-depence of the ionization potential of Al6 and Al7 clusters is studied by using ab initio molecular dynamics. The threshold regions of theoretical photoionization efficiency curves are obtained from the calculated ionization potential distributions by integration and the determined ionization potentials are compared with the experimental ones. Two important effects, which complicate the determination of ionization potential from photoionization efficiency curves, are observed: the thermal tail effect and the isomerization. Also a link between the adiabatic ionization potential and the threshold of the photoionization efficiency curve is discussed. In the case of Al7, this of…

The general expression for the transition amplitude of two-photon ionization of atomic hydrogen

2003

Two-photon ionization of atomic hydrogen with an excess photon is revisited. The non-relativistic dipole approximation and Coulomb Green function (CGF) formalism are applied. Using the CGF Sturmian expansion straightforwardly, one gets the radial transition amplitude in the form of an infinite sum over Gauss hypergeometric functions which are polynomials. It is convergent if all intermediate states are in the discrete spectrum. In the case of two-photon ionization with an excess photon, when photoionization is also possible, intermediate states are in the continuum. We performed the explicit summation over intermediate states and got a simple general expression for the radial transition amp…

Multiphoton-ionization transition amplitudes and the Keldysh approximation.

1989

The Keldysh approximation to treat the multiphoton ionization of atoms is reconsidered. It is shown that, if one consistently uses the hypothesis under which the approximation should be valid (essentially, that of a weak, short-range binding potential), a Keldysh-like term results as an approximation to the first term of a uniformly convergent series in powers of the binding potential. No cancellation occurs when higher-order terms are taken into account. This result allows one to consider the Keldysh approximation as a well-defined theoretical model, without implying, however, that it is adequate to describe multiphoton ionization of real atoms.

Line Identification of Atomic and Ionic Spectra of Holmium in the Near-UV. II. Spectra of Ho ii and Ho iii

2017

Fourier Transform spectra of holmium (Ho) in the UV spectral range from 31,530 to 25,000 cm−1 (317 to 400 nm) have been investigated, particularly focusing on the ionic lines. The distinction between the different degrees of ionization (I, II, and III) is based on differences in signal-to-noise ratios from two Ho spectra, which have been measured with different buffer gases, i.e., neon and argon. Based on 106 known Ho ii and 126 known Ho iii energy levels, 97 lines could be classified as transitions of singly ionized Ho and 9 lines could be classified as transitions of doubly ionized Ho. Of the 97 Ho ii lines, 6 have not been listed in the extant literature. Another 215 lines have been assi…